journal article·2024-08-09

Emerging Amorphized Metastable Structures to Break Limitations of 2D Materials for More Promising Electrocatalysis

Yu Gao, Huanhuan Liang, Hui Xu, Dandan Cui, Chao Wu, Jun Chen, Yang Liu, Shi-xue Dou, Wei Huang, Liangxu Lin

ACS Energy Letters· Volume 9· Issue 8
Publisher page

Abstract

Ultrathin two-dimensional (2D) materials, including both layered and nonlayered structures show promise as electrocatalysts. Their catalytic performance is limited by their natural electronic structure and 2D stacking. Regulating the 2D structure with exotic atoms can tailor the chemical affinity. Even in metastable phases, the surfaces of 2D materials are not sufficiently active for simple chemical modifications to enhance the catalytic activity and diversify catalytic reactions. Differentially, the emerging ultrathin 2D amorphized metastable material lacks a phase structure and exhibits high activity with rich dangling bond states. This material may offer solutions to the aforementioned challenges faced by traditional 2D materials. This report discusses the ultrathin 2D amorphized metastable material as an ideal platform to break limitations of traditional 2D materials in electrocatalysis and suggests how these materials can be developed for more promising electrocatalysis. The potential stabilizations, fabrications, and challenges of these materials are also discussed to provide guidance on areas of focus.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Electrocatalysts for Energy Conversion · Advanced Photocatalysis Techniques · Supercapacitor Materials and Fabrication

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou 350117, China

School of Materials and Chemistry, University of Shanghai for Science & Technology, Shanghai 200093, China

School of Physics, Beihang University, Beijing 100191, China

Institute of Energy Materials Science, University of Shanghai for Science and Technology, Shanghai 200093, China

ARC Centre of Excellence for Electromaterials Science, Intelligent Polymer Research Institute, Australia Institute for Innovative Materials, Innovation Campus, University of Wollongong, Wollongong 2522, Australia

Frontiers Science Center for Flexible Electronics (FSCFE), MIIT Key Laboratory of Flexible Electronics (KLoFE), Northwestern Polytechnical University, Xi’an 710072, China

Funding

National Natural Science Foundation of China · Independent Innovation Projects of the Hubei Longzhong Laboratory

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