journal article·2025-06-10Open access

Strong In-plane Magnetic Anisotropy in Semiconducting Monolayer CoCl2

Samuel Kerschbaumer, Sebastien Elie Hadjadj, Andrea Aguirre-Baños, Danilo Longo, Andrés Pinar Solé, Oleksandr Stetsovych, Adriana Elizabet Candia, Paula Angulo-Portugal, David Caldevilla, Fadi Choueikani, Martina Corso, David Serrate, Jorge Lobo-Checa, Pavel Jelínek, Maxim Ilyn, Celia Rogero

ACS Nano· Volume 19· Issue 22

Abstract

High Resolution Image Download MS PowerPoint Slide Transition-metal dihalides (TMDH) are emerging as a highly promising class of 2D magnetic materials due to their simplicity, stability, and compatibility with nanofabrication techniques. In this work, we explore the structural, electronic, and magnetic properties of monolayer CoCl 2 grown epitaxially on Au(111) using a multitechnique approach. Our results reveal that epitaxial CoCl 2 exhibits ferromagnetic order below 24 K with strong in-plane magnetic anisotropy, setting it apart from other TMDH materials. Additionally, we identify in-gap states arising from the CoCl 2 –Au(111) interface, which provide insights into its electronic behavior. These findings position CoCl 2 as a versatile 2D material for spintronic applications and nanoscale devices, bridging the gap between fundamental research and real-world technological solutions.
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Research context

OpenAlex topics: 2D Materials and Applications · Perovskite Materials and Applications · MXene and MAX Phase Materials

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Affiliations

Centro de Física de Materiales (CSIC/UPV-EHU)

CIC nanoGUNE-BRTA

FZU – Institute of Physics of the Czech Academy of Sciences, Cukrovarnická 10, Prague 6 CZ 16200, Czech Republic

Laboratorio de Microscopias Avanzadas (LMA)

Universidad de Zaragoza

Synchrotron SOLEIL

Instituto de Nanociencia y Materiales de Aragón (INMA)

CSIC-Universidad de Zaragoza

Departamento de Física de la Materia Condensada

Funding

Consejo Superior de Investigaciones Cient?ficas · Gobierno de Arag?n · Agencia Estatal de Investigaci?n · Ikerbasque, Basque Foundation for Science · Grantov? Agentura Cesk? Republiky · H2020 Marie Sklodowska-Curie Actions · Eusko Jaurlaritza · Hezkuntza, Hizkuntza Politika Eta Kultura Saila, Eusko Jaurlaritza · NextGenerationEU

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