Multiscale Heterogeneous and Asynchronous Electrochemical Reactions in Lithium-Ion Batteries
Source abstract
Abstract
Battery operation involves sophisticated spatiotemporal evolutions that critically govern their behaviors and degradation. Understanding and manipulating structural heterogeneity and chemical dynamics are key to improving battery performance, lifespan, and safety. This review examines spatial heterogeneity across multiple scales and explores the temporal asynchronicity characteristics of lithium-ion batteries. Furthermore, it underscores the importance of multimodal, high-throughput, and in-situ/operando characterization techniques, paired with advanced data mining methods, in advancing knowledge of battery evolution. We intend for this review to provide a systematic perspective on the spatiotemporal evolution of batteries and to inspire further research into its implications for next-generation battery research and development.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Advancements in Battery Materials · Advanced Battery Technologies Research · Extraction and Separation Processes
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Materials Science and Engineering Program & Texas Materials Institute, Walker Department of Mechanical Engineering
The University of Texas at Austin
Funding
PETRONAS · National Science Foundation
References (66)
Show source-provided references
1. 10.1038/s41560-020-00764-810.1038/s41560-020-00764-8 ↗
2. 10.1002/adma.20180056110.1002/adma.201800561 ↗
3. 10.1016/0025-5408(80)90012-410.1016/0025-5408(80)90012-4 ↗
4. 10.1016/j.ensm.2023.10300110.1016/j.ensm.2023.103001 ↗
5. Lu, Z.; Dahn, J. R.; 3M Innovative Properties Company. Cathode Compositions for Lithium-Ion Batteries. US 6,964,828 B2, Nov 15, 2005.
6. 10.1021/acs.chemrev.2c0025110.1021/acs.chemrev.2c00251 ↗
7. 10.1149/1.183757110.1149/1.1837571 ↗
8. 10.1016/j.jpowsour.2010.11.11310.1016/j.jpowsour.2010.11.113 ↗
9. 10.1016/S0022-0728(74)80146-410.1016/S0022-0728(74)80146-4 ↗
10. 10.1016/j.ensm.2020.12.02710.1016/j.ensm.2020.12.027 ↗
11. 10.1038/nnano.2007.41110.1038/nnano.2007.411 ↗
12. 10.1002/adma.20200457710.1002/adma.202004577 ↗
13. 10.1002/aenm.20240206810.1002/aenm.202402068 ↗
14. 10.1002/adfm.20201029110.1002/adfm.202010291 ↗
15. 10.1038/ncomms452910.1038/ncomms4529 ↗
16. 10.1038/s41563-024-02032-610.1038/s41563-024-02032-6 ↗
17. 10.1038/s41563-024-01833-z10.1038/s41563-024-01833-z ↗
18. 10.1038/s41467-020-19528-910.1038/s41467-020-19528-9 ↗
19. 10.1126/science.abm896210.1126/science.abm8962 ↗
20. 10.1016/j.jpowsour.2015.11.10810.1016/j.jpowsour.2015.11.108 ↗
21. 10.1002/aenm.20190067410.1002/aenm.201900674 ↗
22. 10.1016/j.xcrp.2021.10055410.1016/j.xcrp.2021.100554 ↗
23. 10.1149/2.1441707jes10.1149/2.1441707jes ↗
24. 10.1021/acs.nanolett.2c0181810.1021/acs.nanolett.2c01818 ↗
25. 10.1021/acsmaterialsau.2c0006010.1021/acsmaterialsau.2c00060 ↗
26. 10.1149/1945-7111/ac035910.1149/1945-7111/ac0359 ↗
27. 10.1038/s41467-024-54310-110.1038/s41467-024-54310-1 ↗
28. 10.1016/j.jpowsour.2024.23491610.1016/j.jpowsour.2024.234916 ↗
29. 10.1016/j.joule.2020.02.01010.1016/j.joule.2020.02.010 ↗
30. 10.1016/j.est.2024.11116510.1016/j.est.2024.111165 ↗
31. 10.1016/j.jpowsour.2023.23373610.1016/j.jpowsour.2023.233736 ↗
32. 10.1002/adma.20241691510.1002/adma.202416915 ↗
33. 10.1093/nsr/nwac27210.1093/nsr/nwac272 ↗
34. 10.1038/s41578-019-0157-510.1038/s41578-019-0157-5 ↗
35. 10.1126/sciadv.ado447210.1126/sciadv.ado4472 ↗
36. 10.1038/s41586-023-05970-410.1038/s41586-023-05970-4 ↗
37. 10.1021/acsenergylett.7b0026310.1021/acsenergylett.7b00263 ↗
38. 10.1021/jacs.4c0982410.1021/jacs.4c09824 ↗
39. 10.1002/aenm.20230316510.1002/aenm.202303165 ↗
40. 10.1038/s41467-024-45372-210.1038/s41467-024-45372-2 ↗
41. 10.1016/j.ensm.2025.10411010.1016/j.ensm.2025.104110 ↗
42. 10.1038/s41467-019-13884-x10.1038/s41467-019-13884-x ↗
43. 10.1002/smtd.20210051210.1002/smtd.202100512 ↗
44. 10.1021/acs.chemmater.7b0526910.1021/acs.chemmater.7b05269 ↗
45. 10.1002/aenm.20180396310.1002/aenm.201803963 ↗
46. Tesla Model S Battery System: An Engineer’s Perspective. https://circuitdigest.com/article/tesla-model-s-battery-system-an-engineers-perspective (accessed 2025-01-16).
47. Clever Engineering Behind the New iPhone XS Battery. https://www.wired.com/story/iphone-xs-battery-shape/ (accessed 2025-01-16).
48. 10.1109/EPTC.2018.865434910.1109/EPTC.2018.8654349 ↗
49. 10.1016/j.joule.2024.07.02410.1016/j.joule.2024.07.024 ↗
50. 10.1038/s41467-023-44222-x10.1038/s41467-023-44222-x ↗
51. 10.1149/2.038306jes10.1149/2.038306jes ↗
52. 10.1126/science.aaf491410.1126/science.aaf4914 ↗
53. 10.1073/pnas.220319911910.1073/pnas.2203199119 ↗
54. 10.1016/j.ensm.2021.12.01910.1016/j.ensm.2021.12.019 ↗
55. 10.1021/acs.nanolett.7b0398510.1021/acs.nanolett.7b03985 ↗
56. 10.1038/s41467-020-16233-510.1038/s41467-020-16233-5 ↗
57. 10.1107/S160057751801669710.1107/S1600577518016697 ↗
58. 10.1021/acsenergylett.4c0247610.1021/acsenergylett.4c02476 ↗
59. 10.1021/acsnano.0c0889110.1021/acsnano.0c08891 ↗
60. 10.1002/aenm.20140204010.1002/aenm.201402040 ↗
61. 10.1039/D4EE01497A10.1039/D4EE01497A ↗
62. 10.1088/1361-6501/aafcae10.1088/1361-6501/aafcae ↗
63. 10.1038/s41586-023-06326-810.1038/s41586-023-06326-8 ↗
64. 10.1038/s41467-021-26480-910.1038/s41467-021-26480-9 ↗
65. 10.1038/s41524-020-0340-710.1038/s41524-020-0340-7 ↗
66. 10.1038/s41524-022-00709-710.1038/s41524-022-00709-7 ↗