journal article·2025-10-21

Low-lying electronic structure of the rare earth based topological nodal line semimetal candidate DySbTe

Nathan Valadez, Iftakhar Bin Elius, Dante James, Peter Radanovich, Tetiana Romanova, Sami Elgalal, Grzegorz Chajewski, Florie Mesple, Ellis Thompson, Keng Tou Chu, Matthew Yankowitz, Andrzej Ptok, Dariusz Kaczorowski, Madhab Neupane

Physical Review B· Volume 112· Issue 15
Publisher page

Abstract

Lanthanide ($Ln$) based $Ln\mathrm{SbTe}$ materials have garnered significant attention due to the rich interplay of long-range magnetic ordering and topological properties, driven by unique crystalline symmetry, $4f$ electron interactions, and pronounced spin-orbit coupling (SOC) effects. DySbTe, as a heavier lanthanide based member of the $Ln\mathrm{SbTe}$ family, stands out with its SOC and larger on-site interactions on its $4f$ electrons, which arise due to the heavier Dy element. Here, we present a comprehensive study on the low-temperature bulk physical properties and the electronic structure of DySbTe using magnetic susceptibility, heat capacity, and electrical resistivity measurements, along with high-resolution angle-resolved photoemission spectroscopy (ARPES), scanning tunneling microscopy and spectroscopy (STM/S), and density functional theory calculations. Our thermodynamic measurements revealed an antiferromagnetic ordering below ${T}_{\mathrm{N}}=7.45$ K and a subsequent magnetic phase transition at ${T}_{\mathrm{N}1}=7.15$ K. Our transport studies indicate a semimetallic behavior with unusual feature in the ordered state. Our ARPES measurements revealed a diamond-shaped Fermi pocket centered at the $\overline{\mathrm{\ensuremath{\Gamma}}}$ point, with band features that evolve distinctly across various binding energies. STM/S results indicate a minimum in the density of states at around 100 meV below the Fermi level, and ARPES measurements reveal a significant gap present around the $\overline{\mathrm{X}}$ point, differentiating DySbTe from other $Ln\mathrm{SbTe}$ compounds. These findings enhance our understanding of the SOC effects on the electronic structure and topological properties in the $Ln\mathrm{SbTe}$ family, highlighting DySbTe as a promising candidate for exploring the interplay between topology and magnetism.
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Research context

OpenAlex topics: Topological Materials and Phenomena · Advanced Semiconductor Detectors and Materials · 2D Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

University of Central Florida

Polish Academy of Sciences

University of Washington

Funding

National Science Foundation · Narodowe Centrum Nauki · U.S. Department of Energy

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