journal article·2022-08

The effect of pressure-promoted thermal rejuvenation on the fracture energy of metallic glasses

Hong Li, Cheng-Gang Jin, Zhen-Dong Sha

Publisher page

Abstract

Despite that the pressure-promoted thermal rejuvenation is a promising remedy for the plasticity enhancement of metallic glasses (MGs), there has been so far little studies of the effect of rejuvenation on the fracture toughness of MGs. Herein, molecular dynamic simulations are performed to study the influence of annealing pressure ( Pa) on the fracture energy ( G) of rejuvenated MGs. Our results manifest that the G increases at first and then decreases with Pa, showing a two-stage behavior. The increase of G is attributed to the improved plasticity but marginal change of strength, while the decrease of G is caused by the significant reduction of strength. Another key finding is that the improved plasticity arises from the more homogeneous activation of shear transformation zones due to its lower activation energy in the high-energy rejuvenated state. The present study establishes the influence of Pa on G based on the internal structure analyses.
Source: expertdata · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Metallic Glasses and Amorphous Alloys · Glass properties and applications · Material Dynamics and Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (67)

Show source-provided references
1. A brief overview of bulk metallic glasses10.1038/asiamat.2011.30 ↗
2. Bulk metallic glasses: at the cutting edge of metals research10.1557/mrs2007.121 ↗
3. Recent development and application products of bulk glassy alloys10.1016/j.actamat.2010.11.027 ↗
4. Structural evolution and strength change of a metallic glass at different temperatures10.1038/srep30876 ↗
5. Process, structure, property and applications of metallic glasses10.3934/matersci.2016.3.1022 ↗
6. Energy landscape picture of overaging and rejuvenation in a sheared glass10.1103/PhysRevLett.93.255501 ↗
7. Atomistic Simulation of Aging and Rejuvenation in Glasses10.1103/PhysRevLett.84.1471 ↗
8. Reversible transition of deformation mode by structural rejuvenation and relaxation in bulk metallic glass10.1063/1.4753998 ↗
9. Structural relaxation and rejuvenation in a metallic glass induced by shot-peening10.1080/09500830903337919 ↗
10. Relaxation processes and physical aging in metallic glasses10.1088/1361-648X/aa9964 ↗
11. Thermomechanical processing of metallic glasses: extending the range of the glassy state10.1038/natrevmats.2016.39 ↗
12. Processing of bulk metallic glass10.1002/adma.200902776 ↗
13. Structural relaxation in Pd-Cu-Ni-P metallic glasses10.1016/j.msea.2003.10.253 ↗
14. Thermal rejuvenation of a heterogeneous metallic glass10.1016/j.jnoncrysol.2018.05.038 ↗
15. Rejuvenation and plasticization of metallic glass by deep cryogenic cycling treatment10.1016/j.intermet.2017.11.015 ↗
16. Rejuvenation of metallic glasses by non-affine thermal strain10.1038/nature14674 ↗
17. Unveiling a new type of ultradense anomalous metallic glass with improved strength and ductility through a high-pressure heat treatment10.1038/s41427-019-0175-1 ↗
18. Embrittlement of Zr-based bulk metallic glasses10.1016/j.actamat.2009.04.016 ↗
19. Recovery of less relaxed state in Zr-Al-Ni-Cu bulk metallic glass annealed above glass transition temperature10.1063/1.4835076 ↗
20. Effect of ion irradiation on tensile ductility, strength and fictive temperature in metallic glass nanowires10.1016/j.actamat.2014.04.002 ↗
21. Structural evolution of nanoscale metallic glasses during high-pressure torsion: a molecular dynamics analysis10.1038/srep36627 ↗
22. Structural rejuvenation in bulk metallic glasses10.1016/j.actamat.2014.12.020 ↗
23. Ductile bulk metallic glasses produced through designed heterogeneities10.1016/j.scriptamat.2011.07.039 ↗
24. Atomistic understanding of deformation-induced heterogeneities in wire drawing and their effects on the tensile ductility of metallic glass wires10.1016/j.jallcom.2019.06.268 ↗
25. Contribution of cryogenic thermal cycling to the atomic dynamics in a La-based bulk metallic glass with different initial states10.1063/5.0005566 ↗
26. The effect of cryogenic thermal cycling on aging, rejuvenation, and mechanical properties of metallic glasses10.1016/j.jnoncrysol.2018.09.041 ↗
27. Metallic glasses: cryogenic rejuvenation10.1038/nmat4394 ↗
28. Improving plasticity of the Zr46Cu46Al8 bulk metallic glass via thermal rejuvenation10.1016/j.scib.2018.04.021 ↗
29. On cryothermal cycling as a method for inducing structural changes in metallic glasses10.1038/s41427-018-0019-4 ↗
30. Thermal rejuvenation in metallic glasses10.1080/14686996.2017.1280369 ↗
31. Controlled rejuvenation of amorphous metals with thermal processing10.1038/srep10545 ↗
32. Thermal annealing of shear bands in deformed metallic glasses: recovery mechanisms in Cu64Zr36 studied by molecular dynamics simulations10.1016/j.actamat.2011.07.063 ↗
33. Energy storage in metallic glasses via flash annealing10.1002/adfm.201805385 ↗
34. Rejuvenation through plastic deformation of a La-based metallic glass measured by fast-scanning calorimetry
35. Tailored hardening of ZrCuAl bulk metallic glass induced by 2D gradient rejuvenation10.1038/s41427-020-0233-8 ↗
36. Prediction of pressure-promoted thermal rejuvenation in metallic glasses10.1038/npjcompumats.2016.13 ↗
37. Mechanical behavior of metallic glasses with pressure-promoted thermal rejuvenation10.1016/j.jallcom.2020.156597 ↗
38. Thermal-pressure effects on energy state of metallic glass Cu50Zr5010.1016/j.commatsci.2018.09.018 ↗
39. High pressure quenched glasses: unique structures and properties10.1038/s41598-020-66418-7 ↗
40. Pressure induced liquid-to-liquid transition in Zr-based supercooled melts and pressure quenched glasses10.1038/s41598-017-06890-w ↗
41. The effect of thermal cycling on the fracture toughness of metallic glasses10.1016/j.actamat.2019.11.046 ↗
42. Pressure effect of glass transition temperature in Zr46.8Ti8.2Cu7.5Ni10Be27.5 bulk metallic glass10.1063/1.1675937 ↗
43. The fracture toughness of bulk metallic glasses10.1007/s11837-010-0052-4 ↗
44. Intrinsic and extrinsic toughening of metallic glasses10.1016/j.scriptamat.2005.10.010 ↗
45. Fracture toughness, fracture morphology, and crack-tip plastic zone of a Zr-based bulk amorphous alloy10.1007/s11661-001-1032-7 ↗
46. Toughness, extrinsic effects and Poisson's ratio of bulk metallic glasses10.1016/j.actamat.2012.05.025 ↗
47. Sample size and preparation effects on the tensile ductility of Pd-based metallic glass nanowires10.1016/j.actamat.2014.12.039 ↗
48. Chemistry (intrinsic) and inclusion (extrinsic) effects on the toughness and Weibull modulus of Fe-based bulk metallic glasses10.1080/09500830802438131 ↗
49. On the variability in fracture toughness of ‘ductile’ bulk metallic glasses10.1016/j.scriptamat.2015.02.017 ↗
50. Fracture of metallic glasses at notches: Effects of notch-root radius and the ratio of the elastic shear modulus to the bulk modulus on toughness10.1016/j.actamat.2009.08.031 ↗
51. Intrinsic and extrinsic effects on the fracture toughness of ductile metallic glasses10.1016/j.mechmat.2021.104066 ↗
52. Fast parallel algorithms for short-range molecular dynamics10.1006/jcph.1995.1039 ↗
53. Polymorphic transitions in single crystals: a new molecular dynamics method10.1063/1.328693 ↗
54. A unified formulation of the constant temperature molecular dynamics methods10.1063/1.447334 ↗
55. Local order influences initiation of plastic flow in metallic glass: Effects of alloy composition and sample cooling history10.1016/j.actamat.2008.07.011 ↗
56. Notch strengthening in nanoscale metallic glasses10.1016/j.actamat.2019.02.044 ↗
57. Cyclic deformation in metallic glasses10.1021/acs.nanolett.5b03045 ↗
58. On measuring the fracture energy of model metallic glasses10.1063/1.5037352 ↗
59. Heterogeneous structural changes correlated to local atomic order in thermal rejuvenation process of Cu-Zr metallic glass10.1080/14686996.2019.1624140 ↗
60. Theory of shear banding in metallic glasses and molecular dynamics calculations10.2320/matertrans.MJ200769 ↗
61. Plastic deformation of pressured metallic glass10.3390/ma10121361 ↗
62. Mechanical and structural assessment of CuZr metallic glasses rejuvenated by thermal-pressure treatments10.1016/j.commatsci.2021.110681 ↗
63. Rejuvenation by weakening the medium range order in Zr46Cu46Al8 metallic glass with pressure preloading: A molecular dynamics simulation study10.1016/j.matdes.2018.08.040 ↗
64. Structural origins for the generation of strength, ductility and toughness in bulk-metallic glasses using hydrogen microalloying10.1016/j.actamat.2019.04.022 ↗
65. Tuning order in disorder10.1038/nmat4300 ↗
66. Atomic-level structure and structure-property relationship in metallic glasses10.1016/j.pmatsci.2010.12.002 ↗
67. A molecular dynamics simulation study of solid-like and liquid-like networks in Zr46Cu46Al8 metallic glass10.1016/j.jnoncrysol.2015.05.003 ↗