journal article·2014-10-16Open access

Combined Experimental and Theoretical Study of Efficient and Ultrafast Energy Transfer in a Molecular Dyad

Mariangela Di Donato, Alessandro Iagatti, Andrea Lapini, Paolo Foggi, Stefano Cicchi, Luisa Lascialfari, Stefano Fedeli, Stefano Caprasecca, Benedetta Mennucci

The Journal of Physical Chemistry C· Volume 118· Issue 41

Abstract

We have characterized the dynamics and the efficiency of electronic energy transfer (EET) in a newly synthesized molecular dyad, composed of a styryl-pyridinium donor and a BODIPY acceptor. The kinetics of the process has been studied with femtosecond transient absorption spectroscopy in different solvents. In all the analyzed media EET is quantitative and very fast, as we find that almost 70% of the overall excitation energy is transferred from the donor to the acceptor on a subpicosecond time scale. The experimental measurements have been supported by a theoretical analysis; the electronic couplings between the donor and acceptor moieties have been calculated at the (TD)DFT level and complemented by a conformational analysis of the full dyad. The computed energy transfer times are in good agreement with the experimental values; this allowed us to verify the correctness of the Förster equation, demonstrating that, although EET in the examined system occurs on an ultrafast time scale, the approximations introduced in the case of the weak coupling regime remain valid.
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Research context

OpenAlex topics: Photochemistry and Electron Transfer Studies · Spectroscopy and Quantum Chemical Studies · Porphyrin and Phthalocyanine Chemistry

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

LENS (European Laboratory for Non Linear Spectroscopy) via N. Carrara 1, 50019 Sesto Fiorentino (FI), Italy

Dipartimento di Chimica “Ugo Schiff”, Universita’ di Firenze, via della Lastruccia 13, 50019 Sesto Fiorentino (FI), Italy

INO (Istituto Nazionale di Ottica), Largo Fermi 6, 50125 Firenze, Italy

Dipartimento di Chimica, Università di Perugia, via Elce di Sotto 8, 06123 Perugia, Italy

Dipartimento di Chimica e Chimica Industriale, Università di Pisa, via Risorgimento 35, I-56126 Pisa, Italy

Funding

European Research Council · Ministero dell'Istruzione, dell'Università e della Ricerca

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