journal article·2017-04

Phase characteristics of rare earth elements in metallic fuel for a sodium-cooled fast reactor by injection casting

Seoung Woo Kuk, Ki Hwan Kim, Jong Hwan Kim, Hoon Song, Seok Jin Oh, Jeong-Yong Park, Chan Bock Lee, Young-Sang Youn, Jong-Yun Kim

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Abstract

Abstract Uranium-zirconium-rare earth (U-Zr-RE) fuel slugs for a sodium-cooled fast reactor were manufactured using a modified injection casting method, and investigated with respect to their uniformity, distribution, composition, and phase behavior according to RE content. Nd, Ce, Pr, and La were chosen as four representative lanthanide elements because they are considered to be major RE components of fuel ingots after pyroprocessing. Immiscible layers were found on the top layers of the melt-residue commensurate with higher fuel slug RE content. Scanning electron microscopy-energy-dispersive X-ray spectroscopy (SEM-EDS) data showed that RE elements in the melt-residue were distributed uniformly throughout the fuel slugs. RE element agglomeration did not contaminate the fuel slugs but strongly affected the RE content of the slugs.
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Research context

OpenAlex topics: Nuclear Materials and Properties · Nuclear reactor physics and engineering · Molten salt chemistry and electrochemical processes

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