Investigation of aerosols released at high temperature from nuclear reactor core models

Abstract Two experiments were performed to simulate severe reactor accident with air ingress into the hot reactor core. The model bundles contained nine PWR type fuel rods. Their cladding was pre-oxidised by argon–oxygen (test 1) and steam (test 2). The released aerosol was measured continuously by laser particle counters. Morphology and elemental composition of the aerosol particles were studied on samples collected by impactors and quartz filters. The highest aerosol release was detected at the steepest rise of the bundle temperature. A second increase of the aerosol release appeared at the cooling down period. Because of the higher maximum temperature at test 2 about two orders of magnitude more uranium was released than in test 1. The highest emission was found for tin at test 1 and for zirconium and iron at test 2.