journal article·2026-02Open access

Nanosecond laser ablation modeling of silicon and tungsten as support activity for LIBS diagnostic

Stefano Cipelli, Arshad Hussain, Giorgio Dilecce, Paolo Francesco Ambrico, Domenico Aceto, Anna Cremona, Irene Casiraghi, Olga De Pascale, Laura Laguardia, Matteo Pedroni, Daria Ricci, Dario Ripamonti, Jimmy Scionti, Andrea Uccello

Abstract

• 2D thermal finite element model for nanosecond laser ablation. • Plasma shielding implemented via exponential attenuation factor. • Tungsten and silicon targets irradiated by Nd:YAG laser in vacuum conditions. • Model validated comparing ablated volume, depth and cater diameter. Laser-Induced Breakdown Spectroscopy (LIBS) analyzes the optical emission of a laser-induced plasma to determine the elemental or isotopic composition of a material. In nuclear fusion research, LIBS is a promising diagnostic for remote monitoring of Plasma-Facing Components (PFCs). Accurate interpretation of LIBS measurements, especially for depth profiling and fuel retention studies, requires the knowledge of ablation rate and laser-induced thermal effects. This work presents a two-dimensional thermal model, developed using COMSOL Multiphysics, to simulate nanosecond laser ablation of tungsten, a fusion-relevant metal, and silicon, selected for its different thermophysical properties. The model solves the heat conduction equation considering temperature-dependent material properties, phase change, latent heat consumption, and plasma plume shielding included via an exponential attenuation factor. Material removal is implemented through a mesh deformation velocity dependent on the assumed ablation regime. Model validation was performed by comparing computations with laser ablation experiments in vacuum, using a 10 ns Nd:YAG laser. Ablation craters were characterized by optical microscopy, mechanical profilometry, and Scanning Electron Microscopy (SEM). For tungsten, normal evaporation was considered to describe ablation for 0.4 − 2 mJ pulse energy ( ∼ 4 − 20 J / c m 2 considering central crater); for silicon phase explosion dominated at 4 − 20 mJ ( ∼ 25 − 60 J / c m 2 ). The model reproduced ablated volume, depth, and crater diameter, obtaining relative discrepancies on depth resolution prediction around 20 %. These results demonstrate the potential of a physics-based model to predict LIBS crater features, supporting parameter optimization and aiding interpretation of depth profiling and fuel retention measurements.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Laser-induced spectroscopy and plasma · Laser Material Processing Techniques · Laser-Plasma Interactions and Diagnostics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (39)

Show source-provided references
1. Plasma–wall interaction, a key issue on the way to a steady state burning fusion device10.1088/0031-8949/2006/T123/004 ↗
2. A review of the LIBS analysis for the plasma-facing components diagnostics10.1016/j.jnucmat.2020.152417 ↗
3. Detection of deuterium retention by LIBS at different background pressures
4. In-situ LIBS and NRA deuterium retention study in porous WO and compact w coatings loaded by magnum-PSI10.1016/j.fusengdes.2021.112403 ↗
5. Calibration-free analysis of a tungsten-based target for diagnostics of relevant fusion materials comparing picosecond and nanosecond LIBS
6. An upgraded LIBS system on linear plasma device PSI-2 for in situ diagnostics of plasma-facing materials10.1016/j.fusengdes.2018.11.044 ↗
7. Development of a LIBS system for in situ surface measurements during plasma exposure in PISCES-A10.1063/1.5034349 ↗
8. LIBS measurements inside the FTU vessel mock-up by using a robotic arm10.1016/j.fusengdes.2020.111685 ↗
9. Dynamic deuterium retention properties of tungsten measured using laser-induced breakdown spectroscopy10.1088/1741-4326/ac26ef ↗
10. Monitoring of tritium and impurities in the first wall of fusion devices using a LIBS based diagnostic10.1088/1741-4326/ac31d6 ↗
11. COMSOL AB, COMSOL Multiphysics® v6.1, COMSOL AB, Stockholm, Sweden, 2023a. https://www.comsol.com.
12. COMSOL AB, Heat Transfer Module User’s Guide, COMSOL AB, Stockholm, Sweden, v6.1 edition, 2023b. Available at https://doc.comsol.com/6.1/doc/com.comsol.help.heat/HeatTransferModuleUsersGuide.pdf.
13. Pulsed laser ablation of solids: transition from normal vaporization to phase explosion10.1007/s003390000686 ↗
14. Plasma-wall interaction impact of the ITER re-baseline10.1016/j.nme.2024.101854 ↗
15. Thermal model for nanosecond laser ablation of alumina10.1016/j.ceramint.2015.01.106 ↗
16. Temperature rise of silicon due to absorption of permeable pulse laser
17. Differences in nanosecond laser ablation and deposition of tungsten, boron, and WB2/B composite due to optical properties
18. Galasso · 2017
19. Non-equilibrium phase change in metal induced by nanosecond pulsed laser irradiation10.1115/1.1445792 ↗
20. The interplay between laser focusing conditions, expansion dynamics, ablation mechanisms, and emission intensity in ultrafast laser-produced plasmas10.1063/5.0069732 ↗
21. Simulation of bi-material nano-second laser ablation
22. Laser-induced thermal processes: heat transfer, generation of stresses, melting and solidification, vaporization, and phase explosion
23. Bäuerle · 2013
24. Numerical simulation and experimental study on picosecond laser ablation of stainless steel10.1016/j.optlastec.2020.106150 ↗
25. Thermal model of pulsed laser ablation under the conditions of formation and heating of a radiation-absorbing plasma10.1070/QE1999v029n05ABEH001503 ↗
26. Characteristics of glow-discharge LIBS in a rarefied environment10.1088/1361-6587/ae0cfe ↗
27. Libs depth profiling of be-containing samples with different gaseous impurity concentrations
28. Investigation of laser ablation features of molybdenum bulk for picosecond laser-based techniques in fusion devices10.1016/j.fusengdes.2019.111379 ↗
29. Response of fusion plasma-facing materials to nanosecond pulses of extreme ultraviolet radiation10.1017/S0263034618000332 ↗
30. Analytical expressions for thermophysical properties of solid and liquid tungsten relevant for fusion applications10.1016/j.nme.2017.08.002 ↗
31. Corrected values for boiling points and enthalpies of vaporization of elements in handbooks10.1021/je1011086 ↗
32. On the critical point of tungsten10.1023/A:1019873110953 ↗
33. Ablation characteristics of tungsten with ultra-short laser pulses10.1063/5.0222073 ↗
34. Lide · 1993
35. Nanosecond pulsed laser ablation of silicon-finite element simulation and experimental validation10.1088/1361-6439/ab208b ↗
36. De Podesta · 2020
37. Theoretical models and qualitative interpretations of fs laser material processing10.2961/jlmn.2007.01.0014 ↗
38. Thermal modeling and experimental study of infrared nanosecond laser ablation of silicon10.1063/1.3271413 ↗
39. Short-term retention in metallic PFCs: modelling in view of mass spectrometry and LIBS10.1088/1402-4896/ac43d6 ↗