journal article·2025-01Open access

Deciphering the Impact of Current, Composition, and Potential on the Lithiation Behavior of Si‐Rich Silicon‐Graphite Anodes (Small 4/2025)

Philipp Schweigart, Weicheng Hua, Pedro Alonso Sánchez, Camilla Lian, Inger‐Emma Nylund, David Wragg, Samson Yuxiu Lai, Federico Cova, Ann Mari Svensson, Maria Valeria Blanco

Small· Volume 21· Issue 4

Abstract

Lithium-Ion Batteries In article number 2406615 Philipp Schweigart, Ann Mari Svensson, Maria Valeria Blanco, and co-workers employ operando X-ray diffraction to unveil the complex lithiation and delithiation dynamics of silicon-graphite anodes with high silicon content. It investigates the competing processes of graphite lithiation, silicon amorphization, and Li15Si4 formation. Understanding the critical impact of electrode composition, lower cutoff potential, and applied current is key to optimizing operating conditions for advanced silicon-graphite anodes in lithium-ion batteries.
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Research context

OpenAlex topics: Advancements in Battery Materials · Recycling and Waste Management Techniques · Extraction and Separation Processes

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Affiliations

Department of Materials Science and Engineering Norwegian University of Science and Technology (NTNU) Sem Sælands Vei 12 Trondheim 7034 Norway

Department of Condensed Matter Physics Faculty of Sciences Aragón Nanoscience and Materials Institute (CSIC – University of Zaragoza) C/Pedro Cerbuna 12 Zaragoza 50009 Spain

Battery Technology Department Institute for Energy Technology (IFE) Instituttveien 18 Kjeller 2007 Norway

BL31 FaXToR Beamline CELLS‐ ALBA Synchrotron Light Source Cerdanyola del Vallès Barcelona 08290 Spain

References

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