Structural investigations of Ge nanoparticles embedded in an amorphous SiO2 matrix
Source abstract
Abstract
Transmission electron microscopy and X-ray photoelectron spectroscopy analyses are performed to investigate Ge nanoparticles embedded in an amorphous SiO2 matrix. GeSiO thin films are prepared by two methods, sol–gel and radio frequency magnetron sputtering. After the deposition, the sol–gel films are annealed in either N2 (at 1 atm and 800 °C) or H2 (at 2 atm and 500 °C), and the sputtered films in H2 (at 2 atm and 500 °C), to allow Ge segregation. Amorphous Ge-rich nanoparticles (3–7 nm size) are observed in sol–gel films. Crystalline Ge nanoparticles in the high pressure tetragonal phase (10–50 nm size) are identified in the sputtered films. The size of the nanoparticles increases with Ge concentration in the volume of the film. At the film surface, the Ge concentration is much larger that in the volume for both sol–gel and sputtered films. At the same time, at the film surface, only oxidized Ge is observed.
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Research context
OpenAlex topics: Silicon Nanostructures and Photoluminescence · Semiconductor materials and devices · Nanowire Synthesis and Applications
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References (52)
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1. Allen LC (1989) Electronegativity is the average one-electron energy of the valence-shell electrons in ground-state free atoms. J Am Chem Soc 111:9003–9014. doi: 10.1021/ja00207a00310.1021/ja00207a003 ↗
2. Atzrodt V, Wirth T, Lange H (1980) Investigation of NiSi and Pd3Si thin films by AES and XPS. Phys Status Solidi A 62:531–537. doi: 10.1002/pssa.221062022210.1002/pssa.2210620222 ↗
3. Basa P, Alagoz AS, Lohner T, Kulakci M, Turan R, Nagy K, Horváth ZsJ (2008) Electrical and ellipsometry study of sputtered SiO2 structures with embedded Ge nanocrystals. Appl Surf Sci 254:3626–3629. doi: 10.1016/j.apsusc.2007.10.07510.1016/j.apsusc.2007.10.075 ↗
4. Bearden JA, Burr AF (1967) Reevaluation of X-ray atomic energy levels. Rev Mod Phys 39:125–142. doi: 10.1103/RevModPhys.39.12510.1103/RevModPhys.39.125 ↗
5. Brenier R, Urlacher C, Mugnier J, Brunel M (1999) Stress development in amorphous zirconium oxide films prepared by sol–gel processing. Thin Solid Films 338:136–141. doi: 10.1016/S0040-6090(98)01092-X10.1016/S0040-6090(98)01092-X ↗
6. Ciurea ML, Teodorescu VS, Iancu V, Balberg I (2006) Electronic transport in Si–SiO2 nanocomposite films. Chem Phys Lett 423:225–228. doi: 10.1016/j.cplett.2006.03.07010.1016/j.cplett.2006.03.070 ↗
7. Clarke TA, Rizkalla EN (1976) X-ray photoelectron spectroscopy of some silicates. Chem Phys Lett 37:523–526. doi: 10.1016/0009-2614(76)85029-410.1016/0009-2614(76)85029-4 ↗
8. Conibeer G, Green M, Corkish R, Cho Y, Cho EC, Jiang CW, Fangsuwannarak T, Pink E, Huang YD, Puzzer T, Trupke T, Richards B, Shalav A, Lin KL (2006) Silicon nanostructures for third generation photovoltaic solar cells. Thin Solid Films 511–512:654–662. doi: 10.1016/j.tsf.2005.12.11910.1016/j.tsf.2005.12.119 ↗
9. Das K, NandaGoswami M, Mahapatra R, Kar GS, Dhar A, Acharya HN, Maikap S, Lee J-H, Ray SK (2004) Charge storage and photoluminescence characteristics of silicon oxide embedded Ge nanocrystal trilayer structures. Appl Phys Lett 84:1386–1388. doi: 10.1063/1.164675010.1063/1.1646750 ↗
10. Desnica UV, Salamon K, Buljan M, Dubcek P, Radic N, Desnica-Frankovic ID, Siketic Z, Bogdanovic-Radovic I, Ivanda M, Bernstorff S (2008) Formation of Ge-nanocrystals in SiO2 matrix by magnetron sputtering and post-deposition thermal treatment. Superlattices Microstruct 44:323–330. doi: 10.1016/j.spmi.2008.01.02110.1016/j.spmi.2008.01.021 ↗
11. Duguay S, Grob JJ, Slaoui A, Le Gall Y , Amann-Liess M (2005) Structural and electrical properties of Ge nanocrystals embedded in SiO2 by ion implantation and annealing. J Appl Phys 97(104330):1–5. doi: 10.1063/1.190928610.1063/1.1909286 ↗
12. Gacem K, El Hdiy A, Troyon M, Berbezier I, Szkutnik PD, Karmous A, Ronda A (2007) Memory and Coulomb blockade effects in germanium nanocrystals embedded in amorphous silicon on silicon dioxide. J Appl Phys 102(093704):1–4. doi: 10.1063/1.280401310.1063/1.2804013 ↗
13. Gao F, Green MA, Conibeer G, Cho EC, Huang YD, Pere-Wurfl I, Flynn C (2008) Fabrication of multilayered Ge nanocrystals by magnetron sputtering and annealing. Nanotechnology 19(455611):1–5. doi: 10.1088/0957-4484/19/45/45561110.1088/0957-4484/19/45/455611 ↗
14. Heitmann J, Müller F, Yi LX, Zacharias M, Kovalev D, Eichhorn F (2004) Confinement and migration effects: excitons in Si nanocrystals. Phys Rev B 69(195309):1–7. doi: 10.1103/PhysRevB.69.19530910.1103/PhysRevB.69.195309 ↗
15. Heng CL, Teo NW, Ho V, Tay MS, Lei Y, Choi WK, Chim WK (2003) Effects of rapid thermal annealing time and ambient temperature on the charge storage capability of SiO2/pure Ge/rapid thermal oxide memory structure. Microelectron Eng 66:218–223. doi: 10.1016/S0167-9317(03)00050-910.1016/S0167-9317(03)00050-9 ↗
16. Heng CL, Tjiu WW, Finstad TG (2004) Charge-storage effects in a metal-insulator semiconductor structure containing germanium nano-crystals formed by rapid thermal annealing of an electron-beam evaporated germanium layer. Appl Phys A 78:1181–1186. doi: 10.1007/s00339-003-2482-010.1007/s00339-003-2482-0 ↗
17. Hollinger G (1981) Structures chimique et electronique de l’interface SiO2–Si. Appl Surf Sci 8:318–336. doi: 10.1016/0378-5963(81)90126-410.1016/0378-5963(81)90126-4 ↗
18. Hong SH, Kim MC, Jeong PS, Choi SH, Kim KJ (2008) Ge-nanodot multilayer nonvolatile memories, Nanotechnology 19(305203):1–4. doi: 10.1088/0957-4484/19/30/30520310.1088/0957-4484/19/30/305203 ↗
19. Hüffner S (2003) Photoelectron spectroscopy: principles and applications. Springer-Verlag, Berlin, 3rd revised and enlarged edition, XV, 662 p. 461 illus., Hardcover. ISBN: 978-3-540-41802-3
20. Kanjilal A, Lundsgaard Hansen J, Gaiduk P, Nylandsted Larsen A, Cherkashin N, Claverie A, Normand P, Kapelanakis E, Skarlatos D, Tsoukalas D (2003) Structural and electrical properties of silicon dioxide layers with embedded germanium nanocrystals grown by molecular beam epitaxy. Appl Phys Lett 82:1212–1214. doi: 10.1063/1.155570910.1063/1.1555709 ↗
21. Kanoun M, Souifi A, Baron T, Mazen F (2004) Electrical study of Ge-nanocrystal-based metal-oxide-semiconductor structures for p-type nonvolatile memory applications. Appl Phys Lett 84:5079–5081. doi: 10.1063/1.175122710.1063/1.1751227 ↗
22. Kerkhof FPJ, Moulijn JA, Heeres A (1978) The XPS spectra of the metathesis catalyst tungsten oxide on silica gel. J Electron Spectrosc Relat Phenom. 14:453–466. doi: 10.1016/0368-2048(78)87004-210.1016/0368-2048(78)87004-2 ↗
23. Kovalev D, Heckler H, Ben-Chorin M, Polisski G, Schwartzkopff M, Koch F (1998) Breakdown of the k-conservation rule in Si nanocrystals. Phys Rev Lett 81:2803–2806. doi: 10.1103/PhysRevLett.81.280310.1103/PhysRevLett.81.2803 ↗
24. Luca D, Macovei D, Teodorescu CM (2006) Characterization of titania thin films prepared by reactive pulsed-laser ablation. Surf Sci 600:4342–4346. doi: 10.1016/j.susc.2006.01.16210.1016/j.susc.2006.01.162 ↗
25. Maeda Y (1995) Visible photoluminescence from nanocrystallite Ge embedded in a glassy SiO2 matrix: evidence in support of the quantum-confinement mechanism. Phys Rev B 51:1658–1670. doi: 10.1103/PhysRevB.51.165810.1103/PhysRevB.51.1658 ↗
26. Maeda Y, Tsukamoto N, Yazawa Y, Kanemitsu Y, Masumoto Y (1991) Visible photoluminescence of Ge microcrystals embedded in SiO2 glassy matrices. Appl Phys Lett 59:3168–3170. doi: 10.1063/1.10577310.1063/1.105773 ↗
27. Mardare D, Luca D, Teodorescu CM, Macovei D (2007) On the hydrophilicity of nitrogen-doped TiO2 thin films. Surf Sci 601:4515–4520. doi: 10.1016/j.susc.2007.04.15610.1016/j.susc.2007.04.156 ↗
28. Morgan WE, Van Wazer JR (1973) Binding energy shifts in the x-ray photoelectron spectra of a series of related Group IVa compounds. J Phys Chem 77:964–969. doi: 10.1021/j100626a02310.1021/j100626a023 ↗
29. Nguyen TP, Lefrant S (1989) XPS study of SiO thin films and SiO–metal interfaces. J Phys Cond Matter 1:5197–5204. doi: 10.1088/0953-8984/1/31/01910.1088/0953-8984/1/31/019 ↗
30. NIST X-ray photoelectron spectroscopy database. http://srdata.nist.gov/xps/EngElmSrchQuery.aspx?EType=PE&CSOpt=Retri_ex_dat&Elm=O
31. Nogami M, Abe Y (1994) Sol–gel method for synthesizing visible photoluminescent nanosized Ge-crystal-doped silica glasses. Appl Phys Lett 65:2545–2547. doi: 10.1063/1.11263010.1063/1.112630 ↗
32. Nogami M, Abe Y (1997) Sol–gel synthesis of Ge nanocrystals-doped glass and its photoluminescence. J Sol Gel Sci Tehnol 9:139–143. doi: 10.1023/A:1026461029767
33. Nozaki S, Sato S, Rath S, Ono H, Morisaki H (1999) Optical properties of tetragonal germanium nanocrystals deposited by the cluster-beam evaporation technique: light emitting new material for future. Bull Mater Sci 22:377–381. doi: 10.1007/BF0274994510.1007/BF02749945 ↗
34. Park CJ, Cho KH, Yang W-C, Cho HY, Choi S-H, Elliman RG, Han JH, Kim C (2006) Large capacitance-voltage hysteresis loops in SiO2 films containing Ge nanocrystals produced by ion implantation and annealing. Appl Phys Lett 88(071916):1–3. doi: 10.1063/1.217549510.1063/1.2175495 ↗
35. Peibst R, Durkop T, Bugiel E, Fissel A, Costina I, Hofmann KR (2009) Driving mechanisms for the formation of nanocrystals by annealing of ultrathin Ge layers in SiO2. Phys Rev B 79(195316):1–13. doi: 10.1103/PhysRevB.79.19531610.1103/PhysRevB.79.195316 ↗
36. Powder Diffraction File. http://www.icdd.com
37. Rodríguez A, Morana B, Sangrador J, Rodríguez T, Kling A, Ortiz MI, Ballesteros C (2009) Formation of Ge nanocrystals and evolution of the oxide matrix in as-deposited and annealed LPCVD SiGeO films. Superlattices Microstruct 45:343–348. doi: 10.1016/j.spmi.2008.10.03710.1016/j.spmi.2008.10.037 ↗
38. Shalvoy RB, Fisher GB, Stiles PJ (1977) Bond ionicity and structural stability of some average-valence-five materials studied by x-ray photoemission. Phys Rev B 15:1680–1697. doi: 10.1103/PhysRevB.15.168010.1103/PhysRevB.15.1680 ↗
39. Shen JK, Wu XL, Yuan RK, Tang N, Zou JP, Mei YF, Tan C, Bao XM (2000) Enhanced ultraviolet photoluminescence from SiO2/Ge:SiO2/SiO2 sandwiched structure. Appl Phys Lett 77:3134–3136. doi: 10.1063/1.132539910.1063/1.1325399 ↗
40. Stoica TF, Gartner M, Teodorescu VS, Stoica T (2007) Ge dots embedded in silicon dioxide using sol–gel deposition. J Optoelectron Adv Mater 9:3271–3274. http://inoe.inoe.ro/joam/index.php?option=magazine&op=view&idu=1004&catid=18
41. Takeoka S, Fujii M, Hayashi S, Yamamoto K (1998) Size-dependent near-infrared photoluminescence from Ge nanocrystals embedded in SiO2 matrices. Phys Rev B 58:7921–7925. doi: 10.1103/PhysRevB.58.792110.1103/PhysRevB.58.7921 ↗
42. Teodorescu VS, Blanchin MG (2009) Fast and simple specimen preparation for TEM studies of oxide films deposited on silicon wafers. Microsc Microanal 15:15–19. doi: 10.1017/S143192760909001110.1017/S1431927609090011 ↗
43. Teodorescu CM, Socol G, Negrila C, Luca D, Macovei D (2010) Nanostructured thin layers of vanadium oxides doped with cobalt, prepared by pulsed laser ablation: chemistry, local atomic structure, morphology and magnetism. J Exp Nanosci. doi: 10.1080/17458081003671675 .10.1080/17458081003671675 ↗
44. Wagner CD, Zatko DA, Raymond RH (1980) Use of the oxygen KLL Auger lines in identification of surface chemical states by electron spectroscopy for chemical analysis. Anal Chem 52:1445–1451. doi: 10.1021/ac50059a01710.1021/ac50059a017 ↗
45. Wagner CD, Davis LE, Zeller MV, Taylor JA, Raymond RM, Gale LH (1981) Empirical atomic sensitivity factors for quantitative analysis by electron spectroscopy for chemical analysis. Surf Interface Anal 3:211–225. doi: 10.1002/sia.74003050610.1002/sia.740030506 ↗
46. Walters RJ, Bourianoff GI, Atwater HA (2005) Field-effect electroluminescence in silicon nanocrystals. Nat Mater 4:143–146. doi: 10.1038/nmat130710.1038/nmat1307 ↗
47. Wosylus A, Prots Y, Schnelle W, Hanfland M, Schwarz U (2008) Crystal structure refinements of Ge(tP12), physical properties and pressure-induced phase transformation Ge(tP12) ↔ Ge(tI4). Z Naturforsch B 63b:608–614. http://www.znaturforsch.com/ab/v63b/63b0608.pdf10.1515/znb-2008-0603 ↗
48. Yang HQ, Wang XJ, Shi HZ, Xie SH, Wang FJ, Gu XX, Yao X (2002) Photoluminescence of Ge nanodots embedded in SiO2 glasses fabricated by a sol–gel method. Appl Phys Lett 81:5144–5146. doi: 10.1063/1.150694310.1063/1.1506943 ↗
49. Yang HQ, Yang RL, Wan XQ, Wan WL (2004) Structure and photoluminescence of Ge nanodots with different sizes embedded in SiO2 glasses fabricated by a sol–gel method. J Cryst Growth 261:549–556. doi: 10.1016/j.jcrysgro.2003.08.08110.1016/j.jcrysgro.2003.08.081 ↗
50. Yang HQ, Yao X, Xie SH, Wang XJ, Liu SX, Fang Y, Gu XX, Wang FJ (2005) Structure and photoluminescence of Ge nanodots embedded in SiO2 gel glasses fabricated at different temperatures. Opt Mater 27:725–730. doi: 10.1016/j.optmat.2004.09.01710.1016/j.optmat.2004.09.017 ↗
51. Yang M, Chen TP, Ding L, Wong JI, Liu Y, Zhang WL, Zhang S, Zhu F, Goh WP (2009) Implant energy-dependent enhancement of electroluminescence from Ge-implanted SiO2 thin films. Electrochem Solid State Lett 12:H238–H240. doi: 10.1149/1.311852410.1149/1.3118524 ↗
52. Zhang FX, Wang WK (1995) Crystal structure of germanium quenched from the melt under high pressure. Phys Rev B 52:3113–3116. doi: 10.1103/PhysRevB.52.311310.1103/PhysRevB.52.3113 ↗