journal article·2024-02-05Open access

Vascular Bundle for Exceptional Water Confinement, Transport, and Evaporation

El Said A. Nouh, Tianyu Liu, Zacary L. Croft, Guoliang Liu

ACS Materials Letters· Volume 6· Issue 2

Abstract

High Resolution Image Download MS PowerPoint Slide Nature, through billions of years of evolution, has constructed extremely efficient biosystems for transporting, confining, and vaporizing water. Mankind’s ability to master water, however, is far from impeccable, and a sustainable supply of clean fresh water remains a global challenge. Here, we learn from Nature and prepare papyrus carbon (PC) from Egyptian papyrus paper as a sustainable solar desalination material. By taking advantage of the capillary pores from vascular bundles that are inherently built for transporting water in plants, PC achieves an evaporation rate of 4.1 kg m –2 h –1 in a passive single-stage device. Raman spectroscopy and thermal calorimetry show that the capillary pores pose a confinement effect to generate loosely hydrogen-bonded intermediate water, which substantially reduces the enthalpy of vaporization, allowing for exceptionally high energy efficiencies. The understanding is applicable to all nature-designed vascular plants and man-made separation and purification systems.
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Research context

OpenAlex topics: Solar-Powered Water Purification Methods · Solar Thermal and Photovoltaic Systems · Membrane Separation Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Nuclear Materials Authority, P.O. 530, El Maadi, Cairo Egypt

Funding

American Chemical Society Petroleum Research Fund · Division of Materials Research

References (56)

Show source-provided references
1. 10.1038/nnano.2017.12210.1038/nnano.2017.122 ↗
2. 10.1038/nature0659910.1038/nature06599 ↗
3. 10.1126/science.120048810.1126/science.1200488 ↗
4. 10.1038/s41560-018-0260-710.1038/s41560-018-0260-7 ↗
5. 10.1126/sciadv.aax076310.1126/sciadv.aax0763 ↗
6. 10.1039/C8EE01146J10.1039/C8EE01146J ↗
7. 10.1038/s41893-020-00619-w10.1038/s41893-020-00619-w ↗
8. 10.1126/sciadv.aax076310.1126/sciadv.aax0763 ↗
9. 10.1126/sciadv.aaz090610.1126/sciadv.aaz0906 ↗
10. 10.1021/nn304948h10.1021/nn304948h ↗
11. 10.1038/nphoton.2016.7510.1038/nphoton.2016.75 ↗
12. 10.1038/ncomms1010310.1038/ncomms10103 ↗
13. 10.1002/adma.20150013510.1002/adma.201500135 ↗
14. 10.1007/s12274-023-5546-910.1007/s12274-023-5546-9 ↗
15. 10.1038/s41565-018-0097-z10.1038/s41565-018-0097-z ↗
16. 10.1021/accountsmr.1c0005710.1021/accountsmr.1c00057 ↗
17. 10.1002/anie.20220848710.1002/anie.202208487 ↗
18. 10.1038/s41578-020-0182-410.1038/s41578-020-0182-4 ↗
19. 10.1021/acs.accounts.9b0045510.1021/acs.accounts.9b00455 ↗
20. 10.1021/acs.macromol.2c0009210.1021/acs.macromol.2c00092 ↗
21. 10.1002/adma.20150183210.1002/adma.201501832 ↗
22. 10.1038/nnano.2015.3710.1038/nnano.2015.37 ↗
23. 10.1002/adma.20160181910.1002/adma.201601819 ↗
24. 10.1073/pnas.161303111310.1073/pnas.1613031113 ↗
25. 10.1038/s44221-023-00152-y10.1038/s44221-023-00152-y ↗
26. 10.1073/pnas.190531111610.1073/pnas.1905311116 ↗
27. 10.1038/ncomms544910.1038/ncomms5449 ↗
28. 10.1038/nenergy.2016.12610.1038/nenergy.2016.126 ↗
29. 10.1038/s41467-018-07494-210.1038/s41467-018-07494-2 ↗
30. Nicholson P. T. · 2000
31. 10.1002/admt.20180059310.1002/admt.201800593 ↗
32. 10.1002/adma.20160676210.1002/adma.201606762 ↗
33. 10.1016/j.cej.2020.12610810.1016/j.cej.2020.126108 ↗
34. 10.1179/sic.1989.34.1.110.1179/sic.1989.34.1.1 ↗
35. 10.1016/j.carbon.2014.12.03010.1016/j.carbon.2014.12.030 ↗
36. 10.1021/acsomega.0c0191810.1021/acsomega.0c01918 ↗
37. 10.1039/C4NJ01545B10.1039/C4NJ01545B ↗
38. 10.1080/0144235X.2012.76083610.1080/0144235X.2012.760836 ↗
39. 10.1002/adma.20170410710.1002/adma.201704107 ↗
40. 10.1039/D0TA03872E10.1039/D0TA03872E ↗
41. 10.1039/C9EE00945K10.1039/C9EE00945K ↗
42. 10.1021/acsami.7b0130710.1021/acsami.7b01307 ↗
43. World Ocean Database,; National Oceanic and Atmospheric Administration, 2013.
44. 10.1007/s10973-010-1170-510.1007/s10973-010-1170-5 ↗
45. 10.1126/science.109603710.1126/science.1096037 ↗
46. 10.1063/1.486299610.1063/1.4862996 ↗
47. 10.1063/1.305861610.1063/1.3058616 ↗
48. 10.1039/C8EE00567B10.1039/C8EE00567B ↗
49. 10.1126/sciadv.aaw548410.1126/sciadv.aaw5484 ↗
50. 10.1038/s41467-021-27128-410.1038/s41467-021-27128-4 ↗
51. 10.1016/j.joule.2018.03.01310.1016/j.joule.2018.03.013 ↗
52. 10.1002/advs.20180022210.1002/advs.201800222 ↗
53. 10.1039/C9EE04122B10.1039/C9EE04122B ↗
54. World Health Organization (WHO). Safe Drinking-Water from Desalination. Available via the Internet at: http://apps.who.int/iris/bitstream/10665/70621/1/WHO_HSE_WSH_11.03_eng.pdf (accessed: Dec. 29, 2023).
55. 10.1038/s41467-022-34528-710.1038/s41467-022-34528-7 ↗
56. 10.1038/nnano.2016.30010.1038/nnano.2016.300 ↗