journal article·2025-08-05Open access

Light-Matter Interaction in Ultrastable Tunneling Nanogaps

Yuankai Tang, Saurav Prakash, Proloy Nandi, Ariando Ariando, Amit Agrawal, Hayk Harutyunyan

ACS Nano· Volume 19· Issue 30

Abstract

Light emission and detection through tunnel junctions have emerged as a promising platform for studying nanoscale light-matter interactions, including electroluminescence and photoassisted transport. However, controlling these interactions in the tunneling regime has been challenging due to complex underlying mechanisms that remain poorly understood. A major obstacle is the difficulty in forming stable junctions that can function reliably over extended periods. In this study, we fabricate ultrastable tunneling junctions consisting of epitaxial indium-tin-oxide, epitaxial lutetium oxide, and gold. With their stable and consistent tunneling currents, we investigate photon-assisted transport phenomena using simple direct-current detection. Our results demonstrate that optical rectification is the primary contributor to the laser-induced current, alongside thermal effects and hot-electron currents. Furthermore, owing to their epitaxial nature and high breakdown threshold, this ultrastable platform holds promise for future real-world applications, including nanoscale light sources and multifunctional photodetectors.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Molecular Junctions and Nanostructures · Plasmonic and Surface Plasmon Research · Nanowire Synthesis and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics

Emory University

National University of Singapore

Department of Engineering

University of Cambridge

Kyung Hee University, 26 Kyungheedae-ro, Dongdaemun-gu, Seoul 02447, Korea

Funding

Basic Energy Sciences · Ministry of Education (MOE), Singapore

References (62)

Show source-provided references
1. Griffiths D. J. · 201810.1017/9781316995433 ↗
2. Bohm D. · 2012
3. 10.1126/science.183.4130.114910.1126/science.183.4130.1149 ↗
4. 10.1063/1.173597310.1063/1.1735973 ↗
5. 10.1103/PhysRev.140.A17910.1103/PhysRev.140.A179 ↗
6. 10.1103/PhysRev.109.60310.1103/PhysRev.109.603 ↗
7. Sze S. M. · 2021
8. 10.1103/PhysRevLett.49.5710.1103/PhysRevLett.49.57 ↗
9. 10.1063/5.012882210.1063/5.0128822 ↗
10. 10.1021/acsphotonics.8b0072610.1021/acsphotonics.8b00726 ↗
11. 10.1088/1361-6633/ab423910.1088/1361-6633/ab4239 ↗
12. 10.1103/PhysRevLett.37.92310.1103/PhysRevLett.37.923 ↗
13. 10.1103/PhysRevLett.106.22680210.1103/PhysRevLett.106.226802 ↗
14. 10.1021/acsphotonics.1c0175710.1021/acsphotonics.1c01757 ↗
15. 10.1002/adom.20210180410.1002/adom.202101804 ↗
16. 10.1002/advs.20190029110.1002/advs.201900291 ↗
17. 10.1021/acs.nanolett.3c0368410.1021/acs.nanolett.3c03684 ↗
18. 10.1021/acsphotonics.3c0038310.1021/acsphotonics.3c00383 ↗
19. 10.1038/nphoton.2015.14110.1038/nphoton.2015.141 ↗
20. 10.1038/nnano.2015.20310.1038/nnano.2015.203 ↗
21. 10.1038/s41467-021-23512-210.1038/s41467-021-23512-2 ↗
22. 10.1038/s41467-018-08266-810.1038/s41467-018-08266-8 ↗
23. 10.1021/acsnano.7b0916310.1021/acsnano.7b09163 ↗
24. 10.1021/acs.nanolett.1c0050310.1021/acs.nanolett.1c00503 ↗
25. 10.1021/acs.nanolett.0c0212110.1021/acs.nanolett.0c02121 ↗
26. 10.1021/acs.nanolett.0c0394510.1021/acs.nanolett.0c03945 ↗
27. 10.1109/JQE.1979.106993110.1109/JQE.1979.1069931 ↗
28. 10.1038/nnano.2010.17610.1038/nnano.2010.176 ↗
29. 10.1021/nl201517k10.1021/nl201517k ↗
30. 10.1021/acsnano.1c0410010.1021/acsnano.1c04100 ↗
31. 10.1515/nanoph-2022-027810.1515/nanoph-2022-0278 ↗
32. 10.1021/nl404707t10.1021/nl404707t ↗
33. 10.1021/nl203196z10.1021/nl203196z ↗
34. 10.1038/ncomms272810.1038/ncomms2728 ↗
35. 10.1021/nl404437310.1021/nl4044373 ↗
36. 10.1021/acs.nanolett.6b0509110.1021/acs.nanolett.6b05091 ↗
37. 10.1002/advs.20210157210.1002/advs.202101572 ↗
38. 10.1021/acs.nanolett.8b0461210.1021/acs.nanolett.8b04612 ↗
39. 10.1515/nanoph-2018-008310.1515/nanoph-2018-0083 ↗
40. 10.1021/acs.jpclett.7b0050710.1021/acs.jpclett.7b00507 ↗
41. 10.1063/1.171382010.1063/1.1713820 ↗
42. 10.1103/PhysRevB.84.23543110.1103/PhysRevB.84.235431 ↗
43. 10.1021/acs.nanolett.7b0315310.1021/acs.nanolett.7b03153 ↗
44. 10.1038/s41563-023-01591-410.1038/s41563-023-01591-4 ↗
45. 10.1126/science.abb345710.1126/science.abb3457 ↗
46. 10.1063/1.170000810.1063/1.1700008 ↗
47. 10.1063/1.170268210.1063/1.1702682 ↗
48. 10.1063/1.165914110.1063/1.1659141 ↗
49. 10.1063/1.171321110.1063/1.1713211 ↗
50. Prakash, S. Oxide-Based Novel Light Emitter and Tunable Absorber, National University of Singapore, Singapore, 2020. thesis.
51. 10.1021/ac048600u10.1021/ac048600u ↗
52. 10.1063/1.37170810.1063/1.371708 ↗
53. 10.1021/cr940055h10.1021/cr940055h ↗
54. 10.1063/1.243144310.1063/1.2431443 ↗
55. 10.1109/TNANO.2012.221189310.1109/TNANO.2012.2211893 ↗
56. 10.1063/1.488979810.1063/1.4889798 ↗
57. 10.1021/acs.nanolett.5b0186110.1021/acs.nanolett.5b01861 ↗
58. 10.1063/1.279909110.1063/1.2799091 ↗
59. 10.1007/s00340-003-1391-410.1007/s00340-003-1391-4 ↗
60. 10.1038/s41566-017-0003-510.1038/s41566-017-0003-5 ↗
61. 10.1063/1.172977410.1063/1.1729774 ↗
62. Hugonin J. P. · arXiv · 2021 · 2101.00901