Reversible Photoinduced Luminescence Modulation from Nanospheres Containing CdSe/ZnS Quantum Dots and Photochromic Diarylethene

Anastasia A. Scherbovich; Sergei A. Maskevich; Pavel V. Karpach; Gennady T. Vasilyuk; Vitali I. Stsiapura; Olga V. Venidiktova; Anton O. Ayt; Valery A. Barachevsky; Artur A. Khuzin; Airat R. Tuktarov; Mikhail V. Artemyev

doi:10.1021/acs.jpcc.0c06651

journal article·2020-12-10

Reversible Photoinduced Luminescence Modulation from Nanospheres Containing CdSe/ZnS Quantum Dots and Photochromic Diarylethene

Anastasia A. Scherbovich, Sergei A. Maskevich, Pavel V. Karpach, Gennady T. Vasilyuk, Vitali I. Stsiapura, Olga V. Venidiktova, Anton O. Ayt, Valery A. Barachevsky, Artur A. Khuzin, Airat R. Tuktarov, Mikhail V. Artemyev

The Journal of Physical Chemistry C· Volume 124· Issue 49

Publisher page

Source abstract

Abstract

We prepared for the first time photoactive colloidal nanospheres consisting of hydrophobic CdSe/ZnS core–shell quantum dots encapsulated in an amphiphilic PMAT polymeric shell containing photochromic diarylethene DAE1 with stoichiometry of ∼6 dye molecules per single quantum dot. The UV-induced photoisomerization of DAE1 molecules results in the partial quenching of the quantum dot emission due to FRET from the quantum dot to DAE1 photoisomer with its absorption band spectrally overlapped with the quantum dot emission. The modulation of the quantum dot emission is reversible under cyclic UV–vis-induced open–closed photoisomerization of DAE1.

Source: openalex_inverted_index · Quality: baseline

Research context

Polymers Nanomaterials

OpenAlex topics: Photochromic and Fluorescence Chemistry · Advanced Photocatalysis Techniques · Nanoplatforms for cancer theranostics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Research Institute for Physical Chemical Problems of the Belarusian State University, 220030 Minsk, Belarus

Belarusian State University, ISEI BSU, 220070 Minsk, Belarus

Yanka Kupala State University of Grodno, Grodno, Belarus

Photochemistry Center, Federal Scientific Research Centre “Crystallography and Photonics”, RAS, Moscow, Russia

Interdepartmental Center of Analytical Research of the Russian Academy of Sciences, Moscow, Russia

Institute of Petrochemistry and Catalysis, RAS, Ufa, Russia

Funding

Russian Foundation for Basic Research · Belarusian Republican Foundation for Fundamental Research · Ministry of Science and Higher Education of the Russian Federation

References (45)

Show source-provided references

1. 10.1002/adma.20120152110.1002/adma.201201521 ↗

2. 10.1039/b920377j10.1039/b920377j ↗

3. 10.1016/j.ccr.2009.12.03610.1016/j.ccr.2009.12.036 ↗

4. 10.1002/ejoc.20080124410.1002/ejoc.200801244 ↗

5. 10.1021/jp052440o10.1021/jp052440o ↗

6. Feringa B. L. · 200110.1002/3527600329 ↗

7. 10.1021/cr500249p10.1021/cr500249p ↗

8. 10.1021/nn103243c10.1021/nn103243c ↗

9. 10.1039/b804151m10.1039/b804151m ↗

10. 10.1039/b809952a10.1039/b809952a ↗

11. 10.1016/j.ica.2006.07.02910.1016/j.ica.2006.07.029 ↗

12. 10.1039/B618510J10.1039/B618510J ↗

13. 10.1021/la061801410.1021/la0618014 ↗

14. 10.1021/nl015512610.1021/nl0155126 ↗

15. 10.1021/nl025596y10.1021/nl025596y ↗

16. 10.1016/j.optmat.2013.03.00510.1016/j.optmat.2013.03.005 ↗

17. 10.1002/chem.20160468810.1002/chem.201604688 ↗

18. 10.1134/S106377451802002510.1134/S1063774518020025 ↗

19. 10.1134/S106377451905005510.1134/S1063774519050055 ↗

20. 10.1021/acs.langmuir.5b0460210.1021/acs.langmuir.5b04602 ↗

21. 10.1007/s11172-010-0203-310.1007/s11172-010-0203-3 ↗

22. 10.1002/hc.2033410.1002/hc.20334 ↗

23. 10.1007/s10895-019-02455-410.1007/s10895-019-02455-4 ↗

24. 10.1038/protex.2012.04210.1038/protex.2012.042 ↗

25. 10.1039/an983080106710.1039/an9830801067 ↗

26. 10.1021/jp805822c10.1021/jp805822c ↗

27. 10.1021/cm034081k10.1021/cm034081k ↗

28. Lakowicz J. R. · 2013

29. 10.1146/annurev.bi.40.070171.00050310.1146/annurev.bi.40.070171.000503 ↗

30. 10.1016/j.dyepig.2014.02.01310.1016/j.dyepig.2014.02.013 ↗

31. 10.1073/pnas.080931610610.1073/pnas.0809316106 ↗

32. 10.1021/jp003088b10.1021/jp003088b ↗

33. 10.1021/nn200268910.1021/nn2002689 ↗

34. 10.1021/jp055795g10.1021/jp055795g ↗

35. 10.1002/cphc.20120105910.1002/cphc.201201059 ↗

36. Von Borczyskowski C. · 2017 · 14310.1201/9781315364636-4 ↗

37. 10.1063/1.157092310.1063/1.1570923 ↗

38. 10.1103/PhysRevB.74.08532010.1103/PhysRevB.74.085320 ↗

39. 10.1021/acs.jpcc.8b0454410.1021/acs.jpcc.8b04544 ↗

40. 10.1103/PhysRevLett.88.13740110.1103/PhysRevLett.88.137401 ↗

41. 10.1021/nn502347310.1021/nn5023473 ↗

42. 10.1021/nl060483q10.1021/nl060483q ↗

43. 10.1016/S0006-3495(87)83264-210.1016/S0006-3495(87)83264-2 ↗

44. Brochon J.-C. · Methods Enzymol. · 1994 · 240 · 26210.1016/S0076-6879(94)40052-0 ↗

45. 10.1007/s10812-010-9314-810.1007/s10812-010-9314-8 ↗