Immobilized iron Schiff base histidine complexes on Al-MCM-41 and zeolite Y as catalyst for oxidation of cycloalkanes
Source abstract
Abstract
Iron complexes of N-salicylidene-L-histidine with or without bipyridine ligand immobilized on Al-MCM41 and zeolite Y designated as Fe(sal-L-his)(bipy)complex/ Al-MCM-41 or Fe(sal-L-his)complex/Al-MCM-41 and Fe (sal-L-his)(bpy)complex/YorFe(sal-L-his)complex/Yrespectively, were prepared and characterized by X-ray powder diffraction (XRD), FT-IR, N2 adsorption/desorption and chemical analysis techniques. Fe(sal-L-his)/Al-MCM-41 and Fe(sal-L-his)(bipy)complex/Al-MCM-41 were found to successfully catalyze the oxidation of cyclohexane, methyl cyclohexane, cyclooctane and adamantane with H2O2. The oxidation results and promising catalytic behavior of Fe(salL-his)(bipy)complex/Al-MCM-41 for oxidation of cyclooctane with 90 % conversion and excellent selectivity toward the formation of cyclooctanone will be discussed in this presentation.
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Research context
OpenAlex topics: Metal-Catalyzed Oxygenation Mechanisms · Oxidative Organic Chemistry Reactions · Porphyrin and Phthalocyanine Chemistry
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
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