journal article·2017-11-22

Highly Efficient Regeneration of Deactivated Au/C Catalyst for 4-Nitrophenol Reduction

Mingbo Ruan, Ping Song, Jing Liu, Erling Li, Weilin Xu

The Journal of Physical Chemistry C· Volume 121· Issue 46
Publisher page

Abstract

In the present work, we proposed an effective method to regenerate sintered gold catalyst by improving the dispersion of gold nanoparticles. With the liquid oxychlorination reaction, a sintered carbon-supported gold (Au/C) nanocatalyst was effectively regenerated by improving the redispersion of Au nanoparticles with additional carbon support. The Au-catalyzed model reaction between 4-nitrophenol and sodium borohydride (NaBH 4 ) indicates that the apparent activity of the optimal Au/C regenerated (Au 0.45 wt %) exceeds that of the initial fresh Au/C (Au 1 wt %), making Au utilization tripled and potentially sustainable for their extensive application in industry.
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Research context

OpenAlex topics: Nanomaterials for catalytic reactions · Catalytic Processes in Materials Science · Copper-based nanomaterials and applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Jilin Province Key Laboratory of Low Carbon Chemical Power, Chinese Academy of Science, 5625 Renmin Street, Changchun 130022, P. R. China

Graduate University of Chinese Academy of Science, Beijing, 100049, China

Funding

Ministry of Science and Technology of the People's Republic of China · National Natural Science Foundation of China · K. C. Wong Education Fundation · Youth Foundation of Jilin Province · Science and Technology Innovation Foundation for Talents Cultivation of Jilin Province

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