journal article·2023-07-28

Collective modes in the charge density wave state of K0.3MoO3 : Role of long-range Coulomb interactions revisited

Max O. Hansen, Yash Palan, Viktor Hahn, Mark D. Thomson, Konstantin Warawa, Hartmut G. Roskos, Jure Demsar, Falko Pientka, Oleksandr Tsyplyatyev, Peter Kopietz

Physical Review B· Volume 108· Issue 4
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Abstract

We re-examine the effect of long-range Coulomb interactions on the collective amplitude and phase modes in the incommensurate charge-density-wave ground state of quasi-one-dimensional conductors.Using an effective action approach we show that the longitudinal acoustic phonon protects the gapless linear dispersion of the lowest phase mode in the presence of long-range Coulomb interactions. Moreover, in Gaussian approximation, amplitude fluctuations are not affected by long-range Coulomb interactions. We also calculate the collective mode dispersions at finite temperatures and compare our results with the measured energies of amplitude and phase modes in ${\mathrm{K}}0.3{\mathrm{MoO}}3$. With the exception of the lowest phase mode, the temperature dependence of the measured mode energies can be quantitatively described within a multiphonon Fr\"ohlich model for generic electron-phonon interactions neglecting long-range Coulomb interactions.
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Research context

OpenAlex topics: Organic and Molecular Conductors Research · Electronic and Structural Properties of Oxides · Advanced Condensed Matter Physics

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