Mechanisms of Symmetry Breaking in a Multidimensional Flashing Particle Ratchet
Source abstract
Abstract
Ratcheting is a mechanism that produces directional transport of particles by rectifying nondirectional energy using local asymmetries rather than a net bias in the direction of transport. In a flashing ratchet, an oscillating force (here, an AC field) is applied perpendicular to the direction of transport. In an effort to explore the properties of current experimentally realizable ratchet systems, and to design new ones, this paper describes classical simulations of a damped flashing ratchet that transports charged nanoparticles within a transport layer of finite, non-zero thickness. The thickness of the layer, and the decay of the applied field in the z-direction throughout that thickness, provide a mechanism of symmetry breaking in the system that allows the ratchet to produce directional transport using a temporally unbiased oscillation of the AC driving field, a sine wave. Sine waves are conveniently produced experimentally or harvested from natural sources but cannot produce transport in a 1D or pseudo-1D system. The sine wave drive produces transport velocities an order of magnitude higher than those produced by the common on/off drive, but lower than those produced by a temporally biased square wave drive (unequal durations of the positive and negative states). The dependence of the particle velocity on the thickness of the transport layer, and on the homogeneity of the oscillating field within the layer, is presented for all three driving schemes.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: stochastic dynamics and bifurcation · Spectroscopy and Quantum Chemical Studies · Photosynthetic Processes and Mechanisms
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Center for Bio-Inspired Energy Science, Northwestern University, 303 East Superior Street, 11th floor, Chicago, Illinois 60611-3015, United States
Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States
Funding
Basic Energy Sciences
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