journal article·2021-03-22Open access

Challenges for and Pathways toward Li-Metal-Based All-Solid-State Batteries

Paul Albertus, Venkataramani Anandan, Chunmei Ban, Nitash Balsara, Ilias Belharouak, Josh Buettner-Garrett, Zonghai Chen, Claus Daniel, Marca Doeff, Nancy J. Dudney, Bruce Dunn, Stephen J. Harris, Subramanya Herle, Eric Herbert, Sergiy Kalnaus, Joesph A. Libera, Dongping Lu, Steve Martin, Bryan D. McCloskey, Matthew T. McDowell, Y. Shirley Meng, Jagjit Nanda, Jeff Sakamoto, Ethan C. Self, Sanja Tepavcevic, Eric Wachsman, Chunsheng Wang, Andrew S. Westover, Jie Xiao, Thomas Yersak

Abstract

Solid-state batteries utilizing Li metal anodes have the potential to enable improved performance (specific energy >500 Wh/kg, energy density >1500 Wh/L), safety, recyclability, and potentially lower cost (<$100/kWh) compared to advanced Li-ion systems.1,2 These improvements are critical for the widespread adoption of electric vehicles (EVs) and trucks and could create a short-haul electric aviation industry.1-3 Expectations for solid-state batteries are high, but there are significant materials and processing challenges to overcome.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Advanced Battery Materials and Technologies · Advancements in Battery Materials · Advanced Battery Technologies Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, Maryland 20742, United States

Ford Motor Company, Dearborn, Michigan 48121, United States

Mechanical Engineering Department, University of Colorado, Boulder, Colorado 80309, United States

Department of Chemical and Biomolecular Engineering and Lawrence Berkeley National Laboratory, Materials Sciences Division, University of California, Berkeley, California 94720, United States

Energy and Transportation Science Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United States

Solid Power, Inc., Louisville, Colorado 80027, United States

Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, Illinois 60439, United States

Lawrence Berkeley National Laboratory, Energy Storage and Distributed Resources Division, University of California, Berkeley, California 94720, United States

Department of Materials Science and Engineering, University of California, Los Angeles, California 90095, United States

Applied Materials Inc., 3225 Oakmead Village Drive, B12_2F6, Santa Clara, California 95054, United States

Department of Materials Science and Engineering, Michigan Technological University, Houghton, Michigan 49931, United States

Energy and Environmental Directorate, Pacific Northwest National Laboratory, Richland, Washington 99352, United States

Department of Materials Science & Engineering, Iowa State University of Science & Technology, Ames, Iowa 50011, United States

Woodruff School of Mechanical Engineering and School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332, United States

Department of NanoEngineering and Materials Science and Engineering Program, University of California San Diego, La Jolla, California 92093, United States

Department of Materials Science and Engineering and Department of Mechanical Engineering, University of Michigan, Ann Arbor, Michigan 48109, United States

Chemical and Materials Systems Laboratory, General Motors Global R&D, Warren, Michigan 48092-2031, United States

Funding

Oak Ridge National Laboratory

References (22)

Show source-provided references
1. 10.1021/acsenergylett.0c0258410.1021/acsenergylett.0c02584 ↗
2. 10.1021/acsenergylett.0c0197710.1021/acsenergylett.0c01977 ↗
3. 10.1038/s41893-019-0233-210.1038/s41893-019-0233-2 ↗
4. Herle, S.; Chen, Z.; Libera, J.; Tepavcevic, S.; Anandan, V.; Yersak, T.; McDowell, M. T.; Martin, S.; Doeff, M.; Harris, S.Challenges for and Pathways Toward Solid-State Batteries, ORNL/TM-2020/1747; Oak Ridge National Laboratory, Oak Ridge, TN, 2020. 10.2172/173104310.2172/1731043 ↗
5. 10.1038/s41560-020-0565-110.1038/s41560-020-0565-1 ↗
6. 10.1039/C9TA04772G10.1039/C9TA04772G ↗
7. 10.1002/smtd.20200011110.1002/smtd.202000111 ↗
8. 10.1021/acsenergylett.9b0266010.1021/acsenergylett.9b02660 ↗
9. 10.1038/s41560-019-0338-x10.1038/s41560-019-0338-x ↗
10. 10.1039/D0TA02984J10.1039/D0TA02984J ↗
11. 10.1002/aenm.20200080210.1002/aenm.202000802 ↗
12. 10.1002/adma.20190521910.1002/adma.201905219 ↗
13. 10.1016/j.chempr.2018.11.01310.1016/j.chempr.2018.11.013 ↗
14. 10.1038/s41578-019-0157-510.1038/s41578-019-0157-5 ↗
15. 10.1002/aenm.20200064810.1002/aenm.202000648 ↗
16. 10.1038/s41578-019-0165-510.1038/s41578-019-0165-5 ↗
17. 10.1557/jmr.2018.8510.1557/jmr.2018.85 ↗
18. 10.1073/pnas.161573311410.1073/pnas.1615733114 ↗
19. 10.1557/s43578-020-00098-x10.1557/s43578-020-00098-x ↗
20. 10.1021/acsaem.9b0210110.1021/acsaem.9b02101 ↗
21. 10.1126/science.aaz768110.1126/science.aaz7681 ↗
22. 10.1038/s41560-020-0575-z10.1038/s41560-020-0575-z ↗