journal article·2025-11-20

Magnetic phase diagrams of the antiferromagnet DyB 12 with Jahn-Teller lattice instability and electron phase separation

A. N. Azarevich, A. V. Bogach, K. M. Krasikov, V. V. Voronov, S. Yu. Gavrilkin, A. Yu. Tsvetkov, S. Gabani, K. Flachbart, N. B. Bolotina, O. N. Khrykina, N. E. Sluchanko

Physical Review B· Volume 112· Issue 17
Publisher page

Abstract

The origin of charge transport and magnetization anisotropy was studied in ${\mathrm{DyB}}12$, an antiferromagnetic (AF) metal with N\'eel temperature ${T}_{\mathrm{N}}\ensuremath{\approx}16.3$ K that exhibits both small, static Jahn-Teller distortions of the fcc lattice and nanoscale electronic instabilities (dynamic charge stripes). The magnetic field (H) versus temperature (T) phase diagrams were constructed. Moreover, using the angular \ensuremath{\phi} dependences of magnetoresistance and magnetization, butterfly-type patterns of the H-\ensuremath{\phi} magnetic phase diagram in the (110) plane were created, including a number of different magnetic phases separated from each other by radial and circular boundaries. Several positive and negative contributions to magnetoresistance were separated and analyzed, providing arguments in favor of the important role of the spin density wave $5d$ component in the magnetic structure of the antiferromagnetic state. We argue that charge fluctuations in stripes are responsible for the suppression of the Ruderman-Kittel-Kasuya-Yosida indirect exchange between the nearest neighbor $\mathrm{D}{\mathrm{y}}3+$ ions located along the same $\ensuremath{\langle}110\ensuremath{\rangle}$ directions, as these dynamic charge stripes produce the magnetic phase diversity and the butterfly-type anisotropy in ${\mathrm{DyB}}12$.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Rare-earth and actinide compounds · Superconductivity in MgB2 and Alloys · Boron and Carbon Nanomaterials Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Prokhorov General Physics Institute

Lebedev Physical Institute, Russian Academy of Sciences

Institute of Experimental Physics of the Slovak Academy of Sciences

National Research Center Kurchatov Institute

Funding

Agentúra na Podporu Výskumu a Vývoja

References (34)

Show source-provided references
1. 10.1134/S106377611108010310.1134/S1063776111080103 ↗
2. 10.1016/j.jallcom.2019.15320110.1016/j.jallcom.2019.153201 ↗
3. N. E. Sluchanko · 2021
4. 10.1016/j.jssc.2003.04.00310.1016/j.jssc.2003.04.003 ↗
5. 10.1088/1361-648X/aac74210.1088/1361-648X/aac742 ↗
6. N. B. Bolotina · 2021
7. 10.1134/S002136401802002910.1134/S0021364018020029 ↗
8. 10.1088/1361-648X/aaf44e10.1088/1361-648X/aaf44e ↗
9. 10.1103/PhysRevB.99.17443010.1103/PhysRevB.99.174430 ↗
10. 10.1103/PhysRevB.102.21443510.1103/PhysRevB.102.214435 ↗
11. 10.12693/APhysPolA.137.75610.12693/APhysPolA.137.756 ↗
12. 10.1016/j.jmmm.2021.16879610.1016/j.jmmm.2021.168796 ↗
13. 10.1088/1361-648X/ac353610.1088/1361-648X/ac3536 ↗
14. 10.1016/j.jmmm.2023.17067110.1016/j.jmmm.2023.170671 ↗
15. 10.1088/0953-8984/23/6/06540310.1088/0953-8984/23/6/065403 ↗
16. 10.1016/S0921-4526(02)01644-710.1016/S0921-4526(02)01644-7 ↗
17. 10.1063/1.170303910.1063/1.1703039 ↗
18. 10.1103/PhysRevB.91.23510410.1103/PhysRevB.91.235104 ↗
19. 10.1016/j.jssc.2005.10.04610.1016/j.jssc.2005.10.046 ↗
20. 10.1038/nature0682610.1038/nature06826 ↗
21. 10.1103/PhysRevB.90.03513910.1103/PhysRevB.90.035139 ↗
22. 10.1002/1521-3951(200010)221:2%3CR7::AID-PSSB99997%3E3.0.CO;2-110.1002/1521-3951(200010)221:2%3CR7::AID-PSSB99997%3E3.0.CO;2-1 ↗
23. 10.1002/1521-3951(200212)234:3%3CR13::AID-PSSB999913%3E3.0.CO;2-O10.1002/1521-3951(200212)234:3%3CR13::AID-PSSB999913%3E3.0.CO;2-O ↗
24. 10.1103/PhysRevB.70.22441610.1103/PhysRevB.70.224416 ↗
25. 10.1007/s10909-006-9287-410.1007/s10909-006-9287-4 ↗
26. See Supplemental Material at http://link.aps.org/supplemental/10.1103/mtpb-4nk4 for Table S1: crystallographic characteristics, details of x-ray diffraction experiment with DyB12 single crystals at T=30 K and structure refinement results; Table S2: lattice parameters of DyB12 single crystal at 30 K without symmetry restrictions; maximum entropy method (MEM) description; schematic view of the RKKY oscillations of conduction electron spins and dynamic charge stripes in the fcc crystal structure of DyB12 (Fig. S1); induced magnetic anisotropy at T0=2 K (Fig. S2); temperature dependences 4πM/H(H0, T) at fixed magnetic field H0≤50kOe (Fig. S3); magnetic field dependences of resistivity derivatives dρ/dH at T0=2 K (Fig. S4); magnetic field dependences of resistivity derivatives dρ/dH at various temperatures just below TN (Fig. S5); comparison of magnetoresistance at T=2 K of DyB12 and Er11B12 for different H values and angles φ = ( n , H) in the (1-10) plane in combination with the deduced parameters AL,M and BH (Fig. S6).
27. 10.1016/j.solidstatesciences.2023.10723210.1016/j.solidstatesciences.2023.107232 ↗
28. 10.1103/PhysRevB.38.478810.1103/PhysRevB.38.4788 ↗
29. 10.1103/PhysRevB.54.1296910.1103/PhysRevB.54.12969 ↗
30. 10.1134/S106377610904015310.1134/S1063776109040153 ↗
31. 10.1103/PhysRevB.103.03511710.1103/PhysRevB.103.035117 ↗
32. N. Shitsevalova · 2022
33. 10.1134/S002136401822014910.1134/S0021364018220149 ↗
34. 10.1088/0256-307X/39/12/12730210.1088/0256-307X/39/12/127302 ↗