Solid pyrolysis synthesis of excitation-independent emission carbon dots and its application to isoniazid detection
Source abstract
Abstract
In this paper, a novel fluorescence carbon dots (FCDs) were proposed to use folic acid as the sole reactant via the pyrolytic way. The gotten FCDs were uniform in size distribution and had an excitation-independent emission feature, and their fluorescence quantum yield was 39.09%. Without additional modification, the acquired FCDs could be used to detect isoniazid by the fluorescence quenching pattern. The reaction mechanism was the synergy of the internal filtration effect and the static quenching effect. The linear range of the detection of isoniazid was 4.0–140 μM, and the detection limit was 1.15 μM. Therefore, the method for the determination of isoniazid was put forward. The method was applied to the detection of isoniazid in isoniazid tablets with the recovery rates of 98.12 to 102.67%, and the results were satisfactory.
Source: openaire · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Carbon and Quantum Dots Applications · Heavy Metal Exposure and Toxicity · Electrochemical sensors and biosensors
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (37)
Show source-provided references
1. Arshad N, Yunus U, Razzque S, Khan M, Saleem S, Mirza B, Rashid N (2012) Electrochemical and spectroscopic investigations of isoniazide and its analogs with ds. DNA at physiological pH: evaluation of biological activities. Eur J Med Chem 47:452–46110.1016/j.ejmech.2011.11.014 ↗
2. Baker SN, Baker GA (2010) Luminescent carbon nanodots: emergent nanolights. Angew Chem Int Ed 49:6726–674410.1002/anie.200906623 ↗
3. Cai AJ, Wang Q, Chang YF, Wang XP (2017) Graphitic carbon nitride decorated with S,N co-doped graphene quantum dots for enhanced visible-light-driven photocatalysis. J Alloys Compd 692:183–18910.1016/j.jallcom.2016.09.030 ↗
4. Campos BB, Oliva MM, Contreras-Cáceres R, Rodriguez-Castellón E, Jiménez-Jiménez J, da Silva JCGE, Algarra M (2016) Carbon dots on based folic acid coated with PAMAM dendrimer as platform for Pt (IV) detection. J Colloid Interface Sci 465:165–17310.1016/j.jcis.2015.11.059 ↗
5. Cao L, Wang X, Meziani MJ, Lu F, Wang H, Luo PG, Lin Y, Harruff BA, Veca LM, Murray D, Xie SY, Sun YP (2007) Carbon dots for multiphoton bioimaging. J Am Chem Soc 129:11318–1131910.1021/ja073527l ↗
6. El-Brashy AM, El-Ashry SM (1992) Colorimetric and titrimetric assay of isoniazid. J Pharm Biomed Anal 10:421–42610.1016/0731-7085(92)80060-Z ↗
7. Haghighi B, Bozorgzadeh S (2010) Flow injection chemiluminescence determination of isoniazid using luminol and silver nanoparticles. Microchem J 95:192–19710.1016/j.microc.2009.11.012 ↗
8. Hou P, Yang T, Liu H, Li YF, Huang CZ (2017) An active structure preservation method for developing functional graphitic carbon dots as an effective antibacterial agent and a sensitive pH and Al( III ) nanosensor. Nanoscale 9:17334–1734110.1039/C7NR05539K ↗
9. Hu Y, Yang J, Tian J, Yu JS (2015) How do nitrogen-doped carbon dots generate from molecular precursors? An investigation of the formation mechanism and a solution-based large-scale synthesis. J Mater Chem B 3:5608–561410.1039/C5TB01005E ↗
10. Huang J, Zheng Q, Kim JK, Li Z (2013) A molecular beacon and graphene oxide-based fluorescent biosensor for Cu2+ detection. Biosens Bioelectron 43:379–38310.1016/j.bios.2012.12.056 ↗
11. Jena BK, Raj CR (2010) Au nanoparticle decorated silicate network for the amperometric sensing of isoniazid. Talanta 80:1653–165610.1016/j.talanta.2009.10.002 ↗
12. Khan S, Gupta A, Verma NC, Nandi CK (2015) Time-resolved emission reveals ensemble of emissive states as the origin of multicolor fluorescence in carbon dots. Nano Lett 15:8300–830510.1021/acs.nanolett.5b03915 ↗
13. Li H, Kang Z, Liu Y, Lee ST (2012) Carbon nanodots: synthesis, properties and applications. J Mater Chem 22:24230–2425310.1039/c2jm34690g ↗
14. Li XM, Zhang SL, Kulinich SA, Liu YL, Zeng HB (2014) Engineering surface states of carbon dots to achieve controllable luminescence for solid-luminescent composites and sensitive Be2+ detection. Sci Rep 4:497610.1038/srep04976 ↗
15. Li N, Liu T, Liu SG, Lin SM, Fan YZ, Luo HQ, Li NB (2017) Visible and fluorescent detection of melamine in raw milk with one-step synthesized silver nanoparticles using carbon dots as the reductant and stabilizer. Sensors Actuators B Chem 248:597–60410.1016/j.snb.2017.03.068 ↗
16. Liu XX, Liu JR, Zheng BZ, Yan L, Dai J, Zhuang Z, du J, Guo Y, Xiao D (2017) N-doped carbon dots: green and efficient synthesis on a large-scale and their application in fluorescent pH sensing. New J Chem 41:10607–1061210.1039/C7NJ01889D ↗
17. Majidi MR, Jouyban A, Asadpour-Zeynali K (2006) Asadpour-Zeynali K Voltammetric behavior and determination of isoniazid in pharmaceuticals by using overoxidized polypyrrole glassy carbon modified electrode. J Electroanal Chem 589:32–3710.1016/j.jelechem.2006.01.016 ↗
18. Meng A, Xu QH, Zhao K, Li ZJ, Liang J, Li QD (2018) A highly selective and sensitive “on-off-on” fluorescent probe for detecting Hg (II) based on Au/N-doped carbon quantum dots. Sensors Actuators B Chem 255:657–66510.1016/j.snb.2017.08.028 ↗
19. Rastogi PK, Ganesan V, Azad UP (2016) Electrochemical determination of nanomolar levels of isoniazid in pharmaceutical formulation using silver nanoparticles decorated copolymer. Electrochim Acta 188:818–82410.1016/j.electacta.2015.12.058 ↗
20. Safavi A, Karimi MA, Hormozi Nezhad MR, Kamali R, Saghir N (2004) Sensitive indirect spectrophotometric determination of isoniazid. Spectrochim Acta A 60:765–76910.1016/S1386-1425(03)00288-9 ↗
21. Strauss V, Margraf JT, Dolle C, Butz B, Nacken TJ, Walter J, Bauer W, Peukert W, Spiecker E, Clark T, Guldi DM (2014) Carbon nanodots: toward a comprehensive understanding of their photoluminescence. J Am Chem Soc 136:17308–1731610.1021/ja510183c ↗
22. Tian T, Zhong YP, Deng C, Wang H, He Y, Ge YL, Song GW (2017) Brightly near-infrared to blue emission tunable silver-carbon dot nanohybrid for sensing of ascorbic acid and construction of logic gate. Talanta 162:135–14210.1016/j.talanta.2016.10.021 ↗
23. Verma KK, Palod S (1985) The titrimetric determination of 4-pyridine carboxylic acid hydrazide (isoniazid) in drug formulations with thallium (III). Anal Lett 18:11–1910.1080/00032718508066921 ↗
24. Wang EK, Zhou WH (1996) Determination of isoniazid and hydrazine by capillary electrophoresis with amperometric detection at a Pt-particle modified carbon fiber microelectrode. Chin J Chem 14:131–13710.1002/cjoc.19960140207 ↗
25. Wang L, Yin Y, Jain A, Zhou HS (2014) Aqueous phase synthesis of highly luminescent, nitrogen-doped carbon dots and their application as bioimaging agents. Langmuir 30:14270–1427510.1021/la5031813 ↗
26. Wang H, Sun C, Chen XG, Zhang Y, Colvin VL, Rice Q, Seo J, Feng S, Wang S, Yu WW (2017) Excitation wavelength independent visible color emission of carbon dots. Nanoscale 9:1909–191510.1039/C6NR09200D ↗
27. Wang B, Liu F, Wu YY, Chen YF, Weng B, Li CM (2018) Synthesis of catalytically active multielement-doped carbon dots and application for colorimetric detection of glucose. Sensors Actuators B 255:2601–260710.1016/j.snb.2017.09.067 ↗
28. Wu B, Wang Z, Xue Z, Zhou X, Du J, Liu X, Lu X (2012b) A novel molecularly imprinted electrochemiluminescence sensor for isoniazid detection. Analyst 137:3644–365210.1039/c2an35499c ↗
29. Wu D, Zhang F, Liang H, Feng X (2012a) Nanocomposites and macroscopic materials: assembly of chemically modified graphene sheets. Chem Soc Rev 41:6160–617710.1039/c2cs35179j ↗
30. Wu M, Wang Y, Wu W, Hu C, Wang X, Zheng J, Li Z, Jiang B, Qiu J (2014) Preparation of functionalized water-soluble photoluminescent carbon quantum dots from petroleum coke. Carbon 78:480–48910.1016/j.carbon.2014.07.029 ↗
31. Yang Z, Xu MH, Liu Y, He FJ, Gao F, Su YJ, Wei H, Zhang YF (2014) Nitrogen-doped, carbon-rich, highly photoluminescent carbon dots from ammonium citrate. Nanoscale 6:1890–189510.1039/C3NR05380F ↗
32. Zargar B, Hatamie A (2013) Localized surface plasmon resonance of gold nanoparticles as colorimetric probes for determination of isoniazid in pharmacological formulation. Spectrochim Acta A 106:185–18910.1016/j.saa.2013.01.003 ↗
33. Zhai XY, Zhang P, Liu CJ, Bai T, Li WC, Dai LM, Liu WG (2012) Highly luminescent carbon nanodots by microwave-assisted pyrolysis. Chem Commun 48:7955–795710.1039/c2cc33869f ↗
34. Zhang RZ, Chen W (2014) Nitrogen-doped carbon quantum dots: facile synthesis and application as a “turn-off” fluorescent probe for detection of Hg2+ ions. Biosens Bioelectron 55:83–9010.1016/j.bios.2013.11.074 ↗
35. Zheng L, Chi Y, Dong Y, Lin J, Wang B (2009) Electrochemiluminescence of water-soluble carbon nanocrystals released electrochemically from graphite. J Am Chem Soc 131:4564–456510.1021/ja809073f ↗
36. Zhu S, Song Y, Zhao X, Shao J, Zhang J, Yang B (2015) The photoluminescence mechanism in carbon dots (graphene quantum dots, carbon nanodots, and polymer dots): current state and future perspective. Nano Rev 8:355–381
37. Zhuo SJ, Shao MW, Lee ST (2012) Upconversion and downconversion fluorescent graphene quantum dots: ultrasonic preparation and photocatalysis. ACS Nano 2:1059–106410.1021/nn2040395 ↗