journal article·2020-10

Performance of high-temperature thermosetting polyimide composites modified with thermoplastic polyimide

Hongjun Ke, Liwei Zhao, Xiaohong Zhang, Yingjie Qiao, Guoyong Wang, Xiaodong Wang

Polymer Testing· Volume 90
Publisher page

Abstract

Abstract The preparation of polyimide (PI) resin with high heat resistance and toughness is a significant challenge. In this study, thermoplastic PI (TPI) was used to toughen thermosetting PIs, and toughened PI (TPI/PI) blends were prepared. The modified PI resin system exhibited good thermal stability, excellent heat resistance, and high toughness. The results indicated that the TPI/PI blends maintained the curing behavior and characteristics of the PI oligomer. The Tg of the cured TPI/PI blend exceeded 395 °C, and the T5% values were in the range of 533–563 °C, suggesting excellent thermal stability and heat resistance. The maximum impact strength was increased by 46% compared with that of pure PI, indicating the excellent toughening effect of the TPI. Carbon fiber-reinforced PI composites were prepared using the toughening system as a matrix. The compression-after-impact values of the carbon fiber-reinforced PI composites were up to 190 MPa, indicating the excellent toughness of the materials.
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Research context

OpenAlex topics: Synthesis and properties of polymers · Tribology and Wear Analysis · Epoxy Resin Curing Processes

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