Managing Impurities in Direct Battery Recycling: Advancing Separation and Purification for High-Quality Feedstocks
Source abstract
Abstract
Direct recycling offers a more sustainable and energy-efficient alternative to conventional metallurgical methods for treating end-of-life lithium-ion batteries (LIBs). However, the large-scale deployment of direct regeneration is limited by its low tolerance to impurities, making the production of high-purity feedstocks and impurity management essential for viability. Drawing on insights into how impurities affect cathode regeneration, this Perspective discusses current and emerging separation and purification technologies and delineates the remaining gap to the mass production of high-quality feedstocks. We propose integrated, high-efficiency approaches that elevate feedstock quality and broaden impurity control across the entire workflow, positioning impurity management in both preprocessing and regeneration as being essential to the economic and environmental performance of direct recycling. The result is a research roadmap to enable scalable, sustainable, and cost-effective battery recycling practices.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Extraction and Separation Processes · Advanced Battery Technologies Research · Recycling and Waste Management Techniques
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Aiiso Yufeng Li Family Department of Chemical and Nano Engineering
University of California, San Diego
Sustainable Power and Energy Center
Program of Materials Science and Engineering
Funding
BASF · California Energy Commission · U.S. Department of Energy
References (87)
Show source-provided references
1. 2024
2. Fleischmann, J.; Hanicke, M.; Horetsky, E.; Ibrahim, D.; Jautelat, S.; Linder, M.; Schaufuss, P.; Torscht, L.; van de Rijt, A. Battery 2030: Resilient, sustainable, and circular. McKinsey & Company, 2023. https://www.mckinsey.com/industries/automotive-and-assembly/our-insights/battery-2030-resilient-sustainable-and-circular#/.
3. 10.1016/j.xcrp.2025.10245310.1016/j.xcrp.2025.102453 ↗
4. 10.1038/s44359-024-00010-410.1038/s44359-024-00010-4 ↗
5. Dai Q. · 201910.2172/1530874 ↗
6. 10.1002/aenm.20240538310.1002/aenm.202405383 ↗
7. 10.1021/acsenergylett.4c0219810.1021/acsenergylett.4c02198 ↗
8. 10.1126/science.372.6544.78010.1126/science.372.6544.780 ↗
9. 10.1038/s41467-023-43883-y10.1038/s41467-023-43883-y ↗
10. 10.1038/s41578-025-00783-510.1038/s41578-025-00783-5 ↗
11. 10.1002/adfm.20221316810.1002/adfm.202213168 ↗
12. 10.1021/acsenergylett.4c0317610.1021/acsenergylett.4c03176 ↗
13. 10.1016/j.geits.2024.10023510.1016/j.geits.2024.100235 ↗
14. 10.1021/acsami.1c2093810.1021/acsami.1c20938 ↗
15. 10.1021/acssuschemeng.1c0151010.1021/acssuschemeng.1c01510 ↗
16. 10.1016/j.nxener.2023.10009110.1016/j.nxener.2023.100091 ↗
17. 10.1002/adma.20230849410.1002/adma.202308494 ↗
18. 10.1149/1945-7111/abcc2f10.1149/1945-7111/abcc2f ↗
19. 10.1590/0104-1428.2022009410.1590/0104-1428.20220094 ↗
20. 10.1002/aenm.20240608310.1002/aenm.202406083 ↗
21. 10.1016/j.ensm.2022.06.01710.1016/j.ensm.2022.06.017 ↗
22. 10.1021/acssuschemeng.3c0774410.1021/acssuschemeng.3c07744 ↗
23. 10.1016/j.matlet.2011.01.07410.1016/j.matlet.2011.01.074 ↗
24. 10.1038/s41467-018-03324-710.1038/s41467-018-03324-7 ↗
25. 10.1039/D4GC02370F10.1039/D4GC02370F ↗
26. 10.1007/s10854-019-01830-y10.1007/s10854-019-01830-y ↗
27. 10.1002/aenm.20240608410.1002/aenm.202406084 ↗
28. 10.1002/batt.20210011010.1002/batt.202100110 ↗
29. 10.1016/j.est.2016.10.00810.1016/j.est.2016.10.008 ↗
30. 10.1149/1945-7111/ab697a10.1149/1945-7111/ab697a ↗
31. 10.1002/cssc.20240143210.1002/cssc.202401432 ↗
32. 10.1021/cm202661910.1021/cm2026619 ↗
33. 10.1021/acs.chemrev.3c0017410.1021/acs.chemrev.3c00174 ↗
34. 10.1016/j.seppur.2024.12632710.1016/j.seppur.2024.126327 ↗
35. 10.1021/acssuschemeng.8b0218610.1021/acssuschemeng.8b02186 ↗
36. 10.1016/j.joule.2020.10.00810.1016/j.joule.2020.10.008 ↗
37. 10.1002/aenm.20200120410.1002/aenm.202001204 ↗
38. 10.1038/s41893-025-01539-310.1038/s41893-025-01539-3 ↗
39. 10.1002/aenm.20240592410.1002/aenm.202405924 ↗
40. 10.1016/j.ensm.2025.10454210.1016/j.ensm.2025.104542 ↗
41. 10.1021/acssuschemeng.1c0129310.1021/acssuschemeng.1c01293 ↗
42. 10.1021/acssuschemeng.4c0559110.1021/acssuschemeng.4c05591 ↗
43. 10.1039/D5GC03161C10.1039/D5GC03161C ↗
44. 10.1039/D1RA04922D10.1039/D1RA04922D ↗
45. 10.1002/aenm.20220309310.1002/aenm.202203093 ↗
46. 10.1038/s41467-024-53731-210.1038/s41467-024-53731-2 ↗
47. 10.31635/ccschem.022.20220199610.31635/ccschem.022.202201996 ↗
48. 10.1016/j.isci.2023.10767610.1016/j.isci.2023.107676 ↗
49. 10.1021/acs.chemrev.3c0088410.1021/acs.chemrev.3c00884 ↗
50. 10.1007/s10845-022-01936-x10.1007/s10845-022-01936-x ↗
51. 10.1016/j.promfg.2020.02.14510.1016/j.promfg.2020.02.145 ↗
52. 10.1016/j.joule.2023.04.00210.1016/j.joule.2023.04.002 ↗
53. 10.1016/j.jpowsour.2024.23415610.1016/j.jpowsour.2024.234156 ↗
54. 10.1016/j.apenergy.2022.12043710.1016/j.apenergy.2022.120437 ↗
55. 10.1007/s10845-023-02081-910.1007/s10845-023-02081-9 ↗
56. 10.1108/MEQ-04-2024-016310.1108/MEQ-04-2024-0163 ↗
57. Tankou A. · 2023
58. 10.1016/j.susmat.2019.e0013410.1016/j.susmat.2019.e00134 ↗
59. Kitchener J. · 1984 · 310.1007/978-94-009-6926-1_2 ↗
60. 10.1021/acssuschemeng.2c0631110.1021/acssuschemeng.2c06311 ↗
61. 10.1016/j.cep.2021.10831010.1016/j.cep.2021.108310 ↗
62. 10.1021/acssusresmgt.5c0040910.1021/acssusresmgt.5c00409 ↗
63. 10.1021/acssusresmgt.5c0005810.1021/acssusresmgt.5c00058 ↗
64. 10.1021/acsenergylett.8b0123310.1021/acsenergylett.8b01233 ↗
65. 10.1016/j.jpowsour.2013.09.05210.1016/j.jpowsour.2013.09.052 ↗
66. 10.1002/ente.20210046810.1002/ente.202100468 ↗
67. 10.1016/j.seppur.2025.13248010.1016/j.seppur.2025.132480 ↗
68. 10.1016/j.wasman.2019.08.04110.1016/j.wasman.2019.08.041 ↗
69. 10.1016/j.seppur.2022.12148610.1016/j.seppur.2022.121486 ↗
70. 10.1002/aenm.20250100910.1002/aenm.202501009 ↗
71. 10.1016/j.jenvman.2023.11967010.1016/j.jenvman.2023.119670 ↗
72. 10.1149/1.183803610.1149/1.1838036 ↗
73. 10.1029/90WR0240910.1029/90WR02409 ↗
74. 10.1007/s11270-025-08240-310.1007/s11270-025-08240-3 ↗
75. 10.1002/adma.20240148210.1002/adma.202401482 ↗
76. 10.1002/bte2.2024009910.1002/bte2.20240099 ↗
77. 10.1039/D4EE03444A10.1039/D4EE03444A ↗
78. 10.1021/acsaem.0c0085910.1021/acsaem.0c00859 ↗
79. 10.1039/C1EE01263K10.1039/C1EE01263K ↗
80. 10.1016/j.ensm.2021.03.01510.1016/j.ensm.2021.03.015 ↗
81. 10.1002/adma.20240846310.1002/adma.202408463 ↗
82. 10.1002/anie.20250195810.1002/anie.202501958 ↗
83. 10.1557/s43580-024-00890-510.1557/s43580-024-00890-5 ↗
84. 10.1038/s41467-025-56063-x10.1038/s41467-025-56063-x ↗
85. 10.1021/acs.est.4c1383810.1021/acs.est.4c13838 ↗
86. 10.1016/j.seppur.2025.13584710.1016/j.seppur.2025.135847 ↗
87. Wang M. · 202110.2172/1824336 ↗