Photoinduced Phase Transition in Infinite‐Layer Nickelates
Source abstract
Abstract
Abstract The quantum phase transition caused by regulating the electronic correlation in strongly correlated quantum materials has been a research hotspot in condensed matter science. Herein, a photon‐induced quantum phase transition from the Kondo‐Mott insulating state to the low temperature metallic one accompanying with the magnetoresistance changing from negative to positive in the infinite‐layer NdNiO2 films is reported, where the antiferromagnetic coupling among the Ni1+ localized spins and the Kondo effect are effectively suppressed by manipulating the correlation of Ni‐3d and Nd‐5d electrons under the photoirradiation. Moreover, the critical temperature Tc of the superconducting‐like transition exhibits a dome‐shaped evolution with the maximum up to ≈42 K, and the electrons dominate the transport process proved by the Hall effect measurements. These findings not only make the photoinduction a promising way to control the quantum phase transition by manipulating the electronic correlation in Mott‐like insulators, but also shed some light on the possibility of the superconducting in electron‐doped nickelates.
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Research context
OpenAlex topics: Magnetic and transport properties of perovskites and related materials · Electronic and Structural Properties of Oxides · Advanced Condensed Matter Physics
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences Beijing 100190 China
University of Chinese Academy of Science Beijing 100049 China
Songshan Lake Materials Laboratory Dongguan Guangdong 523808 China
Key Laboratory of Magnetic Materials and Devices and Zhejiang Province Key Laboratory of Magnetic Materials and Application Technology Ningbo Institute of Materials Technology and Engineering (NIMTE) Chinese Academy of Sciences Ningbo 315201 China
State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano‐optoelectronics School of Physics Peking University Beijing 100871 China
Funding
National Natural Science Foundation of China · Youth Innovation Promotion Association of the Chinese Academy of Sciences · China Postdoctoral Science Foundation
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