Anti-Stokes Raman Scattering of Single Carbyne Chains
Source abstract
Abstract
We investigate the anti-Stokes Raman scattering of single carbyne chains confined inside double-walled carbon nanotubes. Individual chains are identified using tip-enhanced Raman scattering (TERS) and heated by resonant excitation with varying laser powers. We study the temperature dependence of carbyne's Raman spectrum and quantify the laser-induced heating based on the anti-Stokes/Stokes ratio. Due to its molecular size and its large Raman cross section, carbyne holds great promise for local temperature monitoring, with potential applications ranging from nanoelectronics to biology.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Carbon Nanotubes in Composites · Thermal properties of materials · Graphene research and applications
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Photonics Laboratory, ETH Zürich, 8093 Zürich, Switzerland
Department of Physics, Freie Universität Berlin, 14195 Berlin, Germany
Materials Metrology Division, Instituto Nacional de Metrologia Qualidade e Tecnologia (INMETRO), 25250-020 Duque de Caxias, RJ, Brazil
School of Materials Science and Engineering, State Key Laboratory of Optoelectronic Materials and Technologies, Nanotechnology Research Center, Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices, Sun Yat-sen University, Guangzhou 510275, P. R. China
Faculty of Physics, Universität Wien, 1090 Wien, Austria
Department of Physics, Humboldt Universität zu Berlin, 12489 Berlin, Germany
Funding
Minist??rio da Ci??ncia, Tecnologia e Inova????o · Schweizerischer Nationalfonds zur F??rderung der Wissenschaftlichen Forschung · Deutsche Forschungsgemeinschaft · Conselho Nacional de Desenvolvimento Cient??fico e Tecnol??gico · National Natural Science Foundation of China · Natural Science Foundation of Guangdong Province
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