journal article·2024-02-05

Mass imbalance and electron-phonon correlation impact on the excitonic insulator state in semimetal/semiconducting materials

Thi-Hong-Hai Do, Thi-Hau Nguyen, Van-Nham Phan

Physical Review B· Volume 109· Issue 8
Publisher page

Abstract

Signatures of the excitonic insulator in the mass-imbalance extended Falicov-Kimball model with the electron-phonon correlation are investigated. Based on the unrestricted Hartree-Fock approximation, we derive a set of self-consistent equations specifying the excitonic insulator order parameter and then construct the complex phase diagram of the excitonic insulator states. For a given intermediate Coulomb interaction, the excitonic insulator states at nearly zero temperature are found if the electronic hybridization-phonon coupling is sufficiently large. The window of the excitonic insulator states expands as suppression of the mass anisotropy. The influence of the mass imbalance and electron-phonon correlations on the nature of the BCS-BEC crossover of the condensation states is also addressed in the signatures of the optical conductivity. The preformed excitonic bound states in the normal semiconducting side are inspected in the features of the imaginary part of the dynamical excitonic susceptibility function. By increasing the electronic hybridization-phonon coupling or suppressing the mass imbalance, we find the dominance of the excitonic coherent bound states. The compact influence of the mass imbalance and electron-phonon correlations on the whole picture of the excitonic insulator state thus has been discussed.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Organic and Molecular Conductors Research · Quantum and electron transport phenomena

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, Hanoi University of Mining and Geology, Duc Thang, Bac Tu Liem, Hanoi 10072, Vietnam

Faculty of Physics, Graduate University of Science and Technology, Vietnam Academy of Science and Technology, Hanoi 10072, Vietnam

Institute of Research and Development, Duy Tan University, 3-Quang Trung, Danang 550000, Vietnam

Faculty of Natural Sciences, Duy Tan University, 3-Quang Trung, Danang 550000, Vietnam

Funding

Hanoi University of Mining and Geology

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