journal article·2024-10-22

On-Surface Atomic Scale Qubit Platform

Christoph Wolf, Andreas J. Heinrich, Soo-hyon Phark

ACS Nano· Volume 18· Issue 42
Publisher page

Abstract

Recent advances in scanning probe microscopy combined with electron spin resonance have revealed that localized electron spins on or near surfaces can be utilized as building blocks for the bottom-up assembly of functional quantum-coherent nanostructures. In this perspective, we review the recent advances, lay out advantages of this platform and outline the challenges that lie ahead on the way to the application of on-surface atomic spins to quantum information science and quantum computing.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Quantum and electron transport phenomena · Surface and Thin Film Phenomena · Quantum Information and Cryptography

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Center for Quantum Nanoscience, Institute for Basic Science (IBS), Seoul 03760, Korea

Ewha Womans University, Seoul 03760, Korea

Department of Physics, Ewha Womans University, Seoul 03760, Korea

Funding

Institute for Basic Science

References (78)

Show source-provided references
1. 10.1038/3500500110.1038/35005001 ↗
2. 10.1038/s41565-021-00994-110.1038/s41565-021-00994-1 ↗
3. 10.1103/PhysRevB.74.16120310.1103/PhysRevB.74.161203 ↗
4. 10.1103/PhysRevB.88.16141210.1103/PhysRevB.88.161412 ↗
5. 10.1103/PRXQuantum.5.02033410.1103/PRXQuantum.5.020334 ↗
6. 10.1038/344524a010.1038/344524a0 ↗
7. 10.1038/s41467-021-21274-510.1038/s41467-021-21274-5 ↗
8. 10.1126/science.abg822310.1126/science.abg8223 ↗
9. 10.1126/science.adf268510.1126/science.adf2685 ↗
10. 10.1103/RevModPhys.89.03500210.1103/RevModPhys.89.035002 ↗
11. 10.1038/nnano.2017.1810.1038/nnano.2017.18 ↗
12. 10.1038/s41565-024-01724-z10.1038/s41565-024-01724-z ↗
13. 10.1126/science.aac870310.1126/science.aac8703 ↗
14. 10.1126/science.aay677910.1126/science.aay6779 ↗
15. 10.1103/PhysRevResearch.2.01303210.1103/PhysRevResearch.2.013032 ↗
16. 10.1063/5.009608110.1063/5.0096081 ↗
17. 10.1103/PhysRevB.96.20542010.1103/PhysRevB.96.205420 ↗
18. 10.1103/PhysRevB.100.03541110.1103/PhysRevB.100.035411 ↗
19. 10.1103/PhysRevB.104.24543510.1103/PhysRevB.104.245435 ↗
20. 10.1103/PhysRevB.107.23540410.1103/PhysRevB.107.235404 ↗
21. 10.1016/j.progsurf.2021.10062510.1016/j.progsurf.2021.100625 ↗
22. 10.1021/acsnano.1c0639410.1021/acsnano.1c06394 ↗
23. 10.1126/sciadv.aaq154310.1126/sciadv.aaq1543 ↗
24. 10.1038/nphys396510.1038/nphys3965 ↗
25. 10.1021/acsnano.3c0475410.1021/acsnano.3c04754 ↗
26. 10.1126/science.ade505010.1126/science.ade5050 ↗
27. 10.1103/PhysRevResearch.6.02312610.1103/PhysRevResearch.6.023126 ↗
28. 10.1021/acsnano.4c0019610.1021/acsnano.4c00196 ↗
29. Broekhoven, R.; Lee, C.; Phark, S.h.; Otte, S.; Wolf, C. Protocol for certifying entanglement in surface spin systems using a scanning tunneling microscope. arXiv, 2024, 2401.15017. http://arxiv.org/abs/2401.15017 (accessed 09 11, 2024).
30. 10.1103/PhysRevLett.68.251210.1103/PhysRevLett.68.2512 ↗
31. 10.1103/PhysRevB.50.552810.1103/PhysRevB.50.5528 ↗
32. 10.1103/PhysRevB.70.19534510.1103/PhysRevB.70.195345 ↗
33. 10.1002/advs.20230203310.1002/advs.202302033 ↗
34. timeESR, ver. 1.0.1; 2024. https://github.com/qphensurf/TimeESR (accessed 09 11, 2024).
35. 10.1103/PhysRevLett.121.02720110.1103/PhysRevLett.121.027201 ↗
36. 10.1021/acs.nanolett.1c0274410.1021/acs.nanolett.1c02744 ↗
37. 10.1038/s41467-021-24465-210.1038/s41467-021-24465-2 ↗
38. Reina-Gálvez, J.; Le, H.A.; Bui, H. T.; Phark, S.h.; Lorente, N.; Wolf, C. Efficient driving of a spin-qubit using single-atom magnets. arXiv, 2024, 2408.07289. https://arxiv.org/abs/2408.07289 (accessed 09 11, 2024).
39. 10.1038/s41534-023-00716-610.1038/s41534-023-00716-6 ↗
40. 10.1038/s41586-023-06754-610.1038/s41586-023-06754-6 ↗
41. 10.1038/s41467-024-49447-y10.1038/s41467-024-49447-y ↗
42. 10.1103/PhysRevLett.82.241710.1103/PhysRevLett.82.2417 ↗
43. 10.1103/PhysRevB.93.20543410.1103/PhysRevB.93.205434 ↗
44. 10.1063/1.171629610.1063/1.1716296 ↗
45. 10.1103/PhysRev.94.63010.1103/PhysRev.94.630 ↗
46. 10.1126/science.abc518610.1126/science.abc5186 ↗
47. 10.1126/science.aad989810.1126/science.aad9898 ↗
48. 10.1103/PhysRevB.107.04542710.1103/PhysRevB.107.045427 ↗
49. 10.1038/s41557-021-00827-710.1038/s41557-021-00827-7 ↗
50. 10.1039/D2NH00375A10.1039/D2NH00375A ↗
51. 10.1126/science.adh475310.1126/science.adh4753 ↗
52. 10.1038/s41565-018-0296-710.1038/s41565-018-0296-7 ↗
53. Veldman, L. M.; Stolte, E. W.; Canavan, M. P.; Broekhoven, R.; Willke, P.; Farinacci, L.; Otte, S. Coherent spin dynamics between electron and nucleus within a single atom. arXiv, 2023, 2309.03749. https://arxiv.org/abs/2309.03749 (accessed 09 11, 2024).
54. 10.1021/acs.nanolett.2c0278210.1021/acs.nanolett.2c02782 ↗
55. 10.1021/acs.nanolett.2c0278310.1021/acs.nanolett.2c02783 ↗
56. 10.1126/science.124980210.1126/science.1249802 ↗
57. 10.1063/5.007813710.1063/5.0078137 ↗
58. 10.1038/s41467-023-42287-210.1038/s41467-023-42287-2 ↗
59. 10.1038/nature0416610.1038/nature04166 ↗
60. 10.1038/s41557-019-0232-y10.1038/s41557-019-0232-y ↗
61. 10.1103/PhysRevX.10.03105010.1103/PhysRevX.10.031050 ↗
62. 10.1021/acs.nanolett.2c0098010.1021/acs.nanolett.2c00980 ↗
63. 10.1021/acs.nanolett.2c0404910.1021/acs.nanolett.2c04049 ↗
64. 10.1063/5.004001110.1063/5.0040011 ↗
65. 10.1038/nphys225210.1038/nphys2252 ↗
66. 10.1038/nature0939210.1038/nature09392 ↗
67. 10.1038/nature0269310.1038/nature02693 ↗
68. 10.1038/s41534-024-00888-910.1038/s41534-024-00888-9 ↗
69. 10.1103/PhysRevB.108.11541310.1103/PhysRevB.108.115413 ↗
70. 10.1038/s41534-023-00781-x10.1038/s41534-023-00781-x ↗
71. 10.1038/s41586-020-2619-810.1038/s41586-020-2619-8 ↗
72. 10.1103/PhysRevLett.117.06050410.1103/PhysRevLett.117.060504 ↗
73. Löschnauer, C. M.; Toba, J. M.; Hughes, A. C.; King, S. A.; Weber, M. A.; Srinivas, R.; Matt, R.; Nourshargh, R.; Allcock, D. T. C.; Ballance, C. J.; Matthiesen, C.; Malinowski, M.; Harty, T. P. Scalable, high-fidelity all-electronic control of trapped-ion qubits. arXiv, 2024, 2407.07694. https://arxiv.org/abs/2407.07694 (accessed 09 11, 2024).
74. 10.1103/PhysRevLett.100.20050210.1103/PhysRevLett.100.200502 ↗
75. 10.1103/PhysRevLett.113.22050110.1103/PhysRevLett.113.220501 ↗
76. 10.1002/qute.20200000510.1002/qute.202000005 ↗
77. 10.1038/s41467-018-02982-x10.1038/s41467-018-02982-x ↗
78. 10.1038/s41586-019-1381-210.1038/s41586-019-1381-2 ↗