journal article·2025-03-18

Blackbody Radiation and Thermal Effects on Chemical Reactions and Phase Transitions in Cavities

Sindhana Pannir-Sivajothi, Joel Yuen-Zhou

ACS Nano· Volume 19· Issue 10
Publisher page

Abstract

An important question in polariton chemistry is whether reacting molecules are in thermal equilibrium with their surroundings. If not, can experimental changes observed in reaction rates of molecules in a cavity (even without optical pumping) be attributed to a higher/lower temperature inside the cavity? In this work, we address this question by computing the temperature differences between reacting molecules inside a cavity and the air outside. We found this temperature difference to be negligible for most reactions. On the other hand, for phase transitions inside cavities, as the temperature of the material is actively maintained by a heating/cooling source in experiments, we show that cavities can modify observed transition temperatures when mirrors and cavity windows are ideal (nonabsorbing); however, this modification vanishes when real mirrors and windows are used. This conclusion relies on having a low contact resistance between mirrors and molecules. Finally, we find substantial differences in blackbody spectral energy density between free space and infrared cavities, which reveal resonance effects and could potentially play a role in explaining changes in the chemical reactivity in the dark.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Strong Light-Matter Interactions · Thermal Radiation and Cooling Technologies · Quantum Electrodynamics and Casimir Effect

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemistry and Biochemistry

University of California San Diego

Funding

W. M. Keck Foundation

References (58)

Show source-provided references
1. 10.1002/anie.20160550410.1002/anie.201605504 ↗
2. 10.1126/science.aau774210.1126/science.aau7742 ↗
3. 10.1126/science.ade714710.1126/science.ade7147 ↗
4. 10.1002/anie.20190887610.1002/anie.201908876 ↗
5. 10.1002/anie.20191563210.1002/anie.201915632 ↗
6. 10.1021/acs.jpclett.0c0300310.1021/acs.jpclett.0c03003 ↗
7. 10.1002/anie.20190540710.1002/anie.201905407 ↗
8. 10.1039/C4NR01971G10.1039/C4NR01971G ↗
9. 10.1038/s41557-024-01723-610.1038/s41557-024-01723-6 ↗
10. 10.1038/s41586-023-06596-210.1038/s41586-023-06596-2 ↗
11. 10.1103/PhysRevX.5.04102210.1103/PhysRevX.5.041022 ↗
12. 10.1103/PhysRevLett.116.23830110.1103/PhysRevLett.116.238301 ↗
13. 10.1103/PhysRevLett.121.11300210.1103/PhysRevLett.121.113002 ↗
14. 10.1038/s41467-019-12636-110.1038/s41467-019-12636-1 ↗
15. 10.1038/s41467-021-21610-910.1038/s41467-021-21610-9 ↗
16. 10.1038/s41467-022-35363-610.1038/s41467-022-35363-6 ↗
17. 10.1021/acsphotonics.1c0174910.1021/acsphotonics.1c01749 ↗
18. 10.1021/acs.chemrev.2c0085510.1021/acs.chemrev.2c00855 ↗
19. 10.1063/5.014325310.1063/5.0143253 ↗
20. 10.1021/acs.chemrev.2c0078810.1021/acs.chemrev.2c00788 ↗
21. 10.1063/1.513632010.1063/1.5136320 ↗
22. 10.1063/5.009495610.1063/5.0094956 ↗
23. 10.1021/acs.jpclett.0c0084110.1021/acs.jpclett.0c00841 ↗
24. 10.1063/5.000754710.1063/5.0007547 ↗
25. 10.1016/j.chemphys.2020.11076710.1016/j.chemphys.2020.110767 ↗
26. 10.1063/5.000647210.1063/5.0006472 ↗
27. 10.22331/q-2020-09-28-33510.22331/q-2020-09-28-335 ↗
28. 10.1103/PhysRevLett.128.09600110.1103/PhysRevLett.128.096001 ↗
29. 10.1364/OPTICA.2.00002710.1364/OPTICA.2.000027 ↗
30. 10.1016/j.jqsrt.2017.01.01410.1016/j.jqsrt.2017.01.014 ↗
31. 10.1021/acsnano.3c0118410.1021/acsnano.3c01184 ↗
32. 10.1002/adma.20230939310.1002/adma.202309393 ↗
33. 10.1038/s42004-022-00660-010.1038/s42004-022-00660-0 ↗
34. 10.1515/nanoph-2023-068510.1515/nanoph-2023-0685 ↗
35. 10.1103/PhysRevLett.130.21360210.1103/PhysRevLett.130.213602 ↗
36. Ellingson S. W. · 2020 · 2
37. 10.1021/acsphotonics.8b0175610.1021/acsphotonics.8b01756 ↗
38. 10.1021/acsphotonics.7b0067710.1021/acsphotonics.7b00677 ↗
39. Kosky P. · 2020
40. Fletcher, L. In Thermal Conductance of Gasket Materials for Spacecraft Joints, 11th Aerospace Sciences Meeting; ARC, 1974; p 119.10.2514/6.1973-119 ↗
41. 10.1103/PhysRevLett.93.21390510.1103/PhysRevLett.93.213905 ↗
42. 10.1103/PhysRevB.70.12510110.1103/PhysRevB.70.125101 ↗
43. 10.1103/PhysRevA.59.473610.1103/PhysRevA.59.4736 ↗
44. 10.1364/AO.44.00753210.1364/AO.44.007532 ↗
45. 10.1177/000370281665756810.1177/0003702816657568 ↗
46. 10.1016/j.optmat.2017.06.05210.1016/j.optmat.2017.06.052 ↗
47. 10.1063/5.007754910.1063/5.0077549 ↗
48. 10.1063/5.004630710.1063/5.0046307 ↗
49. 10.1103/PhysRevB.86.23514710.1103/PhysRevB.86.235147 ↗
50. 10.1103/PhysRevA.87.03380110.1103/PhysRevA.87.033801 ↗
51. 10.1142/S021947752230001410.1142/S0219477522300014 ↗
52. 10.1063/5.007814810.1063/5.0078148 ↗
53. 10.1115/1.400354310.1115/1.4003543 ↗
54. 10.1103/PhysRevB.110.L16110710.1103/PhysRevB.110.L161107 ↗
55. Zangwill A. · 2013
56. Byrnes, S. J. Multilayer Optical Calculations. 2016, arXiv:1603.02720. arXiv.org e-Printarchive. https://arxiv.org/abs/1603.02720.
57. 10.1143/JJAP.50.12230110.1143/JJAP.50.122301 ↗
58. Pannir-Sivajothi, S.; Yuen-Zhou, J. Blackbody Radiation and Thermal Effects on Chemical Reactions and Phase Transitions in Cavities. 2024, arXiv:2402.01043. arXiv.org e-Printarchive. https://arxiv.org/abs/2402.01043. (accessed February 26, 2025).10.1021/acsnano.4c14590 ↗