journal article·2025-01-28Open access

Shaping the Emission Directivity of Single Quantum Dots in Dielectric Nanodisks Exploiting Mie Resonances

Cristina Cruciano, Davide Rocco, Armando Genco, Andrea Tognazzi, Andrea Locatelli, Luca Carletti, Alexey Fedorov, Chiara Trovatello, Giuseppe Di Blasio, Ilaria Bargigia, Charalambos Louca, Paolo Gubian, Giulio Tavani, Luca Lovisolo, Artur Tuktamyshev, Lucio C. Andreani, Matteo Galli, Giulio Cerullo, Giuseppe Leo, Stefano Sanguinetti, Costantino De Angelis, Monica Bollani

ACS Nano· Volume 19· Issue 3

Abstract

Manipulating the optical landscape of single quantum dots (QDs) is essential to increase the emitted photon output, enhancing their performance as chemical sensors and single-photon sources. Micro-optical structures are typically used for this task, with the drawback of a large size compared to the embedded single emitters. Nanophotonic architectures hold the promise to modify dramatically the emission properties of QDs, boosting light-matter interactions at the nanoscale, in ultracompact devices. Here, we investigate the interplay between gallium arsenide (GaAs) single QDs and aluminum gallium arsenide (AlGaAs) nanostructures, capitalizing on the Kerker condition for precise control of the QD emission directivity. An extensive analysis of the photoluminescence spectra of several QDs embedded in nanodisks revealed a pronounced directivity enhancement due to the Kerker effect, confirmed by theoretical simulations, resulting in a 14-fold increase of emitted intensity. Angle-resolved spectroscopy experiments also proved that the integration of GaAs QDs within nanostructures determines a precise angled emission, offering a distinctive avenue for manipulating the spatial characteristics of emitted light by exploiting Mie resonances. This work contributes to the optimization of QD integration in nanostructures and suggests potential improvements for applications in optical communications.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Semiconductor Quantum Structures and Devices · Quantum Dots Synthesis And Properties · Plasmonic and Surface Plasmon Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, Politecnico of Milano, Piazza Leonardo Da Vinci 32, 20133 Milano, Italy

Department of Information Engineering, University of Brescia, via Branze 38, 25123 Brescia, Italy

Department of Engineering, University of Palermo, viale delle scienze 10, 90128Palermo, Italy

Institute of Photonics and of Nanotechnologies- National Researcher Council (IFN-CNR), LNESS Laboratory, Piazza Leonardo Da Vinci 32, 20133 Milano, Italy

Department of Physics, Cavendish Laboratory, JJ Thompson Avenue, CambridgeCB3 0HE,U.K.

Matériaux et Phénomènes Quantiques, Université Paris Cité and CNRS, 10 rue A. Domon et L. Duquet, 75013 Paris, France

Department of Material Science, University of Milano Bicocca, via Cozzi 55, 20126 Milano, Italy

Department of Physics, University of Pavia, via Bassi 6, I-27100 Pavia, Italy

Funding

HORIZON EUROPE European Innovation Council · European Commission · Università degli Studi di Palermo · H2020 Marie Sklodowska-Curie Actions · NextGenerationEU · PRIN 2022 PNRR · PNRR MUR

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