journal article·2017-05

Single-source-precursor derived RGO/CNTs-SiCN ceramic nanocomposite with ultra-high electromagnetic shielding effectiveness

Xingmin Liu, Zhaoju Yu, Ryo Ishikawa, Lingqi Chen, Xiaofei Liu, Xiaowei Yin, Yuichi Ikuhara, Ralf Riedel

Acta Materialia· Volume 130
Publisher page

Abstract

Abstract For the first time, single-source-precursors (SSPs) were synthesized through chemical modification of a commercial poly(methylvinyl)silazane with chemically bonded graphene oxide and carbon nanotube hybrids (GO/CNTs). After pyrolysis of warm-pressed and consolidated SSP-powders at 1000 °C in Ar, monolithic SiCN ceramic nanocomposites modified with in-situ thermally reduced GO/CNTs, namely RGO/CNTs-SiCN, were successfully obtained. The SSP-derived nanocomposite exhibits significantly enhanced dielectric properties if compared with that of a physically-blended-precursor derived reference material. Moreover, the SSP-derived RGO/CNTs-SiCN composite containing 15.0 wt% GO/CNTs in the feed possesses an electromagnetic shielding effectiveness of 67.2 dB with a sample thickness of 2.00 mm, which is the highest value among all the reported graphene-based composites with comparable thickness.
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Research context

OpenAlex topics: Electromagnetic wave absorption materials · Dielectric materials and actuators · Structural Behavior of Reinforced Concrete

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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