journal article·2021-09-15

Anomalous spin waves in CsFeCl3 and RbFeCl3

L. Stoppel, S. Hayashida, Z. Yan, A. Podlesnyak, A. Zheludev

Physical Review B· Volume 104· Issue 9
Publisher page

Abstract

We investigate magnetic excitations in the $S=1$ easy-plane-type triangular antiferromagnets ${\mathrm{CsFeCl}}3$ and ${\mathrm{RbFeCl}}3$ through a combination of inelastic neutron scattering measurements and spin-wave theory calculations based on an established exchange-coupling Hamiltonian. We show that in either material the model falls short of providing an adequate description of the measured intensities and for ${\mathrm{RbFeCl}}3$ even fails to reproduce the measured dispersion relation. The most striking discrepancy is a very anisotropic azimuthal intensity distribution in the acoustic spin-wave branches in the long-wavelength limit, which is incompatible with spin-wave theory on a fundamental level. The observed anomalies are attributed to long-range dipolar interactions.
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Research context

OpenAlex topics: Advanced Condensed Matter Physics · Physics of Superconductivity and Magnetism · Magnetic and transport properties of perovskites and related materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Laboratory for Solid State Physics, ETH Zürich, 8093 Zürich, Switzerland

Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA

Funding

Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung · U.S. Department of Energy · Oak Ridge National Laboratory

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