journal article·2012-12Open access

Post-irradiation analysis of the tantalum container of an ISOLDE LBE target

E. Noah, V. Boutellier, R. Brütsch, R. Catherall, D. Gavillet, J. Krbanjevic, H.P. Linder, M. Martin, J. Neuhausen, D. Schumann, T. Stora, L. Zanini

Journal of Nuclear Materials· Volume 431· Issue 1-3

Abstract

CERN-ISOLDE operates a range of oxides, carbides, refractory metal foils and liquid metal targets for the production of radioactive ion beams. Following irradiation with a pulsed beam of 1 GeV and 1.4 GeV protons at temperatures reaching 600 degrees C, the tantalum container of a liquid lead bismuth eutectic (LBE) target was examined. A thin layer of Pb/Bi was observed on the inner surface of the container. A sample of the surface prepared using the focused ion beam technique was investigated using SEM and EDX. Results show a higher concentration of bismuth at the interface with tantalum and micron-sized cracks in the tantalum filled with LBE. Implications of these results for the lifetime of the target container which has been known to fail under pulsed beam operation are discussed. (C) 2011 Elsevier B.V. All rights reserved.
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Research context

OpenAlex topics: Nuclear Physics and Applications · Nuclear reactor physics and engineering · Radiation Therapy and Dosimetry

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References (15)

Show source-provided references
1. Lettry · Nucl. Instrum. Methods Phys. Res. Sect. B · 2003 · 204 · 25110.1016/S0168-583X(02)01919-5 ↗
2. L. Zanini et al., Volatile elements production rates in a 1.4-GeV proton-irradiated molten lead-bismuth target, in: R.C. Haight et al. (Eds.), International Conference on Nuclear Data for Science and Technology, AIP Conference Proceedings, vol. 769, Melville, New York, 2005, pp. 1525.10.1063/1.1945295 ↗
3. Y. Tall et al. (Eds.), Proceedings of the International Conference on Nuclear Data for Science and Technology, Nice, 2007, pp. 1069.
4. L. Zanini et al., Post-irradiation analysis of a LBE-filled ta target irradiated at ISOLDE, in: Proceedings of TCADS Conference “Technology and Components of Accelerator-Driven Systems”, Karlsruhe, 2010 .
5. Noah · Nucl Instrum Methods Phys Res Sect B · 2008 · 266 · 430410.1016/j.nimb.2008.05.051 ↗
6. G. Battistoni et al., The FLUKA code: description and benchmarking, in: M. Albrow, R. Raja (Eds.), Proceedings of the Hadronic Shower Simulation Workshop 2006, Fermilab 6–8 September 2006, AIP Conference Proceeding, vol. 896, 2007, pp. 31–49.10.1063/1.2720455 ↗
7. A. Fassò et al., Fluka: a multi-particle transport code, CERN-2005-10, INFN/TC_05/11, SLAC-R-773, 2005.
8. Ohno · J. Nucl. Sci. Tech. · 2005 · 42 · 59310.1080/18811248.2004.9726426 ↗
9. Landolt-Börnstein, Numerical data and functional relationships in science and technology, new series, in: O. Madelung (Ed.), Group IV: Macroscopic and Technical Properties of Matter, vol. 5, Phase Equilibria, Crystallographic and Thermodynamic Data of Binary Alloys, Springer; Berlin, 1991.
10. J. Neuhausen, Report on Semi-Empirical Modeling of Thermodynamical Data for the Assessment of the Solubility and Chemical Behavior of Nuclear Reaction and Corrosion Products in a liquid Lead-Bismuth Spallation Target, Deliverable D4.32, DM4 DEMETRA, EUROTRANS.
11. J. Neuhausen et al., Ann. Rep. Lab. of Radio- and Environ. Chemistry, Uni. Bern & PSI, 2010, pp. 34–37.
12. J. Neuhausen et al., Proceedings of DAE-BRNS Symposium on Nuclear and Radiochemistry NUCAR-2011, Visakhapatnam, India, 2011.
13. Miura · Appl. Radiat. Isot. · 2004 · 61 · 130710.1016/j.apradiso.2004.02.023 ↗
14. E. Noah et al., Driver beam-led EURISOL target design constraints, EPAC08. CERN-AB-2008-052, in: Eleventh European Particle Accelerator Conference, Genoa, Italy, 2008 (MOPC090).
15. J.C. Cornell (Ed.), Final Report of the EURISOL Design Study, Ganil, BP 55027, 14076 Caen cedex 5, France, 2009.