journal article·2021-03-23Open access

Alignment of Cellulose Nanofibers: Harnessing Nanoscale Properties to Macroscale Benefits

Kai Li, Caitlyn M. Clarkson, Lu Wang, Yu Liu, Meghan Lamm, Zhenqian Pang, Yubing Zhou, Ji Qian, Mehdi Tajvidi, Douglas J. Gardner, Halil Tekinalp, Liangbing Hu, Teng Li, Arthur J. Ragauskas, Jeffrey P Youngblood, Soydan Ozcan

ACS Nano· Volume 15· Issue 3

Abstract

In nature, cellulose nanofibers form hierarchical structures across multiple length scales to achieve high-performance properties and different functionalities. Cellulose nanofibers, which are separated from plants or synthesized biologically, are being extensively investigated and processed into different materials owing to their good properties. The alignment of cellulose nanofibers is reported to significantly influence the performance of cellulose nanofiber-based materials. The alignment of cellulose nanofibers can bridge the nanoscale and macroscale, bringing enhanced nanoscale properties to high-performance macroscale materials. However, compared with extensive reviews on the alignment of cellulose nanocrystals, reviews focusing on cellulose nanofibers are seldom reported, possibly because of the challenge of aligning cellulose nanofibers. In this review, the alignment of cellulose nanofibers, including cellulose nanofibrils and bacterial cellulose, is extensively discussed from different aspects of the driving force, evaluation, strategies, properties, and applications. Future perspectives on challenges and opportunities in cellulose nanofiber alignment are also briefly highlighted.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Advanced Cellulose Research Studies · Electrospun Nanofibers in Biomedical Applications · Surface Modification and Superhydrophobicity

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Chemical Sciences Division, Oak Ridge National Laboratory, 1 Bethel Valley Road, Oak Ridge, Tennessee 37831, United States

Materials and Manufacturing Directorate, Air Force Research Laboratory, Wright-Patterson AFB, Ohio 45433, United States

School of Forest Resources, University of Maine, 5755 Nutting Hall, Orono, Maine 04469, United States

Advanced Structures and Composites Center, University of Maine, 35 Flagstaff Road, Orono, Maine 04469, United States

Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742, United States

Manufacturing Demonstration Facility, Manufacturing Science Division, Oak Ridge National Laboratory, 2350 Cherahala Boulevard, Knoxville, Tennessee 37932, United States

Department of Mechanical Engineering, University of Maryland, College Park, Maryland 20742, United States

Department of Chemical and Biomolecular Engineering, University of Tennessee, Knoxville, Tennessee 37996, United States

Department of Forestry, Wildlife, and Fisheries, Center for Renewable Carbon, The University of Tennessee Institute of Agriculture, Knoxville, Tennessee 37996, United States

UTK-ORNL Joint Institute for Biological Science, Biosciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United States

School of Materials Engineering, Purdue University, West Lafayette, Indiana 47907, United States

Funding

Oak Ridge National Laboratory · National Science Foundation

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