journal article·2025-09Open access

Enabling carbon dioxide mineralization and active set control in portlandite-based cementitious suspensions

Xiaodi Dai, Sharu Bhagavathi Kandy, Rui Xiao, Manas Sarkar, Shubham Wani, Thiyagarajan Ranganathan, Narayanan Neithalath, Aditya Kumar, Mathieu Bauchy, Edward Garboczi, Torben Gädt, Samanvaya Srivastava, Gaurav Sant

Abstract

No abstract is available for this record. The assistant can identify its topic from the title, but cannot infer the study’s results.

Source: Not provided · Quality: missing

Research context

OpenAlex topics: Concrete and Cement Materials Research · Innovations in Concrete and Construction Materials · Magnesium Oxide Properties and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (76)

Show source-provided references
1. Readily implementable techniques can cut annual CO2 emissions from the production of concrete by over 20%10.1088/1748-9326/11/7/074029 ↗
2. Alkali-activated materials10.1016/j.cemconres.2017.02.009 ↗
3. Geopolymers and related alkali-activated materials10.1146/annurev-matsci-070813-113515 ↗
4. Recent progress in low-carbon binders10.1016/j.cemconres.2019.05.009 ↗
5. Rheological and mechanical properties of 3D printable alkali-activated slag mixtures with addition of nano clay10.1016/j.cemconcomp.2023.104995 ↗
6. Early age hydration of calcium sulfoaluminate (synthetic ye’elimite, C 4A3S) in the presence of gypsum and varying amounts of calcium hydroxide10.1016/j.cemconres.2013.03.001 ↗
7. Alternative cement clinkers10.1016/j.cemconres.2017.02.002 ↗
8. A review of alternative approaches to the reduction of CO2 emissions associated with the manufacture of the binder phase in concrete10.1016/j.cemconres.2015.04.012 ↗
9. Hydration studies of calcium sulfoaluminate cements blended with fly ash10.1016/j.cemconres.2013.07.010 ↗
10. Carbonation behavior of hydraulic and non-hydraulic calcium silicates: potential of utilizing low-lime calcium silicates in cement-based materials10.1007/s10853-016-9909-4 ↗
11. Strength and microstructure of CO2 cured low-calcium clinker10.1016/j.conbuildmat.2018.08.134 ↗
12. Clinkering-free cementation by fly ash carbonation10.1016/j.jcou.2017.11.005 ↗
13. Recent advances in carbonatable binders10.1016/j.cemconres.2023.107286 ↗
14. Carbonation activated binders from pure calcium silicates: reaction kinetics and performance controlling factors10.1016/j.cemconcomp.2018.07.004 ↗
15. Effect of pre-conditioning on CO2 curing of lightweight concrete blocks mixtures10.1016/j.conbuildmat.2011.06.020 ↗
16. Effect of pulverized fuel ash and CO2 curing on the water resistance of magnesium oxychloride cement (MOC)10.1016/j.cemconres.2017.03.005 ↗
17. High-strength KOBM steel slag binder activated by carbonation10.1016/j.conbuildmat.2015.09.028 ↗
18. Alcohol dispersions of calcium hydroxide nanoparticles for stone conservation10.1021/la4017728 ↗
19. New insights into the mechanisms of carbon dioxide mineralization by portlandite10.1002/aic.17160 ↗
20. Direct carbonation of Ca(OH)2 using liquid and supercritical CO2: implications for carbon-neutral cementation10.1021/acs.iecr.5b02356 ↗
21. How microstructure and pore moisture affect strength gain in portlandite-enriched composites that mineralize CO210.1021/acssuschemeng.9b02163 ↗
22. The role of gas flow distributions on CO2mineralization within monolithic cemented composites: Coupled CFD-factorial design approach10.1039/D0RE00433B ↗
23. Calcination-free production of calcium hydroxide at sub-boiling temperatures10.1039/D0RA08449B ↗
24. E. National Academies of Sciences, Gaseous Carbon Waste Streams Utilization : Status and Research Needs, n.d.
25. Vision of 3D printing with concrete — technical , economic and environmental potentials10.1016/j.cemconres.2018.06.001 ↗
26. Stiffening control of cement-based materials using accelerators in inline mixing processes: possibilities and challenges10.1016/j.cemconcomp.2021.103972 ↗
27. Set-on-demand of alkali-activated slag mixture using twin-pipe pumping10.1016/j.conbuildmat.2023.132003 ↗
28. Temperature-induced aggregation in portlandite suspensions10.1021/acs.langmuir.0c01798 ↗
29. N.S. Martys, C.F. Ferraris, V. Gupta, J.H. Cheung, J.G. Hagedorn, A.P. Peskin, E.J. Garboczi, Computational Model Predictions of Suspension Rheology: Comparison to Experiment, n.d.
30. Rheology, early-age hydration and microstructure of alkali-activated GGBFS-Fly ash-limestone mixtures10.1016/j.cemconcomp.2021.104244 ↗
31. Standard Specification for Coal Fly Ash and Raw or Calcined Natural Pozzolan for Use in Concrete, ASTM C618 (n.d.). https://doi.org/10.1520/C0618-19.10.1520/C0618-19 ↗
32. Ultrafast stiffening of concentrated thermoresponsive mineral suspensions10.1016/j.matdes.2022.110905 ↗
33. Rheology and structural build-up of sodium silicate- and sodium hydroxide-activated GGBFS mixtures10.1016/j.cemconcomp.2022.104570 ↗
34. Flow properties of MK-based geopolymer pastes. A comparative study with standard Portland cement pastes10.1039/c3sm51889b ↗
35. Influence of water to binder ratio on the rheology and structural Build-up of Alkali-Activated Slag/Fly ash mixtures10.1016/j.conbuildmat.2020.120253 ↗
36. Effect of relative humidity on the carbonation rate of portlandite, calcium silicate hydrates and ettringite10.1016/j.cemconres.2020.106116 ↗
37. Carbonation of CH and C-S-H in composite cement pastes containing high amounts of BFS10.1016/j.cemconres.2009.10.020 ↗
38. Rilem tc - 238 SCM Recommendation on hydration stoppage by solvent exchange for the study of hydrate assemblages
39. Thermally stimulated stiffening and fly ash's alkaline activation by Ca(OH)2 addition facilitates 3D-printing10.1016/j.cemconcomp.2024.105870 ↗
40. FullControl GCode Designer: open-source software for unconstrained design in additive manufacturing
41. 3D printable concrete: mixture design and test methods10.1016/j.cemconcomp.2018.12.014 ↗
42. 3D printing geopolymers: a review10.1016/j.cemconcomp.2022.104455 ↗
43. 3D printing using concrete extrusion: a roadmap for research10.1016/j.cemconres.2018.05.006 ↗
44. Recent advances on yield stress and elasticity of fresh cement-based materials10.1016/j.cemconres.2019.105798 ↗
45. The origins of thixotropy of fresh cement pastes10.1016/j.cemconres.2011.09.004 ↗
46. Dispersing nano- A nd micro-sized portlandite particulates: via electrosteric exclusion at short screening lengths10.1039/D0SM00045K ↗
47. The rheological properties of ternary binders containing Portland cement, limestone, and metakaolin or fly ash10.1016/j.cemconres.2013.07.007 ↗
48. Effect of fly ash microsphere on the rheology and microstructure of alkali-activated fly ash/slag pastes10.1016/j.cemconres.2018.04.008 ↗
49. Yodel: a yield stress model for suspensions10.1111/j.1551-2916.2005.00888.x ↗
50. 3D printing using concrete extrusion: a roadmap for research10.1016/j.cemconres.2018.05.006 ↗
51. Steady state flow of cement suspensions: a micromechanical state of the art10.1016/j.cemconres.2009.08.026 ↗
52. Munk · 2002
53. Viscosity transition from dilute to concentrated cementitious suspensions: the effect of colloidal interactions and flocs percolation
54. Observations on the rheological response of alkali activated fly ash suspensions: the role of activator type and concentration10.1007/s00397-014-0793-z ↗
55. Evolution of elastic behavior of alite paste at early hydration stages10.1111/jace.17354 ↗
56. Electrosteric control of the aggregation and yielding behavior of concentrated portlandite suspensions10.1021/acs.langmuir.3c00704 ↗
57. Brandrup · 1999
58. Kinetics of surface-initiated atom transfer radical polymerization of acrylamide on silica10.1021/ma011313x ↗
59. Controlled/living radical polymerization in dispersed systems10.1021/cr800242x ↗
60. Fly ash-Ca(OH)2Reactivity in hypersaline NaCl and CaCl2Brines10.1021/acssuschemeng.1c01884 ↗
61. Fly ash effects: II. The active effect of fly ash10.1016/j.cemconres.2003.03.001 ↗
62. Activation of fly ash cementitious systems in the presence of quicklime: Part I. Compressive strength and pozzolanic reaction rate10.1016/j.cemconres.2003.08.008 ↗
63. Effect of temperature on the hydration of Portland cement blended with siliceous fly ash10.1016/j.cemconres.2013.07.006 ↗
64. Activation of the fly ash pozzolanic reaction by hydrothermal conditions10.1016/S0008-8846(03)00085-1 ↗
65. Carbonation, strength development, and characterization of calcined limestone as a potential construction material10.1016/j.cemconres.2020.106263 ↗
66. Investigation of the carbonation front shape on cementitious materials: effects of the chemical kinetics10.1016/j.cemconres.2007.04.002 ↗
67. Measurement methods of carbonation profiles in concrete: thermogravimetry, chemical analysis and gammadensimetry10.1016/j.cemconres.2007.04.015 ↗
68. Role of calcium hydroxide in the alkaline activation of coal fly ash10.1016/j.cemconcomp.2022.104925 ↗
69. Role of calcium hydroxide in the alkaline activation of coal fly ash10.1016/j.cemconcomp.2022.104925 ↗
70. Pore structure characterization of cement pastes blended with high-volume fly-ash10.1016/j.cemconres.2011.09.012 ↗
71. Effect of polyacrylamide on the carbonation behavior of cement paste10.1016/j.cemconres.2022.106756 ↗
72. Rheological requirements for printable concretes10.1016/j.cemconres.2018.04.005 ↗
73. Extrusion-based additive manufacturing with cement-based materials – production steps, processes, and their underlying physics: a review10.1016/j.cemconres.2020.106037 ↗
74. A dual binder concept for 3D printing ink: Triggered polymerization for rapid stiffening and carbonation for final strength10.1016/j.matdes.2025.113598 ↗
75. G. Sant; S. B. kandy; T. Gädt; I. Mehdipour; T. Ranganathan; S. Srivastava; P. Seiler;, Thermoresponsvie suspension composites for 3D printing, US11951682, 2024.
76. Design and function of thermoresponsive-ultrafast stiffening suspension formulations for 3D printing10.1016/j.cemconcomp.2024.105905 ↗