journal article·2015-01-27

Experimental and Theoretical Evidence of an Axially Chiral Borospherene

Qiang Chen, Wei-Li Li, Ya-Fan Zhao, Su-Yan Zhang, Han-Shi Hu, Hui Bai, Hai-Ru Li, Wen-Juan Tian, Hai-Gang Lu, Hua-Jin Zhai, Si-Dian Li, Jun Li, Lai-Sheng Wang

ACS Nano· Volume 9· Issue 1
Publisher page

Abstract

Chirality plays an important role in chemistry, biology, and materials science. The recent discovery of the B40(-/0) borospherenes marks the onset of a class of boron-based nanostructures. Here we report the observation of axially chiral borospherene in the B(39)(-) nanocluster on the bases of photoelectron spectroscopy, global minimum searches, and electronic structure calculations. Extensive structural searches in combination with density functional and CCSD(T) calculations show that B(39)(-) has a C3 cage global minimum with a close-lying C2 cage isomer. Both the C3 and C2 B(39)(-) cages are chiral with degenerate enantiomers. The C3 global minimum consists of three hexagons and three heptagons around the vertical C3 axis. The C2 isomer is built on two hexagons on the top and at the bottom of the cage with four heptagons around the waist. Both the C3 and C2 axially chiral isomers of B(39)(-) are present in the experiment and contribute to the observed photoelectron spectrum. The chiral borospherenes also exhibit three-dimensional aromaticity, featuring σ and π double delocalization for all valence electrons. Molecular dynamics simulations reveal that these chiral B(39)(-) cages are structurally fluxional above room temperature, compared to the highly robust D(2d)B40 borospherene. The current findings add chiral members to the borospherene family and indicate the structural diversity of boron-based nanomaterials.
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Research context

OpenAlex topics: Boron and Carbon Nanomaterials Research · Synthesis and Properties of Aromatic Compounds · Boron Compounds in Chemistry

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Nanocluster Laboratory, Institute of Molecular Science, Shanxi University, Taiyuan 030006, China

Department of Chemistry, Brown University, Providence, Rhode Island 02912, United States

Department of Chemistry & Key Laboratory of Organic Optoelectronics and Molecular Engineering of Ministry of Education, Tsinghua University, Beijing 100084, China

State Key Laboratory of Quantum Optics and Quantum Optics Devices, Shanxi University, Taiyuan 030006, China

Funding

Division of Chemistry · Ministry of Science and Technology of the People's Republic of China · National Natural Science Foundation of China · Shanxi International Cooperation project · State Key Laboratory of Quantum Optics and Quantum Optics Devices, Shanxi University

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