Difference in radiation effects of sodium borosilicate glass and vitreous silica with ions
Source abstract
Abstract
Abstract Borosilicate glass is used to vitrify high-level radioactive waste. Radiation effects on borosilicate glass have been studied extensively. Sodium borosilicate glass samples with compositions of 67.3% SiO2, 16.7% B2O3 and 16% Na2O in molar percent and vitreous silica were irradiated with multi-energy and single-energy Xe ions. After irradiation, hardness and modulus of both materials were accessed by nanoindentation. Volume change in two materials was evaluated using AFM. The hardness, modulus and volume change of both sodium borosilicate glass and vitreous silica varied fast and then saturated with the dose. The trends of both modulus and volume change with the dose for sodium borosilicate glass were respectively opposite to those for vitreous silica. The relative hardness variation of sodium borosilicate glass was −35%, and that of vitreous silica was about −10%. Difference in radiation effects between the sodium borosilicate glass and vitreous silica suggested that hardness decrease in sodium borosilicate glass irradiated with ion might be induced not only by transformation of silicate network but also by the transformation of boron network.
Source: openaire · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Nuclear materials and radiation effects · Glass properties and applications · Luminescence Properties of Advanced Materials
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (54)
Show source-provided references
1. Recent progress to understand stress corrosion cracking in sodium borosilicate glasses: linking the chemical composition to structural, physical and fracture properties10.1088/1361-6463/aa7a8b ↗
2. Fracture toughness in nuclear waste glasses and ceramics: environmental and radiation effects
3. Sodium diffusion in the nuclear waste glass GP 98/1210.1111/j.1151-2916.1989.tb05969.x ↗
4. Effect of alpha radiation on the leaching behaviour of nuclear glass10.1016/j.jnucmat.2007.01.099 ↗
5. Microstructure of simulated high-level waste glass doped with short lived actinides, 238Pu and 244Cm10.1557/PROC-257-199 ↗
6. Radiation effect in nuclear waste glasses10.1016/0168-583X(88)90257-1 ↗
7. Radiation effects in nuclear waste forms for high-level radioactive waste10.1016/0149-1970(94)00016-Y ↗
8. Dose, dose rate and irradiation temperature effects in β-irradiated simplified nuclear waste glasses by EPR spectroscopy10.1016/S0022-3093(01)00338-6 ↗
9. Effect of chemical composition on borosilicate glass behavior under irradiation10.1016/j.jnoncrysol.2009.11.030 ↗
10. The effects of ionizing radiation on HLW glasses10.1016/0022-3093(83)90075-3 ↗
11. Effect of 10B(n, α)7Li irradiation on the structure of a sodium borosilicate glass10.1016/j.nimb.2013.09.042 ↗
12. Electron beam irradiation effects in Trombay nuclear waste glass10.1016/j.nimb.2011.06.009 ↗
13. Gamma radiation induced changes in nuclear waste glass containing Eu10.1016/j.physb.2011.07.043 ↗
14. Influence of electronic irradiation on failure and hardness properties of pure silica glasses10.1016/j.mspro.2014.10.037 ↗
15. Indentation testing of nuclear-waste glasses10.1007/BF00550807 ↗
16. Specific outcomes of the research on the radiation stability of the French nuclear glass towards alpha decay accumulation10.1016/j.jnucmat.2013.09.039 ↗
17. Raman spectra and nano-indentation of Ar-irradiated borosilicate glass10.1016/j.nimb.2013.09.020 ↗
18. Variation of hardness and modulus of borosilicate glass irradiated with Kr ions10.1016/j.nimb.2017.04.057 ↗
19. Variation of hardness and modulus of sodium borosilicate glass irradiated with different ions10.1016/j.nimb.2018.01.006 ↗
20. Radiation induced paramagnetic centres in nuclear glasses by EPR spectroscopy10.1016/S0168-583X(98)00102-5 ↗
21. Molecular dynamics simulation of radiation damage in glasses10.1016/j.jnoncrysol.2011.02.026 ↗
22. Alpha decays impact on nuclear glass structure10.1016/j.mspro.2014.10.033 ↗
23. Discussion on the structural origins of the fracture toughness and hardness changes in rapidly quenched borosilicate glasses: a molecular dynamics study10.1016/j.mspro.2014.10.034 ↗
24. Deformation mechanisms during nanoindentation of sodium borosilicate glasses of nuclear interest10.1063/1.4885850 ↗
25. Structural origin of hardness decrease in irradiated sodium borosilicate glass10.1063/1.5004220 ↗
26. SRIM—the stopping and range of ions in matter10.1016/j.nimb.2010.02.091 ↗
27. Microscopic structural changes ofSiO2glasses as a function of temperature investigated byin situRaman spectroscopy10.1103/PhysRevB.73.214206 ↗
28. Identification of Raman defect lines as signatures of ring structures in vitreous silica10.1103/PhysRevLett.80.5145 ↗
29. Micro-Raman studies on 50keV electron irradiated silicate glass10.1016/j.jnoncrysol.2006.08.026 ↗
30. Raman spectroscopy study of β-irradiated silica glass10.1016/S0022-3093(03)00334-X ↗
31. Raman studies of vitreous SiO2 versus fictive temperature10.1103/PhysRevB.28.3266 ↗
32. Analysis of molecular oxygen formation in irradiated glasses: a Raman depth profile study10.1016/j.jnucmat.2004.11.011 ↗
33. Raman spectra of indented pristine and irradiated sodium borosilicate glasses10.1016/j.jnoncrysol.2017.03.012 ↗
34. Advances in understanding the structure of borosilicate glasses: a Raman spectroscopy study10.2138/am.2009.3027 ↗
35. Structure of borosilicate glasses and melts: a revision of the Yun, Bray and Dell model10.1016/j.jnoncrysol.2009.08.033 ↗
36. Quantitative measurement of Q3 species in silicate and borosilicate glasses using Raman spectroscopy10.1016/j.jnoncrysol.2007.06.105 ↗
37. Raman study of b-irradiated glasses10.1016/S0022-3093(98)00822-9 ↗
38. Comparison of hardness variation of ion irradiated borosilicate glasses with different projected ranges10.1016/j.nimb.2018.01.017 ↗
39. Effects of deposited nuclear and electronic energy on the hardness of R7T7-type containment glass10.1016/j.nimb.2005.12.053 ↗
40. Understanding of the mechanical and structural changes induced by alpha particles and heavy ions in the French simulated nuclear waste glass10.1016/j.jnucmat.2016.04.022 ↗
41. Densification, anisotropic deformation, and plastic flow of SiO2 during MeV heavy ion irradiation10.1063/1.112646 ↗
42. Neutron irradiation effects and structure of noncrystalline SiO210.1063/1.1681714 ↗
43. Radiation and thermal ageing of nuclear waste glass10.1016/j.mspro.2014.10.031 ↗
44. Radiation effects in glasses used for immobilization of high-level waste and plutonium disposition10.1557/JMR.1997.0266 ↗
45. Molecular dynamics study of structural changes versus deposited energy dose in a sodium borosilicate glass10.1016/j.nimb.2008.03.217 ↗
46. Effect of irradiation on hardness of borosilicate glass10.1016/j.jnoncrysol.2016.04.027 ↗
47. Mono and sequential ion irradiation induced damage formation and damage recovery in oxide glasses: stopping power dependence of the mechanical properties10.1016/j.jnucmat.2015.12.004 ↗
48. Understanding and simulating the material behavior during multi-particle irradiations10.1038/srep30191 ↗
49. Comparative effects of thermal quenching and ballistic collisions in SiO2–B2O3–Na2O glass10.1016/j.nimb.2013.10.061 ↗
50. Raman spectroscopy study of beta-irradiated silica glass10.1016/S0022-3093(03)00334-X ↗
51. Irradiation effects in simplified nuclear waste glasses10.1016/j.nimb.2005.06.105 ↗
52. Surface and bulk electron irradiation effects in simple and complex glasses10.1016/j.jnoncrysol.2016.10.009 ↗
53. Study of irradiation damage in borosilicate glass induced by He ions and electrons10.1016/j.nimb.2012.12.113 ↗
54. Evolutions of molecular oxygen formation and sodium migration in Xe ion irradiated borosilicate glasses10.1016/j.jnoncrysol.2016.06.029 ↗