journal article·2014-06-24

Air-Stable Electron Depletion of Bi2Se3 Using Molybdenum Trioxide into the Topological Regime

Mark T. Edmonds, Jack T. Hellerstedt, Anton Tadich, Alex Schenk, Kane Michael O’Donnell, Jacob Tosado, Nicholas P. Butch, Paul Syers, Johnpierre Paglione, Michael S. Fuhrer

ACS Nano· Volume 8· Issue 6
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Abstract

We perform high-resolution photoelectron spectroscopy on in situ cleaved topological insulator Bi2Se3 single crystals and in situ transport measurements on Bi2Se3 films grown by molecular beam epitaxy. We demonstrate efficient electron depletion of Bi2Se3 via vacuum deposition of molecular MoO3, lowering the surface Fermi energy to within ∼100 meV of the Dirac point, well into the topological regime. A 100 nm MoO3 film provides an air-stable doping and passivation layer.
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Research context

OpenAlex topics: Topological Materials and Phenomena · Graphene research and applications · Electronic and Structural Properties of Oxides

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Affiliations

School of Physics, Monash University, Clayton, VIC 3800, Australia

Center for Nanophysics and Advanced Materials, University of Maryland, College Park, Maryland 20742-4111, United States

Australian Synchrotron, Clayton, VIC 3168, Australia

Department of Physics, La Trobe University, Bundoora, VIC 3086, Australia

National Institute of Standards and Technology, Gaithersburg, Maryland 20899, United States

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