journal article·2009-03

Enhancing BWR proliferation resistance fuel with minor actinides

Gray S. Chang

Journal of Nuclear Materials· Volume 385· Issue 1
Publisher page

Abstract

Abstract To reduce spent fuel for storage and enhance the proliferation resistance for the intermediate-term, there are two major approaches (a) increase the discharged spent fuel burnup in the advanced light water reactor- LWR (Gen-III Plus), which not only can reduce the spent fuel for storage, but also increase the 238 Pu isotopes ratio to enhance the proliferation resistance, and (b) use of transuranic nuclides ( 237 Np and 241 Am) in the high burnup fuel, which can drastically increase the proliferation resistance isotope ratio of 238 Pu/Pu. For future advanced nuclear systems, minor actinides (MA) are viewed more as a resource to be recycled, and transmuted to less hazardous and possibly more useful forms, rather than simply disposed of as a waste stream in an expensive repository facility. As a result, MAs play a much larger part in the design of advanced systems and fuel cycles, not only as additional sources of useful energy, but also as direct contributors to the reactivity control of the systems into which they are incorporated. In the study, a typical boiling water reactor (BWR) fuel unit lattice cell model with UO 2 fuel pins will be used to investigate the effectiveness of minor actinide reduction approach (MARA) for enhancing proliferation resistance and improving the fuel cycle performance in the intermediate-term goal for future nuclear energy systems. To account for the water coolant density variation from the bottom (0.76 g/cm 3 ) to the top (0.35 g/cm 3 ) of the core, the axial coolant channel and fuel pin were divided to 24 nodes. The MA transmutation characteristics at different elevations were compared and their impact on neutronics criticality discussed. The concept of MARA, which involves the use of transuranic nuclides ( 237 Np and/or 241 Am), significantly increases the 238 Pu/Pu ratio for proliferation resistance, as well as serves as a burnable absorber to hold-down the initial excess reactivity. It is believed that MARA can play an important role in atoms for peace and the intermediate-term of nuclear energy reconnaissance.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Nuclear reactor physics and engineering · Nuclear Materials and Properties · Fusion materials and technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (7)

Show source-provided references
1. Mark · Sci. Glob. Security · 1993 · 4 · 11110.1080/08929889308426394 ↗
2. M. Saito, Advanced Core Concepts with Enhanced Proliferation Resistance by Transmutation of Minor Actinides, in: Proceedings of GLOBAL 2005, Tsukuba, Japan, October 9–13, 2005, Paper No. 172.
3. T. Goorley, J. Bull, F. Brown, et al., Release of MCNP5_RSICC_1.30, MCNP Monte Carlo Team X-5, LA-UR-04-4519, Los Alamos National Laboratory, November 2004.
4. Croff · Nucl. Technol. · 1983 · 62 · 33510.13182/NT83-1 ↗
5. Chang · Nucl. Technol. · 2000 · 129 · 32610.13182/NT00-A3065 ↗
6. National Academy of Sciences Committee on International Security and Arms, Management and Disposition of Excess Weapons Plutonium, National Academy Press, 1994.
7. Kessler · Nucl. Sci. Eng. · 2007 · 155 · 5310.13182/NSE07-A2644 ↗