journal article·2024-08-20Open access

Picosecond Femtojoule Resistive Switching in Nanoscale VO2 Memristors

Sebastian Werner Schmid, László Pósa, Tímea Nóra Török, Botond Sánta, Zsigmond Pollner, György Molnár, Yannik Horst, János Volk, Juerg Leuthold, András Halbritter, Miklós Csontos

ACS Nano· Volume 18· Issue 33

Abstract

High Resolution Image Download MS PowerPoint Slide Beyond-Moore computing technologies are expected to provide a sustainable alternative to the von Neumann approach not only due to their down-scaling potential but also via exploiting device-level functional complexity at the lowest possible energy consumption. The dynamics of the Mott transition in correlated electron oxides, such as vanadium dioxide, has been identified as a rich and reliable source of such functional complexity. However, its full potential in high-speed and low-power operation has been largely unexplored. We fabricated nanoscale VO 2 devices embedded in a broadband test circuit to study the speed and energy limitations of their resistive switching operation. Our picosecond time-resolution, real-time resistive switching experiments and numerical simulations demonstrate that tunable low-resistance states can be set by the application of 20 ps long, <1.7 V amplitude voltage pulses at 15 ps incubation times and switching energies starting from a few femtojoule. Moreover, we demonstrate that at nanometer-scale device sizes not only the electric field induced insulator-to-metal transition but also the thermal conduction limited metal-to-insulator transition can take place at time scales of 100s of picoseconds. These orders of magnitude breakthroughs can be utilized to design high-speed and low-power dynamical circuits for a plethora of neuromorphic computing applications from pattern recognition to numerical optimization.
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Research context

OpenAlex topics: Advanced Memory and Neural Computing · Transition Metal Oxide Nanomaterials · Photoreceptor and optogenetics research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, Institute of Physics, Budapest University of Technology and Economics, Műegyetem rkp. 3, H-1111 Budapest, Hungary

Experimental Physics V, Center for Electronic Correlations and Magnetism, University of Augsburg, Augsburg 86159, Germany

Institute of Technical Physics and Materials Science, HUN-REN Centre for Energy Research, Konkoly-Thege M. út 29-33, 1121 Budapest, Hungary

HUN-REN-BME Condensed Matter Research Group, Műegyetem rkp. 3, H-1111 Budapest, Hungary

Institute of Electromagnetic Fields, ETH Zurich, Gloriastrasse 35, 8092 Zürich, Switzerland

Funding

Werner Siemens-Stiftung · Magyar Tudományos Akadémia · Nemzeti Kutatási Fejlesztési és Innovációs Hivatal

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