journal article·2020-09Open access

Modeling and simulation of oxygen transport in high burnup LWR fuel

Srdjan Simunovic, Theodore M. Besmann, Emily Moore, Max Poschmann, Markus H.A. Piro, Kevin T. Clarno, Jake W. McMurray, William A. Wieselquist

Abstract

Abstract We have developed a formulation for oxygen transport in uranium dioxide nuclear fuel that accounts for the effects of irradiation. The overall simulation combines the evolving isotopic composition, thermochemistry, and oxygen transport in irradiated fuel. The driving forces for oxygen transport are computed from local thermodynamic equilibrium calculations and account for the effects of temperature gradients and composition, including fission products. The proposed method provides a mechanism for including complex thermodynamic models of nuclear fuel in modeling of mass redistribution, and alleviates difficulties associated with the common thermodiffusion formulation. The transport model has been implemented within the nuclear fuel performance code BISON utilizing the thermochemistry code Thermochimica, with burnup calculations provided by the ORIGEN isotopic transmutation code.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Nuclear Materials and Properties · Nuclear reactor physics and engineering · Radioactive element chemistry and processing

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