DataVXACS Materials LettersPaper
journal article·2024-04-01

Monoatomic Nickel Wires via Columnar Self-Assembly of Tribenzocyclyne Nickel Complexes

Bin Li, Glenn P. A. Yap, Vincent St-Onge, Niki Mavragani, Thi Thanh Hà Dao, Pierre Baillargeon, Patrick Fournier, Yves L. Dory, Jerome P. Claverie

ACS Materials Letters· Volume 6· Issue 4
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Source abstract

Abstract

Monoatomic metal wires (MAMW) possess unique physical properties and exciting potential applications. In particular, Ni MAMW has been predicted to be ferromagnetic. However, the inherent instability of MAMW due to the Peierls distortion phenomenon renders its fabrication and isolation extremely difficult. Here we fabricate monatomic Ni MAMW through the columnar self-assembly of tribenzocyclyne (TBC) derivatives. Three types of Ni MAMWs have been constructed: MAMW I, II and III with average Ni–Ni distances of 0.480, 0.342, and 0.336 nm, which were found to be diamagnetic. The Peierls distortions were absent when three H-bonds were installed on each TBC unit, giving insight into the energy level required to overcome Peierls distortions. These results not only enriched the methods for the fabrication of MAMWs but also are of value to understand the magnetic properties of MAMWs.
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Research context

OpenAlex topics: Molecular Junctions and Nanostructures · Surface Chemistry and Catalysis · Porphyrin and Phthalocyanine Chemistry

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemistry, Faculty of Sciences, Université de Sherbrooke, Sherbrooke, Quebec J1K 2R1, Canada

Department of Chemistry and Biochemistry, University of Delaware, Newark, Delaware 19716, United States

Department of Chemistry and Biomolecular Sciences, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada

Department of Chemistry, Faculty of Sciences & Institut de Pharmacologie et Centre de Recherche du CHUS, Université de Sherbrooke, Sherbrooke, Quebec J1K 2R1, Canada

Department of Chemistry, Cégep de Sherbrooke, Sherbrooke, Quebec J1E 4K1, Canada

Quantum Institute, Department of Physics, University of Sherbrooke, Sherbrooke, Quebec J1K 2R1, Canada

Funding

Canada Foundation for Innovation · Fonds de recherche du Qu?bec ? Nature et technologies · Canada Research Chairs · Stavros Niarchos Foundation · Natural Sciences and Engineering Research Council of Canada

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