journal article·2025-01-10

Enhancing Water Management with Three-Dimensionally Micropatterned Anion Exchange Membranes for Alkaline Fuel Cells

Chang Liu, Tianyue Gao, Leanna Schulte, Sariah Marth, Heemin Park, Chulsung Bae, Thomas E. Mallouk

ACS Energy Letters· Volume 10· Issue 1
Publisher page

Abstract

Alkaline exchange membrane fuel cells (AEMFCs) offer a promising solution for clean hydrogen utilization. However, effective water management remains a challenge due to the concurrent generation and consumption of water at the electrodes, which impacts the efficiency of AEMFCs at high current densities. Here, we report the fabrication of alkaline fuel cells with improved water management by employing a three-dimensionally patterned alkaline exchange membrane (AEM) at the interface with the cathode catalyst layer. This micropatterned AEM, made by soft lithography, enables a power density of 628 mW cm –2 at a current density of 1100 mA cm –2, representing an approximately 50% performance improvement over identical AEMFCs made from conventional two-dimensional AEMs. The patterned AEM also improves platinum utilization due to the increased catalyst-membrane contact area and tailored catalyst layer thickness.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Fuel Cells and Related Materials · Electrocatalysts for Energy Conversion · Advanced battery technologies research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

University of Pennsylvania, Department of Chemistry, 231 S 34th St, Philadelphia, Pennsylvania 19104, United States

Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United States

Department of Chemistry and Chemical Biology, Rensselaer Polytechnic Institute, Troy, New York 12180, United States

Funding

Energy Frontier Research Centers · National Science Foundation · Vagelos Institute for Energy Science and Technology, University of Pennsylvania

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