journal article·2023-08-22

Ti3C2Tx MXene-Based Multifunctional Tactile Sensors for Precisely Detecting and Distinguishing Temperature and Pressure Stimuli

Fu-Lin Gao, Ji Liu, Xiao-Peng Li, Qian Ma, Tingting Zhang, Zhong-Zhen Yu, Jie Shang, Run-Wei Li, Xiaofeng Li

ACS Nano· Volume 17· Issue 16
Publisher page

Abstract

Although skin-like sensors that can simultaneously detect various physical stimuli are of fair importance in cutting-edge human–machine interaction, robotic, and healthcare applications, they still face challenges in facile, scalable, and cost-effective production using conventional active materials. The emerging two-dimensional transition metal carbide, Ti 3 C 2 T x MXene, integrated with favorable thermoelectric properties, metallic-like conductivity, and a hydrophilic surface, is promising for solving these problems. Herein, skin-like multifunctional sensors are designed to precisely detect and distinguish temperature and pressure stimuli without cross-talk by decorating elastic and porous substrates with MXene sheets. Because the combination of the thermoelectric and conductive MXene with the thermally insulating, elastic, and porous substrate integrates efficient Seebeck and piezoresistive effects, the resultant sensor exhibits not only an ultralow detection limit (0.05 K), high signal-to-noise ratio, and excellent cycling stability for temperature detection but also high sensitivity, fast response time, and outstanding durability for pressure detection. Based on the impressive dual-mode sensing properties and independent temperature and pressure detections, a multimode input terminal and an electronic skin are created, exhibiting great potential in robotic and human–machine interaction applications. This work provides a scalable fabrication of multifunctional tactile sensors for precisely detecting and distinguishing temperature and pressure stimuli.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: MXene and MAX Phase Materials · Advanced Sensor and Energy Harvesting Materials · 2D Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

State Key Laboratory of Organic−Inorganic Composites, College of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, China

Beijing Key Laboratory of Advanced Functional Polymer Composites, Beijing University of Chemical Technology, Beijing 100029, China

School of Chemistry, CRANN and AMBER, Trinity College Dublin, Dublin 2, Ireland

State Key Laboratory of NBC Protection for Civilian, Institute of Chemical Defense, Beijing 100191, China

State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing 100029, China

CAS Key Laboratory of Magnetic Materials and Devices, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China

Funding

National Natural Science Foundation of China

References (75)

Show source-provided references
1. 10.1002/inf2.1206010.1002/inf2.12060 ↗
2. 10.1002/adma.20190476510.1002/adma.201904765 ↗
3. 10.1038/s41467-022-33454-y10.1038/s41467-022-33454-y ↗
4. 10.1038/s41467-022-33716-910.1038/s41467-022-33716-9 ↗
5. 10.1002/adma.20220536910.1002/adma.202205369 ↗
6. 10.1002/adfm.20221490710.1002/adfm.202214907 ↗
7. 10.1021/acs.nanolett.0c0251910.1021/acs.nanolett.0c02519 ↗
8. 10.1038/ncomms935610.1038/ncomms9356 ↗
9. 10.1002/adfm.20170354910.1002/adfm.201703549 ↗
10. 10.1002/advs.20180212810.1002/advs.201802128 ↗
11. 10.1039/D0TA05651K10.1039/D0TA05651K ↗
12. 10.1021/acsami.2c1289210.1021/acsami.2c12892 ↗
13. 10.1002/adma.20150536410.1002/adma.201505364 ↗
14. 10.1126/sciadv.abb908310.1126/sciadv.abb9083 ↗
15. 10.1021/acs.nanolett.0c0425210.1021/acs.nanolett.0c04252 ↗
16. 10.1021/acs.nanolett.2c0069610.1021/acs.nanolett.2c00696 ↗
17. 10.1016/j.cej.2021.13019710.1016/j.cej.2021.130197 ↗
18. 10.1002/smm2.103410.1002/smm2.1034 ↗
19. 10.1021/acsnano.1c0738810.1021/acsnano.1c07388 ↗
20. 10.1021/acs.chemrev.1c0021810.1021/acs.chemrev.1c00218 ↗
21. 10.1016/j.pmatsci.2017.09.00410.1016/j.pmatsci.2017.09.004 ↗
22. 10.1021/nn204153h10.1021/nn204153h ↗
23. 10.1016/j.cej.2021.13147210.1016/j.cej.2021.131472 ↗
24. 10.1002/adma.20210856010.1002/adma.202108560 ↗
25. 10.1002/adfm.20210885610.1002/adfm.202108856 ↗
26. 10.1002/adfm.20221119910.1002/adfm.202211199 ↗
27. 10.1002/adma.20110230610.1002/adma.201102306 ↗
28. 10.1126/science.abf158110.1126/science.abf1581 ↗
29. 10.1021/acsnano.1c0047210.1021/acsnano.1c00472 ↗
30. 10.1021/acsnano.1c0024810.1021/acsnano.1c00248 ↗
31. 10.1021/acsnano.2c0764610.1021/acsnano.2c07646 ↗
32. 10.1021/acsnano.1c0823910.1021/acsnano.1c08239 ↗
33. 10.1021/acsnano.1c0992510.1021/acsnano.1c09925 ↗
34. 10.1002/adma.20211060810.1002/adma.202110608 ↗
35. 10.1021/acsnano.2c0315510.1021/acsnano.2c03155 ↗
36. 10.1039/D3TA00403A10.1039/D3TA00403A ↗
37. 10.1039/C7NR09144C10.1039/C7NR09144C ↗
38. 10.1016/j.jallcom.2020.15463410.1016/j.jallcom.2020.154634 ↗
39. 10.1021/acsami.9b2118510.1021/acsami.9b21185 ↗
40. 10.1039/D1TA00331C10.1039/D1TA00331C ↗
41. 10.1002/adfm.20211053410.1002/adfm.202110534 ↗
42. 10.1016/j.ensm.2022.12.03610.1016/j.ensm.2022.12.036 ↗
43. 10.1021/acsami.9b2274410.1021/acsami.9b22744 ↗
44. 10.1002/adfm.20210138110.1002/adfm.202101381 ↗
45. 10.1021/acsnano.2c0993310.1021/acsnano.2c09933 ↗
46. 10.1021/acs.nanolett.2c0114510.1021/acs.nanolett.2c01145 ↗
47. 10.1039/C9TA09225K10.1039/C9TA09225K ↗
48. 10.1021/acsnano.1c0316110.1021/acsnano.1c03161 ↗
49. 10.1016/j.nanoen.2017.11.04410.1016/j.nanoen.2017.11.044 ↗
50. 10.1039/D1MH00968K10.1039/D1MH00968K ↗
51. 10.1002/smll.20220612610.1002/smll.202206126 ↗
52. 10.1016/j.ensm.2022.05.03310.1016/j.ensm.2022.05.033 ↗
53. 10.1002/adma.20210314810.1002/adma.202103148 ↗
54. 10.1016/j.cej.2023.14133910.1016/j.cej.2023.141339 ↗
55. 10.1016/j.carbpol.2019.03.07710.1016/j.carbpol.2019.03.077 ↗
56. 10.1016/j.cej.2022.13625510.1016/j.cej.2022.136255 ↗
57. 10.1002/adfm.20221161310.1002/adfm.202211613 ↗
58. 10.1016/j.cej.2022.13570610.1016/j.cej.2022.135706 ↗
59. 10.1021/acsami.2c0500310.1021/acsami.2c05003 ↗
60. 10.1016/j.cej.2021.13315810.1016/j.cej.2021.133158 ↗
61. 10.1039/D2TA04862K10.1039/D2TA04862K ↗
62. 10.1038/s41467-019-12030-x10.1038/s41467-019-12030-x ↗
63. 10.1021/acsnano.0c0067210.1021/acsnano.0c00672 ↗
64. 10.1016/j.cej.2022.13971610.1016/j.cej.2022.139716 ↗
65. 10.1021/acsnano.2c0426010.1021/acsnano.2c04260 ↗
66. 10.1039/D1TA08521B10.1039/D1TA08521B ↗
67. 10.1016/j.nanoen.2021.10615110.1016/j.nanoen.2021.106151 ↗
68. 10.1016/j.jmst.2022.09.05010.1016/j.jmst.2022.09.050 ↗
69. 10.1002/eom2.1229910.1002/eom2.12299 ↗
70. 10.1016/j.xcrp.2022.10105010.1016/j.xcrp.2022.101050 ↗
71. 10.1146/annurev-matsci-062910-10044510.1146/annurev-matsci-062910-100445 ↗
72. 10.1002/adfm.20220480310.1002/adfm.202204803 ↗
73. 10.1021/acsnano.2c0154810.1021/acsnano.2c01548 ↗
74. 10.1021/acsnano.2c0131010.1021/acsnano.2c01310 ↗
75. 10.1021/acssensors.0c0087010.1021/acssensors.0c00870 ↗