Exotic Magnetic Anisotropy Near Digitized Dimensional Mott Boundary

Abstract The magnetic anisotropy of low‐dimensional Mott systems exhibits unexpected magnetotransport behavior useful for spin‐based quantum electronics. Yet, the anisotropy of natural materials is inherently determined by the crystal structure, highly limiting its engineering. The magnetic anisotropy modulation near a digitized dimensional Mott boundary in artificial superlattices composed of a correlated magnetic monolayer SrRuO₃ and nonmagnetic SrTiO₃, is demonstrated. The magnetic anisotropy is initially engineered by modulating the interlayer coupling strength between the magnetic monolayers. Interestingly, when the interlayer coupling strength is maximized, a nearly degenerate state is realized, in which the anisotropic magnetotransport is strongly influenced by both the thermal and magnetic energy scales. The results offer a new digitized control for magnetic anisotropy in low‐dimensional Mott systems, inspiring promising integration of Mottronics and spintronics.