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journal article·2025-01Open access

Isomerization of Covalent Organic Frameworks for Efficiently Activating Molecular Oxygen and Promoting Hydrogen Peroxide Photosynthesis (Small 3/2025)

Wenjiao Wang, Rui Zhang, Hongqi Chu, Zhen Zhan, Qi Huang, Zhenzi Li, Xuepeng Wang, Fuquan Bai, Wei Zhou

Small· Volume 21· Issue 3
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Source abstract

Abstract

Covalent Organic Frameworks For a pair of isomeric covalent organic frameworks (COFs), different rate determining steps were proved in the generation process of H2O2. PB-PT-COF showed strong interaction with H2O, facilitating the direct oxidation of H2O (H2O + h+→H2O2), while PT-PB-COF exhibited effective O2 adsorption and activation (O2 + e- → •O2− + e− → H2O2), resulting in a twofold enhancement in the H2O2 photosynthesis. More in article number 2406527, Xuepeng Wang, Fuquan Bai, Wei Zhou, and co-workers.
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Research context

OpenAlex topics: Chemical Synthesis and Reactions · Covalent Organic Framework Applications · Oxidative Organic Chemistry Reactions

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Affiliations

Shandong Provincial Key Laboratory of Molecular Engineering School of Chemistry and Chemical Engineering Qilu University of Technology (Shandong Academy of Sciences) Jinan Shandong 250353 P. R. China

Institute of Theoretical Chemistry and College of Chemistry Jilin University Changchun Jilin Province 130021 P. R. China

Department of Applied Physics The Hong Kong Polytechnic University Hong Kong 999077 P. R. China

School of Engineering The University of Edinburgh Robert Stevenson Road Edinburgh EH93JL UK

References

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