Resin Wettability Correlates Linearly to Interfacial Fracture Energy between Thermosetting Elastomers and Glass
Source abstract
Abstract
Interfacial adhesion influences mechanical strength, structural integrity, and overall performance for adhesively bonded structures and composite materials. In this work, we investigate the effect of resin formulation chemistry on wetting behavior and interfacial adhesion with a glass substrate. Thermosetting elastomer resin and cured network properties, including viscosity, surface tension, glass transition temperature, and molecular weight between cross-links, were also characterized, and the relative importance of these properties on adhesive strength was evaluated. Resin wettability was found to be the factor most predictive of adhesive strength between thermosetting elastomers and glass surfaces, with increasing wettability (decreasing resin contact angle) correlated with increasing interfacial fracture energy. This finding provides a convenient and fast method to screen polymer networks and enables informed tailoring of interfacial fracture energy.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Adhesion, Friction, and Surface Interactions · Surface Modification and Superhydrophobicity · Advanced Sensor and Energy Harvesting Materials
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Department of Plastics Engineering, University of Massachusetts Lowell, Lowell, Massachusetts 01854, United States
Department of Mechanical Engineering, University of Massachusetts Lowell, Lowell, Massachusetts 01854, United States
Weapons and Materials Research Directorate, US Army Combat Capabilities Development Command-Army Research Laboratory, Aberdeen Proving Ground, Maryland 21005, United States
Funding
Army Research Laboratory
References (73)
Show source-provided references
1. 10.1016/j.matdes.2009.07.04510.1016/j.matdes.2009.07.045 ↗
2. 10.1016/j.matlet.2017.12.03310.1016/j.matlet.2017.12.033 ↗
3. 10.1016/j.dt.2019.04.00810.1016/j.dt.2019.04.008 ↗
4. 10.1007/s10853-018-3006-910.1007/s10853-018-3006-9 ↗
5. 10.1016/j.compositesb.2018.10.09810.1016/j.compositesb.2018.10.098 ↗
6. 10.3390/ma1314316710.3390/ma13143167 ↗
7. 10.3390/ijms1012511510.3390/ijms10125115 ↗
8. 10.1098/rsta.2016.005710.1098/rsta.2016.0057 ↗
9. 10.1016/j.cis.2013.12.01410.1016/j.cis.2013.12.014 ↗
10. 10.1016/j.surfcoat.2020.12638910.1016/j.surfcoat.2020.126389 ↗
11. 10.1007/s10443-020-09854-y10.1007/s10443-020-09854-y ↗
12. 10.1016/j.ccr.2021.21384610.1016/j.ccr.2021.213846 ↗
13. 10.1016/j.ijadhadh.2005.03.00410.1016/j.ijadhadh.2005.03.004 ↗
14. 10.1007/978-1-4899-2070-610.1007/978-1-4899-2070-6 ↗
15. 10.1021/nn202453910.1021/nn2024539 ↗
16. 10.1016/j.porgcoat.2008.11.00610.1016/j.porgcoat.2008.11.006 ↗
17. 10.1002/pc.2276910.1002/pc.22769 ↗
18. 10.1016/S0266-3538(97)00033-X10.1016/S0266-3538(97)00033-X ↗
19. 10.1039/d1ra07602g10.1039/d1ra07602g ↗
20. 10.1016/j.compositesb.2018.07.03110.1016/j.compositesb.2018.07.031 ↗
21. 10.1016/j.polymer.2004.07.00310.1016/j.polymer.2004.07.003 ↗
22. 10.1016/j.polymer.2005.02.01110.1016/j.polymer.2005.02.011 ↗
23. 10.1039/c5py01631b10.1039/c5py01631b ↗
24. 10.1002/app.189710.1002/app.1897 ↗
25. 10.1039/c2gc35672d10.1039/c2gc35672d ↗
26. 10.1016/j.compscitech.2010.11.02210.1016/j.compscitech.2010.11.022 ↗
27. 10.1021/am302383v10.1021/am302383v ↗
28. 10.1016/S0079-6700(97)00004-X10.1016/S0079-6700(97)00004-X ↗
29. 10.1016/j.progpolymsci.2009.10.00610.1016/j.progpolymsci.2009.10.006 ↗
30. 10.1016/j.polymer.2013.07.05910.1016/j.polymer.2013.07.059 ↗
31. 10.1080/01694243.2012.74615910.1080/01694243.2012.746159 ↗
32. 10.1163/15685610677765777910.1163/156856106777657779 ↗
33. 10.1007/s00289-017-2022-210.1007/s00289-017-2022-2 ↗
34. 10.1080/0021846720807222210.1080/00218467208072222 ↗
35. 10.1007/BF0142188710.1007/BF01421887 ↗
36. 10.1007/s11998-013-9522-210.1007/s11998-013-9522-2 ↗
37. 10.1016/j.ijadhadh.2013.12.01310.1016/j.ijadhadh.2013.12.013 ↗
38. 10.1016/j.ijadhadh.2019.10245010.1016/j.ijadhadh.2019.102450 ↗
39. 10.1039/D1RA05916E10.1039/D1RA05916E ↗
40. 10.1016/j.tsf.2006.04.00610.1016/j.tsf.2006.04.006 ↗
41. 10.1002/app.1969.07013081510.1002/app.1969.070130815 ↗
42. 10.1016/j.jcis.2015.05.01210.1016/j.jcis.2015.05.012 ↗
43. 10.1088/0034-4885/79/4/04660110.1088/0034-4885/79/4/046601 ↗
44. 10.1002/pen.2416710.1002/pen.24167 ↗
45. 10.1007/s00348-020-02971-110.1007/s00348-020-02971-1 ↗
46. Roberto Vieira Junior P. · 2019
47. 10.1021/ma990175x10.1021/ma990175x ↗
48. 10.3390/polym1313216210.3390/polym13132162 ↗
49. 10.1016/j.jcis.2012.09.00810.1016/j.jcis.2012.09.008 ↗
50. 10.3389/fchem.2014.0001010.3389/fchem.2014.00010 ↗
51. 10.1021/ma961170s10.1021/ma961170s ↗
52. 10.1002/978111933720110.1002/9781119337201 ↗
53. 10.1016/j.jiec.2017.10.00410.1016/j.jiec.2017.10.004 ↗
54. 10.1039/c3ta12918g10.1039/c3ta12918g ↗
55. 10.1016/j.ijadhadh.2020.10263010.1016/j.ijadhadh.2020.102630 ↗
56. 10.1002/app.1107710.1002/app.11077 ↗
57. 10.1002/pc.1036410.1002/pc.10364 ↗
58. 10.1122/1.55080410.1122/1.550804 ↗
59. 10.1021/acsapm.0c0096610.1021/acsapm.0c00966 ↗
60. 10.1021/acsapm.8b0015010.1021/acsapm.8b00150 ↗
61. 10.1063/1.43384610.1063/1.433846 ↗
62. 10.1039/c7sm02407j10.1039/c7sm02407j ↗
63. 10.1016/j.polymer.2009.01.02110.1016/j.polymer.2009.01.021 ↗
64. 10.1016/S0032-3861(97)00585-510.1016/S0032-3861(97)00585-5 ↗
65. 10.1002/app.4368410.1002/app.43684 ↗
66. 10.1007/b13747610.1007/b137476 ↗
67. 10.1016/j.dental.2016.06.00110.1016/j.dental.2016.06.001 ↗
68. 10.3390/polym911056710.3390/polym9110567 ↗
69. 10.1016/0266-3538(90)90042-410.1016/0266-3538(90)90042-4 ↗
70. 10.1533/9780857097637.1.6210.1533/9780857097637.1.62 ↗
71. 10.1002/pc.75012010810.1002/pc.750120108 ↗
72. 10.1007/s12633-010-9043-x10.1007/s12633-010-9043-x ↗
73. 10.1016/j.polymertesting.2019.03.03310.1016/j.polymertesting.2019.03.033 ↗