journal article·2017-06-27Open access

Probing Gap Plasmons Down to Subnanometer Scales Using Collapsible Nanofingers

Boxiang Song, Yuhan Yao, Roelof E. Groenewald, Yunxiang Wang, He Liu, Yifei Wang, Yuanrui Li, Fanxin Liu, Stephen B. Cronin, Adam M. Schwartzberg, Stefano Cabrini, Stephan Haas, Wei Wu

ACS Nano· Volume 11· Issue 6

Abstract

Gap plasmonic nanostructures are of great interest due to their ability to concentrate light into small volumes. Theoretical studies, considering quantum mechanical effects, have predicted the optimal spatial gap between adjacent nanoparticles to be in the subnanometer regime in order to achieve the strongest possible field enhancement. Here, we present a technology to fabricate gap plasmonic structures with subnanometer resolution, high reliability, and high throughput using collapsible nanofingers. This approach enables us to systematically investigate the effects of gap size and tunneling barrier height. The experimental results are consistent with previous findings as well as with a straightforward theoretical model that is presented here.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Plasmonic and Surface Plasmon Research · Gold and Silver Nanoparticles Synthesis and Applications · Orbital Angular Momentum in Optics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Ming Hsieh Department of Electrical Engineering, University of Southern California, Los Angeles, California 90089, United States

Department of Physics and Astronomy, University of Southern California, Los Angeles, California 90089, United States

Department of Applied Physics, Zhejiang University of Technology, Hangzhou, Zhejiang 310023, China

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States

Funding

Air Force Office of Scientific Research · U.S. Department of Energy · Division of Civil, Mechanical and Manufacturing Innovation · National Natural Science Foundation of China · Natural Science Foundation of Zhejiang Province

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