journal article·2025-06-13

Biobased Multilayer Flexible Packaging with Enhanced Gas Barrier Properties due to Cellulose Nanocrystals (CNCs)

Jingxuan Zhang, Yirou Wang, Darien Anders Dewar, Akshat Verma, Nazmul Haque, Ronaldo Franjul, Nicole Stark, Chelsea S. Davis, Jeffrey P. Youngblood

ACS Applied Polymer Materials· Volume 7· Issue 11
Publisher page

Abstract

In this study, a transparent trilayer film was successfully fabricated using blade coating and hot roll lamination techniques, comprising outer layers of polylactic acid (PLA) and an inner layer of a highly shear-oriented cellulose nanocrystal (CNC)/poly(vinyl alcohol) (PVA). The CNC/PVA coating, with a thickness ranging from 5 to 6 μm and exhibiting a high degree of CNC alignment, significantly enhanced the oxygen and carbon dioxide barrier properties, surpassing PLA by several hundred-fold. Furthermore, these laminates were formed into bags, where a fruit storage test showed that PLA-CNC/PVA–PLA could extend the shelf life of fresh apple slices based on weight loss and enzymatic browning. This research showcases the potential of CNC-based coatings integrated with biodegradable polymer films to produce high-performance packaging materials, offering a promising, scalable process.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Advanced Cellulose Research Studies · Nanocomposite Films for Food Packaging · biodegradable polymer synthesis and properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Materials Engineering

Purdue University

Forest Products Laboratory, United States Department of Agriculture

Department of Mechanical Engineering

University of Delaware

Funding

U.S. Endowment for Forestry and Communities · Environmental Security Technology Certification Program · Advanced Research Projects Agency - Energy · Purdue Research Foundation · Strategic Environmental Research and Development Program

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