journal article·2020-11-13

Deformation during Electrosorption and Insertion-Type Charge Storage: Origins, Characterization, and Design of Materials for High Power

Veronica Augustyn, Ruocun Wang, Nina Balke, Matt Pharr, Craig B. Arnold

ACS Energy Letters· Volume 5· Issue 11
Publisher page

Abstract

Ion electrosorption and insertion form the basis of two commercialized electrochemical energy storage technologies: electric double-layer capacitors and lithium ion batteries. These processes are also of interest for emerging applications in water treatment, critical element extraction, and neuromorphic computing. The kinetics of electrosorption and insertion are intimately related to the mechanical deformation of the host material. This Perspective discusses the following: (1) similarities and differences in the deformation response of materials due to ion electrosorption and insertion, (2) correlation between mechanical and electrochemical response via several operando techniques, and (3) how the understanding of deformation can guide the design of new electrosorption and ion insertion materials with faster kinetics.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Membrane-based Ion Separation Techniques · Advanced battery technologies research · Supercapacitor Materials and Fabrication

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Materials Science & Engineering, North Carolina State University, Raleigh, North Carolina 27695, United States

Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, United States

Department of Mechanical Engineering, Texas A&M University, College Station, Texas 77843, United States

Department of Mechanical and Aerospace Engineering and Princeton Institute for the Science and Technology of Materials, Princeton University, New Jersey 08540, United States

Funding

Basic Energy Sciences · Division of Chemical, Bioengineering, Environmental, and Transport Systems · Division of Materials Research

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