journal article·2025-11-03

Electrides with Tunable Electron Delocalization for Applications in Quantum Computing and Catalysis

Andrei Evdokimov, Valentina Nesterova, Marcelo A. Kuroda, Konstantin Klyukin, Evangelos Miliordos

ACS Materials Letters· Volume 7· Issue 11
Publisher page

Abstract

Solvated Electron Precursors (SEPs) are molecular metal–ligand complexes hosting peripheral diffuse electrons that adopt a pseudoatomic electronic structure. These unique characteristics underpin their promising roles in quantum computing applications and redox catalysis. Here we introduce a family of electrides where SEPs are anchored to surfaces – Surface Immobilized Solvated Electron Precursor Electrides (SISEPEs). The electronic properties of SISEPEs can be adjusted through the composition of the SEPs, the nature of the surface support, and the coverage density. Our calculations show that low-density coverage results in either isolated surface-bound diffuse electrons (0D systems) or 1D electron channels, while higher surface coverage yields 2D electron “seas”, closely resembling features of organic and inorganic electrides, respectively. In addition, we demonstrate that the high electron affinity of the surface can lead to partial electron transfer to the bulk of the support material, changing the electrostatic potential of the surface and redox efficiency of SISEPEs.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Ammonia Synthesis and Nitrogen Reduction · Electrocatalysts for Energy Conversion · Advanced Photocatalysis Techniques

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemistry and Biochemistry

Auburn University

Department of Materials Engineering

Department of Physics

Funding

Division of Chemistry · Auburn University · Division of Materials Research

References (61)

Show source-provided references
1. 10.1039/D0TC01165G10.1039/D0TC01165G ↗
2. 10.1021/acs.chemrev.0c0107110.1021/acs.chemrev.0c01071 ↗
3. 10.1103/PhysRevX.8.03106710.1103/PhysRevX.8.031067 ↗
4. 10.1107/S010827018800284710.1107/S0108270188002847 ↗
5. 10.1021/ja964076010.1021/ja9640760 ↗
6. 10.1021/ja960548z10.1021/ja960548z ↗
7. 10.1126/science.108810310.1126/science.1088103 ↗
8. 10.1021/ja053216f10.1021/ja053216f ↗
9. 10.1002/anie.20090037310.1002/anie.200900373 ↗
10. 10.1021/ja109397k10.1021/ja109397k ↗
11. 10.1039/D3CC02956E10.1039/D3CC02956E ↗
12. 10.1146/annurev-matsci-080423-12405010.1146/annurev-matsci-080423-124050 ↗
13. 10.1021/acs.jpcc.6b1242510.1021/acs.jpcc.6b12425 ↗
14. 10.1103/PhysRevLett.75.97810.1103/PhysRevLett.75.978 ↗
15. 10.1039/C8CP05497E10.1039/C8CP05497E ↗
16. 10.1039/C9CP01897B10.1039/C9CP01897B ↗
17. 10.1021/acs.jpca.9b0773410.1021/acs.jpca.9b07734 ↗
18. 10.1088/1361-6455/ab52ef10.1088/1361-6455/ab52ef ↗
19. 10.3389/frqst.2024.142621610.3389/frqst.2024.1426216 ↗
20. 10.1007/s40042-023-00774-110.1007/s40042-023-00774-1 ↗
21. 10.1103/PhysRevLett.127.06360410.1103/PhysRevLett.127.063604 ↗
22. 10.1088/1674-1056/abd76f10.1088/1674-1056/abd76f ↗
23. 10.1039/D1CC04748E10.1039/D1CC04748E ↗
24. 10.3389/fbioe.2021.79084910.3389/fbioe.2021.790849 ↗
25. 10.1039/C9TC03381E10.1039/C9TC03381E ↗
26. 10.1007/s10008-007-0473-310.1007/s10008-007-0473-3 ↗
27. 10.1021/acs.jpcc.3c0067510.1021/acs.jpcc.3c00675 ↗
28. 10.1016/j.mtsust.2024.10105210.1016/j.mtsust.2024.101052 ↗
29. 10.1115/1.406296910.1115/1.4062969 ↗
30. 10.1109/TEM.2023.328468910.1109/TEM.2023.3284689 ↗
31. 10.1109/JPROC.2019.295400510.1109/JPROC.2019.2954005 ↗
32. 10.1039/D0CS01341B10.1039/D0CS01341B ↗
33. 10.1039/D3TA06546D10.1039/D3TA06546D ↗
34. 10.1021/acs.jpclett.1c0363710.1021/acs.jpclett.1c03637 ↗
35. 10.1039/C7TC02488F10.1039/C7TC02488F ↗
36. 10.1103/PhysRevB.53.1551310.1103/PhysRevB.53.15513 ↗
37. 10.1021/acs.jpclett.0c0240510.1021/acs.jpclett.0c02405 ↗
38. 10.1063/5.008981510.1063/5.0089815 ↗
39. 10.1039/c1cp22389e10.1039/c1cp22389e ↗
40. 10.1039/C6CP05345A10.1039/C6CP05345A ↗
41. 10.1021/acs.jpcc.8b0212510.1021/acs.jpcc.8b02125 ↗
42. 10.1021/jacs.3c0124310.1021/jacs.3c01243 ↗
43. 10.1039/C4CC03397C10.1039/C4CC03397C ↗
44. 10.1002/anie.20130065410.1002/anie.201300654 ↗
45. 10.1103/PhysRevLett.121.12360310.1103/PhysRevLett.121.123603 ↗
46. 10.1038/s41586-020-2257-110.1038/s41586-020-2257-1 ↗
47. 10.1016/j.apsusc.2012.02.13710.1016/j.apsusc.2012.02.137 ↗
48. 10.1103/PhysRevB.75.21410910.1103/PhysRevB.75.214109 ↗
49. 10.1021/acs.jpcc.6b1108510.1021/acs.jpcc.6b11085 ↗
50. 10.1680/jnaen.17.0000610.1680/jnaen.17.00006 ↗
51. 10.1039/D2TC01981G10.1039/D2TC01981G ↗
52. 10.1088/0022-3727/43/22/22300110.1088/0022-3727/43/22/223001 ↗
53. Frisch, M. J. Gaussian 16 , Revision C.01; Gaussian Inc.: Wallingford CT, 2016.
54. 10.1126/science.aaz760710.1126/science.aaz7607 ↗
55. 10.1063/1.45615310.1063/1.456153 ↗
56. 10.1063/1.46256910.1063/1.462569 ↗
57. 10.1063/1.46643910.1063/1.466439 ↗
58. 10.1021/acs.jpclett.7b0300010.1021/acs.jpclett.7b03000 ↗
59. 10.1039/D4CP00723A10.1039/D4CP00723A ↗
60. Haynes W. M. · 2012
61. 10.1145/3569951.359755910.1145/3569951.3597559 ↗